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Pathway of D{sup +} in sequential double ionization of D{sub 2} in an intense laser pulse

Journal Article · · Physical Review. A
;  [1]
  1. Laser-Plasma Research Institute, Shahid Beheshti University, G. C., Evin, Tehran 19839-63113 (Iran, Islamic Republic of)
Details of the pathway for the dissociative ionization process of the ground electronic state of aligned D{sub 2}{sup +} produced from the first ionization of D{sub 2} in a short ({approx}100 fs) and intense (4.0x10{sup 14} W cm{sup -2}) 480 nm laser pulse are analyzed and visualized. The initial vibrational state of D{sub 2}{sup +} comes from the vertical transformation of the ground state of D{sub 2}. The initial wave packet in the ground electronic state of D{sub 2}{sup +} is outgoing through a dissociation-ionization channel accompanied by a strong coupling between the 1s{sigma}{sub g} and 2p{sigma}{sub u} electronic states. We show explicitly that the transition from the coupling states 1s{sigma}{sub g} and 2p{sigma}{sub u} to the ionization state is not a direct transition, but takes place through other intermediate states having some dissociative energy that results in a relatively wide internuclear distribution of the ionization state.
OSTI ID:
21408845
Journal Information:
Physical Review. A, Journal Name: Physical Review. A Journal Issue: 5 Vol. 81; ISSN 1050-2947; ISSN PLRAAN
Country of Publication:
United States
Language:
English