Complete Characterization of Molecular Dynamics in Ultrashort Laser Fields
Journal Article
·
· Physical Review Letters
- Max-Planck-Institut fuer Kernphysik, D-69029 Heidelberg (Germany)
Reaction Microscope-based, complete, and time-resolved Coulomb explosion imaging of vibrating and dissociating D{sub 2}{sup +} molecules with femtosecond time-resolution allowed us to perform an internuclear distance (R-)dependent Fourier analysis of the corresponding wave packets. Calculations demonstrate that the obtained two-dimensional R-dependent frequency spectra enable the complete characterization of the wave packet dynamics and directly visualize the field-modified molecular potential curves in intense, ultrashort laser pulses.
- OSTI ID:
- 21024261
- Journal Information:
- Physical Review Letters, Journal Name: Physical Review Letters Journal Issue: 15 Vol. 99; ISSN 0031-9007; ISSN PRLTAO
- Country of Publication:
- United States
- Language:
- English
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Related Subjects
74 ATOMIC AND MOLECULAR PHYSICS
CATIONS
DEUTERIUM IONS
DISSOCIATION
FOURIER ANALYSIS
LASER RADIATION
LASERS
MICROSCOPES
MOLECULAR DYNAMICS METHOD
MOLECULAR IONS
PHOTOLYSIS
PHOTON-MOLECULE COLLISIONS
POTENTIAL ENERGY
POTENTIALS
REACTION KINETICS
SPECTRA
TIME RESOLUTION
TWO-DIMENSIONAL CALCULATIONS
VIBRATIONAL STATES
WAVE PACKETS
CATIONS
DEUTERIUM IONS
DISSOCIATION
FOURIER ANALYSIS
LASER RADIATION
LASERS
MICROSCOPES
MOLECULAR DYNAMICS METHOD
MOLECULAR IONS
PHOTOLYSIS
PHOTON-MOLECULE COLLISIONS
POTENTIAL ENERGY
POTENTIALS
REACTION KINETICS
SPECTRA
TIME RESOLUTION
TWO-DIMENSIONAL CALCULATIONS
VIBRATIONAL STATES
WAVE PACKETS