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Title: Single-shot mega-electronvolt ultrafast electron diffraction for structure dynamic studies of warm dense matter

Journal Article · · Review of Scientific Instruments
DOI:https://doi.org/10.1063/1.4960070· OSTI ID:22596532
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  1. SLAC National Accelerator Laboratory, 2575 Sand Hill Road, Menlo Park, California 94025 (United States)
  2. Faculty of Physics and Centre for Nanointegration Duisburg-Essen, University of Duisburg-Essen, Lotharstrasse 1, D-47048 Duisburg (Germany)

We have developed a single-shot mega-electronvolt ultrafast-electron-diffraction system to measure the structural dynamics of warm dense matter. The electron probe in this system is featured by a kinetic energy of 3.2 MeV and a total charge of 20 fC, with the FWHM pulse duration and spot size at sample of 350 fs and 120 μm respectively. We demonstrate its unique capability by visualizing the atomic structural changes of warm dense gold formed from a laser-excited 35-nm freestanding single-crystal gold foil. The temporal evolution of the Bragg peak intensity and of the liquid signal during solid-liquid phase transition are quantitatively determined. This experimental capability opens up an exciting opportunity to unravel the atomic dynamics of structural phase transitions in warm dense matter regime.

OSTI ID:
22596532
Journal Information:
Review of Scientific Instruments, Vol. 87, Issue 11; Other Information: (c) 2016 Author(s); Country of input: International Atomic Energy Agency (IAEA); ISSN 0034-6748
Country of Publication:
United States
Language:
English

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Heterogeneous to homogeneous melting transition visualized with ultrafast electron diffraction journal June 2018
A compact tunable quadrupole lens for brighter and sharper ultra-fast electron diffraction imaging journal March 2019