Charged Hole‐Transporting Materials Based on Imidazolium for Defect Passivation in Inverted Perovskite Solar Cells

Tingare, Yogesh S.; Li, Meng‐Che; Teng, Sheng‐Hung; Lin, Ja‐Hon; Su, Chaochin; Lin, Shan‐Jung; Lew, Xin‐Rui; Tsai, Hsinhan; Ghosh, Dibyajyoti; Nie, Wanyi; Yeh, Bao‐Lin; Li, Wen‐Ren

doi:10.1002/solr.202300817

Charged Hole‐Transporting Materials Based on Imidazolium for Defect Passivation in Inverted Perovskite Solar Cells

Journal Article · Wed Dec 27 23:00:00 EST 2023 · Solar RRL

DOI:https://doi.org/10.1002/solr.202300817· OSTI ID:2274846

^[1]; Li, Meng‐Che ^[1]; Teng, Sheng‐Hung ^[2]; Lin, Ja‐Hon ^[3]; ^[1]; Lin, Shan‐Jung ^[2]; Lew, Xin‐Rui ^[2]; ^[4]; ^[5]; ^[6]; Yeh, Bao‐Lin ^[2]; ^[2]

Institute of Organic and Polymeric Materials/Research and Development Center for Smart Textile Technology National Taipei University of Technology Taipei 106344 Taiwan
Department of Chemistry National Central University Zhongli 32001 Taiwan
Department of Electro‐Optical Engineering National Taipei University of Technology Taipei 106344 Taiwan
Center for Integrated Nanotechnologies, Materials Physics and Application Division Los Alamos National Laboratory Los Alamos 87545 NM USA, Department of Chemistry University of California, Berkeley Berkeley 94720 CA USA
Department of Chemistry and Department of Materials Science and Engineering (DMSE) Indian Institute of Technology, Delhi Hauz Khas New Delhi 110016 India
Center for Integrated Nanotechnologies, Materials Physics and Application Division Los Alamos National Laboratory Los Alamos 87545 NM USA, Department of Physics University at Buffalo, The State University of New York Buffalo 14260 NY USA

The hole‐transporting material (HTM) in perovskite solar cells (PSCs) provides an ideal interface with the perovskite layer for hole collection while influencing the perovskite crystalline structure and morphology. This article presents SIM and DIM, two new dopant‐free imidazolium‐based HTMs with charged units accompanied by counter ions that show the potential to function as ionic HTMs and ionic liquid additives and help improve the efficiency and stability of inverted PSCs. DIM‐based PSCs demonstrates exceptional performance with a high‐power conversion efficiency of 19.15%, attributed to improved passivation of perovskite interface defects. Furthermore, these new imidazolium salt‐based HTMs can be manufactured economically, making them a viable option for mass production and PSC commercialization.

View Accepted Manuscript (Publisher)

Sponsoring Organization:: USDOE

Grant/Contract Number:: NONE; 89233218CNA000001

OSTI ID:: 2274846

Journal Information:: Solar RRL, Journal Name: Solar RRL Journal Issue: 3 Vol. 8; ISSN 2367-198X

Publisher:: Wiley Blackwell (John Wiley & Sons)Copyright Statement

Country of Publication:: Germany

Language:: English

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