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Study of the structure of PyHReO{sub 4} under high pressure

Journal Article · · Crystallography Reports
 [1]; ;  [2];  [3];  [2];  [1];  [4]
  1. Joint Institute for Nuclear Research (Russian Federation)
  2. Mickiewicz University (Poland)
  3. Russian Research Centre 'Kurchatov Institute' (Russian Federation)
  4. HASYLAB am DESY (Germany)

The structure of deuterated pyridinium perrhenate (d{sub 5}PyH)ReO{sub 4} (C{sub 5}D{sub 5}NHReO{sub 4}) is studied by X-ray diffraction at room temperature and pressures up to 3.5 GPa and by neutron diffraction in the temperature range 10-293 K and at pressures up to 2.0 GPa. Under normal conditions, this compound belongs to the orthorhombic space group Cmc2{sub 1} (ferroelectric phase II). At room temperature and pressures above P > 0.7 GPa, a transition to an orthorhombic phase (paraelectric phase II) is observed. This paraelectric phase is described by the space group Cmcm. At a pressure as high as P = 2.0 GPa, phase I remains stable at temperatures down to 10 K. This fact indicates that the high pressure suppresses the ferroelectric state in deuterated pyridinium perrhenate (d{sub 5}PyH)ReO{sub 4}.

OSTI ID:
21090918
Journal Information:
Crystallography Reports, Journal Name: Crystallography Reports Journal Issue: 3 Vol. 52; ISSN 1063-7745; ISSN CYSTE3
Country of Publication:
United States
Language:
English

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