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Title: Determining X-Ray Nonlinear Susceptibility of Diamond by the Optical Fano Effect

Journal Article · · Physical Review Letters
 [1]; ;  [1]
  1. RIKEN SPring-8 Center, 1-1-1 Kouto, Sayo-cho, Sayo-gun, Hyogo 679-5148 Japan (Japan)

X-ray nonlinear optics, which has been considered as a scientific frontier to be explored with x-ray free-electron lasers, is accessible with existing synchrotron x-ray sources, revealing its unique features. We demonstrate that x-ray parametric down-conversion is observed indirectly through quantum mechanical interference known as the Fano effect. By introducing a novel concept of photonic discrete levels, we determine the second order nonlinear susceptibility of diamond, and find a strong resonance enhancement at the core absorption edge that presents firm experimental evidence to develop x-ray nonlinear optics.

OSTI ID:
21370912
Journal Information:
Physical Review Letters, Vol. 103, Issue 25; Other Information: DOI: 10.1103/PhysRevLett.103.254801; (c) 2009 The American Physical Society; ISSN 0031-9007
Country of Publication:
United States
Language:
English