Turbulence and combustion interaction: High resolution local flame front structure visualization using simultaneous single-shot PLIF imaging of CH, OH, and CH{sub 2}O in a piloted premixed jet flame

Journal Article · Tue Jun 15 04:00:00 EDT 2010 · Combustion and Flame

DOI:https://doi.org/10.1016/J.COMBUSTFLAME.2010.02.017· OSTI ID:21318359

Li, Z S; Li, B; Sun, Z W; Alden, M ^[1]; Bai, X S ^[2]

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1. Division of Combustion Physics, Lund University, P.O. Box 118, S-221 00 Lund (Sweden)
2. Division of Fluid Mechanics, Lund University, P.O. Box 118, S-221 00 Lund (Sweden)

High resolution planar laser-induced fluorescence (PLIF) was applied to investigate the local flame front structures of turbulent premixed methane/air jet flames in order to reveal details about turbulence and flame interaction. The targeted turbulent flames were generated on a specially designed coaxial jet burner, in which low speed stoichiometric gas mixture was fed through the outer large tube to provide a laminar pilot flame for stabilization of the high speed jet flame issued through the small inner tube. By varying the inner tube flow speed and keeping the mixture composition as that of the outer tube, different flames were obtained covering both the laminar and turbulent flame regimes with different turbulent intensities. Simultaneous CH/CH{sub 2}O, and also OH PLIF images were recorded to characterize the influence of turbulence eddies on the reaction zone structure, with a spatial resolution of about 40 {mu}m and temporal resolution of around 10 ns. Under all experimental conditions, the CH radicals were found to exist only in a thin layer; the CH{sub 2}O were found in the inner flame whereas the OH radicals were seen in the outer flame with the thin CH layer separating the OH and CH{sub 2}O layers. The outer OH layer is thick and it corresponds to the oxidation zone and post-flame zone; the CH{sub 2}O layer is thin in laminar flows; it becomes broad at high speed turbulent flow conditions. This phenomenon was analyzed using chemical kinetic calculations and eddy/flame interaction theory. It appears that under high turbulence intensity conditions, the small eddies in the preheat zone can transport species such as CH{sub 2}O from the reaction zones to the preheat zone. The CH{sub 2}O species are not consumed in the preheat zone due to the absence of H, O, and OH radicals by which CH{sub 2}O is to be oxidized. The CH radicals cannot exist in the preheat zone due to the rapid reactions of this species with O{sub 2} and CO{sub 2} in the inner-layer of the reaction zones. The local PLIF intensities were evaluated using an area integrated PLIF signal. Substantial increase of the CH{sub 2}O signal and decrease of CH signal was observed as the jet velocity increases. These observations raise new challenges to the current flamelet type models. (author)

• OSTI ID: 21318359
• Journal Information: Combustion and Flame, Journal Name: Combustion and Flame Journal Issue: 6 Vol. 157; ISSN CBFMAO; ISSN 0010-2180
• Country of Publication: United States
• Language: English

Related Subjects

37 INORGANIC, ORGANIC, PHYSICAL, AND ANALYTICAL CHEMISTRY
AIR
CARBON DIOXIDE
COMBUSTION
COMBUSTION KINETICS
FORMALDEHYDE
Flame broadening
HYDROXYL RADICALS
JETS
Jet flames
LAMINAR FLAMES
LAMINAR FLOW
LAYERS
METHANE
MIXTURES
SPATIAL RESOLUTION
STOICHIOMETRY
THIN FILMS
TIME RESOLUTION
TUBES
TURBULENCE
TURBULENT FLOW
Turbulence flame interaction
ZONES