Isotopic Transmutations in Irradiated Beryllium and Their Implications on MARIA Reactor Operation
Beryllium irradiated by neutrons with energies above 0.7 MeV undergoes (n,{alpha}) and (n,2n) reactions. The Be(n,{alpha}) reaction results in subsequent buildup of {sup 6}Li and {sup 3}He isotopes with large thermal neutron absorption cross sections causing poisoning of irradiated beryllium. The amount of the poison isotopes depends on the neutron flux level and spectrum. The high-flux MARIA reactor operated in Poland since 1975 consists of a beryllium matrix with fuel channels in cutouts of beryllium blocks. As the experimental determination of {sup 6}Li, {sup 3}H, and {sup 3}He content in the operational reactor is impossible, a systematic computational study of the effect of {sup 3}He and {sup 6}Li presence in beryllium blocks on MARIA reactor reactivity and power density distribution has been undertaken. The analysis of equations governing the transmutation has been done for neutron flux parameters typical for MARIA beryllium blocks. Study of the mutual influence of reactor operational parameters and the buildup of {sup 6}Li, {sup 3}H, and {sup 3}He in beryllium blocks has shown the necessity of a detailed spatial solution of transmutation equations in the reactor, taking into account the whole history of its operation. Therefore, fuel management calculations using the REBUS code with included chains for Be(n,{alpha})-initiated reactions have been done for the whole reactor lifetime. The calculated poisoning of beryllium blocks has been verified against the critical experiment of 1993. Finally, the current {sup 6}Li, {sup 3}H, and {sup 3}He contents, averaged for each beryllium block, have been calculated. The reactivity drop caused by this poisoning is {approx}7%.
- OSTI ID:
- 20840201
- Journal Information:
- Nuclear Technology, Vol. 146, Issue 1; Other Information: Copyright (c) 2006 American Nuclear Society (ANS), United States, All rights reserved. http://epubs.ans.org/; Country of input: International Atomic Energy Agency (IAEA); ISSN 0029-5450
- Country of Publication:
- United States
- Language:
- English
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