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Title: Frequency and field dependent dynamic properties of CoFe{sub 2−x}Al{sub x}O{sub 4} ferrite nanoparticles

Journal Article · · Materials Research Bulletin
 [1]; ; ;  [2];  [3];  [4]
  1. Special Centre for Nanoscience, Jawaharlal Nehru University, New Mehrauli Road, New Delhi 110067 (India)
  2. The department of Physics and materials Science, The University of Memphis, Memphis, TN 38152 (United States)
  3. Seagate Technology, 7801 Computer Ave., Bloomington, MN 55435 (United States)
  4. Department of Physics, University of Colorado, 1420 Austin Bluffs Parkway, Colorado Springs, CO 80918 (United States)

Highlights: “CoFe{sub 2−x} Al{sub x}O{sub 4} ferrite nanoparticles: Static and dynamic properties” • Grain size reduction with Al{sup 3+} content. • Reduction in Ms, Hc, with increasing Al{sup 3+} content. • Increase in resonance frequency with applied field. • Decrease in resonance field with increase in Al{sup 3+} content. • Decrease in Gilbert parameter with increase in Al{sup 3+} content. - Abstract: Aluminum doped CoFe{sub 2−x}Al{sub x}O{sub 4} (0 ≤ x ≤ 0.9) nanoparticles were synthesized via auto-combustion. Formation of single phase cubic spinel structure was confirmed by X-ray diffraction (XRD) analysis. XRD analysis suggests a linear decrease in lattice cell parameters and grain size (90–55 nm) with the increase in Al{sup 3+} content. The saturation magnetization of samples decrease with increasing Al{sup 3+} content due to magnetic dilution effect. A concomitant linear reduction in coercivity was also observed mainly due to decrease in magnetic anisotropy. Frequency and field dependent dynamic properties of nanoparticles were studied by ferromagnetic resonance (FMR) technique. The resonance frequency increases linearly with magnetic field for all nanoparticles. Magnetic field dependent experimental absorption data (S{sub 21} vs. frequency) were compared with effective medium theory considering an effective demagnetization field and was observed to be in good agreement with each other. High Al{sup 3+} content reduces the Gilbert damping parameter thus making CoFe{sub 2−x}Al{sub x}O{sub 4} as an attractive material for high frequency applications.

OSTI ID:
22581481
Journal Information:
Materials Research Bulletin, Vol. 76; Other Information: Copyright (c) 2015 Elsevier Science B.V., Amsterdam, The Netherlands, All rights reserved.; Country of input: International Atomic Energy Agency (IAEA); ISSN 0025-5408
Country of Publication:
United States
Language:
English