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Title: Femtosecond diffraction dynamics of laser-induced periodic surface structures on fused silica

Journal Article · · Applied Physics Letters
DOI:https://doi.org/10.1063/1.4790284· OSTI ID:22162732
;  [1]; ;  [2]
  1. Max-Born-Institut fuer Nichtlineare Optik und Kurzzeitspektroskopie (MBI), Max-Born-Strasse 2A, D-12489 Berlin (Germany)
  2. BAM Bundesanstalt fuer Materialforschung und - pruefung, Unter den Eichen 87, D-12205 Berlin (Germany)

The formation of laser-induced periodic surface structures (LIPSS) on fused silica upon irradiation with linearly polarized fs-laser pulses (50 fs pulse duration, 800 nm center wavelength) is studied experimentally using a transillumination femtosecond time-resolved (0.1 ps-1 ns) pump-probe diffraction approach. This allows to reveal the generation dynamics of near-wavelength-sized LIPSS showing a transient diffraction at specific spatial frequencies even before a corresponding permanent surface relief was observed. The results confirm that the ultrafast energy deposition to the materials surface plays a key role and triggers subsequent physical mechanisms such as carrier scattering into self-trapped excitons.

OSTI ID:
22162732
Journal Information:
Applied Physics Letters, Vol. 102, Issue 5; Other Information: (c) 2013 American Institute of Physics; Country of input: International Atomic Energy Agency (IAEA); ISSN 0003-6951
Country of Publication:
United States
Language:
English