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Title: Spectroscopy of Stripe Order in La{sub 1.8}Sr{sub 0.2}NiO{sub 4} Using Resonant Soft X-Ray Diffraction

Journal Article · · Physical Review Letters
; ; ; ; ; ;  [1];  [2]; ; ;  [3];  [1];  [1];  [4]; ;  [5]
  1. II. Physikalisches Institut, Universitaet zu Koeln, Zuelpicher Strasse 77, D-50937 Cologne (Germany)
  2. Department of Quantum Matter, ADSM, Hiroshima University, Higashi-Hiroshima 739-8530 (Japan)
  3. Institut fuer Experimentalphysik, Freie Universitaet Berlin, Arnimallee 14, D-14195 Berlin (Germany)
  4. Department of Physics and Astronomy, University of British Columbia, 6224 Agricultural Road, Vancouver, British Columbia, V6T 1Z1 (Canada)
  5. National Synchrotron Radiation Research Center, Hsinchu 30076, Taiwan (China)

Strong resonant enhancements of the charge-order and spin-order superstructure-diffraction intensities in La{sub 1.8}Sr{sub 0.2}NiO{sub 4} are observed when x-ray energies in the vicinity of the Ni L{sub 2,3} absorption edges are used. The pronounced photon-energy and polarization dependences of these diffraction intensities allow for a critical determination of the local symmetry of the ordered spin and charge carriers. We found that not only the antiferromagnetic order but also the charge-order superstructure resides within the NiO{sub 2} layers; the holes are mainly located on in-plane oxygens surrounding a Ni{sup 2+} site with the spins coupled antiparallel in close analogy to Zhang-Rice singlets in the cuprates.

OSTI ID:
20696548
Journal Information:
Physical Review Letters, Vol. 95, Issue 15; Other Information: DOI: 10.1103/PhysRevLett.95.156402; (c) 2005 The American Physical Society; Country of input: International Atomic Energy Agency (IAEA); ISSN 0031-9007
Country of Publication:
United States
Language:
English