Solid-state batteries: The critical role of mechanics

Kalnaus, Sergiy; Dudney, Nancy J.; Westover, Andrew S.; Herbert, Erik; Hackney, Steve

doi:10.1126/science.abg5998

Solid-state batteries: The critical role of mechanics

Journal Article · Fri Sep 22 00:00:00 EDT 2023 · Science

DOI:https://doi.org/10.1126/science.abg5998· OSTI ID:2007741

^[1]; ^[1]; Westover, Andrew S. ^[1]; Herbert, Erik ^[1]; ^[2]

Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)
Michigan Technological University, Houghton, MI (United States)

Solid-state batteries with lithium metal anodes have the potential for higher energy density, longer lifetime, wider operating temperature, and increased safety. Although the bulk of the research has focused on improving transport kinetics and electrochemical stability of the materials and interfaces, there are also critical challenges that require investigation of the mechanics of materials. In batteries with solid-solid interfaces, mechanical contacts, and the development of stresses during operation of the solid-state batteries, become as critical as the electrochemical stability to keep steady charge transfer at these interfaces. In conclusion, this review will focus on stress and strain that result from normal and extended battery cycling and the associated mechanisms for stress relief, some of which lead to failure of these batteries.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Energy Efficiency and Renewable Energy (EERE), Office of Sustainable Transportation. Vehicle Technologies Office (VTO)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 2007741

Journal Information:: Science, Journal Name: Science Journal Issue: 6664 Vol. 381; ISSN 0036-8075

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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