Selective recovery of critical materials in zero-liquid discharge supercritical water desalination

Yoon, Tae-Jun; Sharan, Prashant; Craddock, Erica Powers; Lewis, Jeremy Charles; Matteson, John Anthony; Seong, Jong Geun; Singh, Rajinder Pal; Maerzke, Katie A.; Currier, Robert Patrick; Findikoglu, Alp Tugrul

doi:10.1016/j.desal.2022.115849

Selective recovery of critical materials in zero-liquid discharge supercritical water desalination

Journal Article · Wed May 25 00:00:00 EDT 2022 · Desalination

DOI:https://doi.org/10.1016/j.desal.2022.115849· OSTI ID:2282535

^[1]; Sharan, Prashant ^[2]; Craddock, Erica Powers ^[2]; Lewis, Jeremy Charles ^[2]; ^[2]; ^[2]; ^[2]; ^[2]; ^[2]; ^[2]

Los Alamos National Laboratory (LANL), Los Alamos, NM (United States); Chungnam National Univ., Daejeon (Korea, Republic of)
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Zero-liquid discharge desalination techniques are being actively studied as alternative means to produce drinkable water and recover valuable resources without polluting the environment. Supercritical water desalination is one of such alternatives that can overcome the technical and environmental challenges in standard desalination techniques. In addition to these attractive features, this work explores the possibility of utilizing supercritical water desalination for the selective recovery of strategic (critical) materials as co-products. Here, to validate the technical and economic feasibility of the process, we prepared model brine solutions that consist of sodium, neodymium, and different anions and conducted a series of desalination experiments. The results were analyzed experimentally and theoretically and were utilized to evaluate the economic feasibility of the process. When a few tens or hundreds of parts-per-million critical materials are dissolved in the feed, the proposed method becomes more cost-effective in producing critical materials than existing technologies. In addition, it does not discharge any concentrated contaminants while producing drinkable water. These results suggest that supercritical water desalination can recover critical materials while producing freshwater in an economically feasible fashion.

View Accepted Manuscript (DOE)

Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE; USDOE Laboratory Directed Research and Development (LDRD) Program; USDOE National Nuclear Security Administration (NNSA)

Grant/Contract Number:: 89233218CNA000001

OSTI ID:: 2282535

Alternate ID(s):: OSTI ID: 1960604

Report Number(s):: LA-UR--21-30241

Journal Information:: Desalination, Journal Name: Desalination Vol. 537; ISSN 0011-9164

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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Selective recovery of critical materials in zero-liquid discharge supercritical water desalination

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