A comprehensive review on regeneration strategies for direct air capture

An, Keju; Li, Kai; Yang, Cheng-Min; Brechtl, Jamieson M.; Nawaz, Kashif

doi:10.1016/j.jcou.2023.102587

A comprehensive review on regeneration strategies for direct air capture

Journal Article · Wed Sep 27 00:00:00 EDT 2023 · Journal of CO2 Utilization

DOI:https://doi.org/10.1016/j.jcou.2023.102587· OSTI ID:2203824

^[1]; Li, Kai ^[1]; Yang, Cheng-Min ^[1]; Brechtl, Jamieson M. ^[1]; ^[1]

Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Direct air capture (DAC), which removes CO₂ directly from ambient air, is a critical negative emission technology for mitigating global climate change. Efficiency and the source of energy are crucial considerations for DAC to enable negative emissions. Substantial technological progress has been made in DAC technologies, and promising opportunities exist for commercial-scale deployments. However, DAC technologies require high regeneration energy to release CO₂ from sorbents. Various approaches have been tested and optimized for different DAC systems. This review demonstrates that the work equivalent regeneration energy demand (supported by either the electric grid or fossil fuel combustion) ranges from 0.5–18.75 GJ/t-CO₂ for solid sorbent DAC systems and 0.62–17.28 GJ/t-CO₂ for liquid solvent DAC systems. The regeneration process is the energy-demanding process in DAC that is a key step for efficient operation. Potential methods to lower the regeneration energy demand include microwave, ultrasound, magnetic particle heating, and electric swing. Although the potential methods to date are still at the lab scale, significant work is being done to optimize DAC system processes.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Laboratory Directed Research and Development (LDRD) Program; USDOE Office of Energy Efficiency and Renewable Energy (EERE), Energy Efficiency Office. Building Technologies Office; USDOE Office of Fossil Energy and Carbon Management (FECM)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 2203824

Journal Information:: Journal of CO2 Utilization, Journal Name: Journal of CO2 Utilization Vol. 76; ISSN 2212-9820

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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