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Hydroformylation of 1-octene in the presence of cobalt alkylidynecarbonyl clusters

Journal Article · · Russian Chemical Bulletin
OSTI ID:223931
; ;  [1]
  1. Scientific Research and Design Inst. of Monomers, Tula (Russian Federation); and others

The hydroformylation of 1-octene in the presence of Co{sub 3}(CO){sub 9}({mu}-CR) (R = H, Me, Ph, CO{sub 2}Me, CO{sub 2}Et, CO{sub 2}Pr{sup i}, CO{sub 2}Bu{sup t}, Cl, Br, OMe) alkylidynecarbonyl clusters, as well as triphenylphosphine derivatives of these complexes and heteronuclear Co{sub 2}Ni compounds have been studied. The nature of the catalytically active species in hydroformylation, as well as the processes of their formation and transformation during the reaction, have been established by means of IR spectroscopy, The effects of the reaction conditions, the nature of the substituent at the apical carbon atom, the electron donating phosphine substituent, and the substituent in the metal cluster framework have been discussed.

OSTI ID:
223931
Journal Information:
Russian Chemical Bulletin, Journal Name: Russian Chemical Bulletin Journal Issue: 8 Vol. 42; ISSN 1066-5285; ISSN RCBUEY
Country of Publication:
United States
Language:
English

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