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Title: LaTiO{sub 3}/KTaO{sub 3} interfaces: A new two-dimensional electron gas system

Journal Article · · APL materials
DOI:https://doi.org/10.1063/1.4914310· OSTI ID:22415259
; ; ;  [1]; ;  [2];  [2]
  1. Department of Applied Physics and Center for Research on Interface Structures and Phenomena (CRISP), Yale University, New Haven, Connecticut 06520 (United States)
  2. Brookhaven National Laboratory, Center for Functional Nanomaterials, Upton, New York 11973 (United States)

We report a new 2D electron gas (2DEG) system at the interface between a Mott insulator, LaTiO{sub 3}, and a band insulator, KTaO{sub 3}. For LaTiO{sub 3}/KTaO{sub 3} interfaces, we observe metallic conduction from 2 K to 300 K. One serious technological limitation of SrTiO{sub 3}-based conducting oxide interfaces for electronics applications is the relatively low carrier mobility (0.5-10 cm{sup 2}/V s) of SrTiO{sub 3} at room temperature. By using KTaO{sub 3}, we achieve mobilities in LaTiO{sub 3}/KTaO{sub 3} interfaces as high as 21 cm{sup 2}/V s at room temperature, over a factor of 3 higher than observed in doped bulk SrTiO{sub 3}. By density functional theory, we attribute the higher mobility in KTaO{sub 3} 2DEGs to the smaller effective mass for electrons in KTaO{sub 3}.

OSTI ID:
22415259
Journal Information:
APL materials, Vol. 3, Issue 3; Other Information: (c) 2015 Author(s); Country of input: International Atomic Energy Agency (IAEA); ISSN 2166-532X
Country of Publication:
United States
Language:
English

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Conducting LaVO 3 /SrTiO 3 Interface: Is Cationic Stoichiometry Mandatory? journal November 2019
Band Structure and Spin–Orbital Texture of the (111)‐KTaO 3 2D Electron Gas journal March 2019
Strain-driven carrier-type switching of surface two-dimensional electron and hole gases in a KTaO 3 thin film journal January 2018
First-principles studies of a two-dimensional electron gas at the interface of polar/polar LaAlO 3 /KNbO 3 superlattices journal January 2019
Design of two-dimensional electron gas systems via polarization discontinuity from large-scale first-principles calculations journal January 2018
Research Update: Conductivity and beyond at the LaAlO 3 /SrTiO 3 interface journal June 2016
Scavenging of oxygen from SrTiO 3 during oxide thin film deposition and the formation of interfacial 2DEGs journal March 2017
Effect of SrTiO 3 oxygen vacancies on the conductivity of LaTiO 3 /SrTiO 3 heterostructures journal November 2018
A universal method to fabricate p-n or Schottky heterojunctions based on two-dimensional electron gas journal December 2019
Molecular dynamics simulations of the response of pre-damaged SrTiO 3 and KTaO 3 to fast heavy ions journal January 2020
Electron mobility in oxide heterostructures journal June 2018
Local structure and defects in ion irradiated KTaO 3 journal March 2018
The effect of fabrication conditions on 2DEGs transport characteristics at amorphous-LaAlO 3 /KTaO 3 interfaces journal May 2019
Band Structure and Spin–Orbital Texture of the $(111)‐KTaO_{3}$ 2D Electron Gas text January 2019