Tracer exchange and catalytic reaction in single-file systems
- Universitaet Leipzig (Germany)
Using a simple jump model of diffusion, Monte Carlo simulations are applied to determine the rate of tracer exchange and the effectiveness factor of chemical reactions in single-file systems. The influence of the characteristic parameters such as the file length, the jump rates, and the reaction rate are investigated. Particular consideration was dedicated to the temperature dependence of the output rate of the chemical reaction. The simulations are compared with the experimentally observed reaction behavior in zeolite L as described in the literature. 18 refs., 9 figs.
- OSTI ID:
- 224036
- Journal Information:
- Journal of Catalysis, Journal Name: Journal of Catalysis Journal Issue: 2 Vol. 157; ISSN 0021-9517; ISSN JCTLA5
- Country of Publication:
- United States
- Language:
- English
Similar Records
Single-file diffusion and reaction in zeolites
Tracer diffusion in concentrated lattice gas models. Rectangular lattices with anisotropic jump rates
Monte Carlo simulations of diffusion in zeolites and comparison with the generalized Maxwell-Stefan theory
Journal Article
·
Sat Aug 01 00:00:00 EDT 1992
· Journal of Catalysis; (United States)
·
OSTI ID:6999219
Tracer diffusion in concentrated lattice gas models. Rectangular lattices with anisotropic jump rates
Journal Article
·
Mon Nov 30 23:00:00 EST 1987
· J. Stat. Phys.; (United States)
·
OSTI ID:5371557
Monte Carlo simulations of diffusion in zeolites and comparison with the generalized Maxwell-Stefan theory
Journal Article
·
Sat Aug 01 00:00:00 EDT 1992
· Journal of Catalysis; (United States)
·
OSTI ID:7241508