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Mesoscale evolution of voids and microstructural changes in HMX-based explosives during heating through the β-δ phase transition

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/1.4927614· OSTI ID:22494715
; ; ; ; ; ;  [1];  [2]
  1. Lawrence Livermore National Laboratory, Livermore, California 94550 (United States)
  2. Argonne National Laboratory, Argonne, Illinois 60439 (United States)

HMX-based explosives LX-10 and PBX-9501 were heated through the β-δ phase transition. Ultra-small angle x-ray scattering (USAXS) and molecular diffraction were simultaneously recorded as the HMX was heated. Mesoscale voids and structure dramatically change promptly with the β-δ phase transition, rather than with other thermal effects. Also, x-ray induced damage, observed in the USAXS, occurs more readily at elevated temperatures; as such, the dose was reduced to mitigate this effect. Optical microscopy performed during a similar heating cycle gives an indication of changes on longer length scales, while x-ray microtomography, performed before and after heating, shows the character of extensive microstructural damage resulting from the temperature cycle and solid-state phase transition.

OSTI ID:
22494715
Journal Information:
Journal of Applied Physics, Journal Name: Journal of Applied Physics Journal Issue: 5 Vol. 118; ISSN JAPIAU; ISSN 0021-8979
Country of Publication:
United States
Language:
English

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Core-Shell Structured HMX@Polydopamine Energetic Microspheres: Synergistically Enhanced Mechanical, Thermal, and Safety Performances journal March 2019
Microscale Electromagnetic Heating in Heterogeneous Energetic Materials Based on X-ray Computed Tomography journal April 2016
The Thermal and Microstructural Effect of Plasticizing HMX-Nitrocellulose Composites journal March 2017