skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Supercontinuum Fourier transform spectrometry with balanced detection on a single photodiode

Journal Article · · Journal of Chemical Physics
DOI:https://doi.org/10.1063/1.4961655· OSTI ID:22678899

We demonstrate a method of combining a supercontinuum light source with a commercial Fourier transform spectrometer, using a novel approach to dual-beam balanced detection, implemented with phase-sensitive detection on a single light detector. A 40 dB reduction in the relative intensity noise is achieved for broadband light, analogous to conventional balanced detection methods using two matched photodetectors. Unlike conventional balanced detection, however, this method exploits the time structure of the broadband source to interleave signal and reference pulse trains in the time domain, recording the broadband differential signal at the fundamental pulse repetition frequency of the supercontinuum. The method is capable of real-time correction for instability in the supercontinuum spectral structure over a broad range of wavelengths and is compatible with commercially designed spectrometers. A proof-of-principle experimental setup is demonstrated for weak absorption in the 1500-1600 nm region.

OSTI ID:
22678899
Journal Information:
Journal of Chemical Physics, Vol. 145, Issue 8; Other Information: (c) 2016 Author(s); Country of input: International Atomic Energy Agency (IAEA); ISSN 0021-9606
Country of Publication:
United States
Language:
English

References (17)

Building Electro‐Optical Systems: Making It All Work journal January 2000
Cavity-enhanced optical frequency comb spectroscopy in the mid-infrared application to trace detection of hydrogen peroxide journal May 2012
A dual-beam infrared interferometer-spectrometer journal June 1967
Dual-beam Fourier transform infrared spectrometer journal March 1978
Fourier transform spectroscopy with a laser frequency comb journal January 2009
Real‐time sampling electronics for double modulation experiments with Fourier transform infrared spectrometers journal June 1991
Balanced detection for interferometry with a noisy source journal June 2012
Fundamental Noise Limitations to Supercontinuum Generation in Microstructure Fiber journal March 2003
Broadband laser enhanced dual-beam interferometry journal January 2012
Vibrational Circular Dichroism in General Anisotropic Thin Solid Films: Measurement and Theoretical Approach journal June 2005
Fourier Transform Spectrometry with a Near-Infrared Supercontinuum Source journal May 2009
The Implications of Fluctuation Noise in Multiplex Spectroscopy journal March 1976
Improved Sensitivity in Dual-Beam Fourier Transform Infrared Spectroscopy journal January 1980
Polarization Modulation FT-IR Spectroscopy of Surfaces and Ultra-Thin Films: Experimental Procedure and Quantitative Analysis journal March 1991
Direct Phase Correction of Differential FT-IR Spectra journal July 1998
Building Electro‐Optical Systems: Making it all Work book January 2008
Fundamental noise limitations to supercontinuum generation in microstructure fiber text January 2002

Cited By (3)

Baseline-free quantitative absorption spectroscopy based on cepstral analysis journal January 2019
Background-free broadband absorption spectroscopy based on interferometric suppression with a sign-inverted waveform journal January 2019
Baseline-free Quantitative Absorption Spectroscopy Based on Cepstral Analysis text January 2019

Similar Records

Supercontinuum Fourier transform spectrometry with balanced detection on a single photodiode
Journal Article · Thu Aug 25 00:00:00 EDT 2016 · Journal of Chemical Physics · OSTI ID:22678899

Thomson scattering calibration with ultrabright supercontinuum light source
Journal Article · Sun Oct 15 00:00:00 EDT 2006 · Review of Scientific Instruments · OSTI ID:22678899

Breaking Barriers in Ultrafast Spectroscopy and Imaging Using 100 kHz Amplified Yb-Laser Systems
Journal Article · Mon Jul 10 00:00:00 EDT 2023 · Accounts of Chemical Research · OSTI ID:22678899