skip to main content
OSTI.GOV title logo U.S. Department of Energy
Office of Scientific and Technical Information

Title: Thermal conductivity of bulk nanostructured lead telluride

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.4862323· OSTI ID:22275721
 [1];  [2];  [1]
  1. Department of Mechanical Engineering, The University of Tokyo, Bunkyo, Tokyo 113-8656 (Japan)
  2. Department of Mechanical Engineering, Massachusetts Institute of Technology, Cambridge, Massachusetts 02139 (United States)

Thermal conductivity of lead telluride with embedded nanoinclusions was studied using Monte Carlo simulations with intrinsic phonon transport properties obtained from first-principles-based lattice dynamics. The nanoinclusion/matrix interfaces were set to completely reflect phonons to model the maximum interface-phonon-scattering scenario. The simulations with the geometrical cross section and volume fraction of the nanoinclusions matched to those of the experiment show that the experiment has already reached the theoretical limit of thermal conductivity. The frequency-dependent analysis further identifies that the thermal conductivity reduction is dominantly attributed to scattering of low frequency phonons and demonstrates mutual adaptability of nanostructuring and local disordering.

OSTI ID:
22275721
Journal Information:
Applied Physics Letters, Vol. 104, Issue 2; Other Information: (c) 2014 AIP Publishing LLC; Country of input: International Atomic Energy Agency (IAEA); ISSN 0003-6951
Country of Publication:
United States
Language:
English

Cited By (2)

Effective phonon mean free path in polycrystalline nanostructures journal April 2015
Research Update: Phonon engineering of nanocrystalline silicon thermoelectrics journal September 2016