Dynamic fracture processes in hydrogen embrittled iron

Lee, Andrew C.; Parakh, Abhinav; Lam, Sebastian; Sleugh, Andrew; Tertuliano, Ottman; Doan, David; Weker, Johanna Nelson; Hosemann, Peter; Gu, X. Wendy

doi:10.1016/j.actamat.2023.119234

Dynamic fracture processes in hydrogen embrittled iron

Journal Article · Sun Oct 01 04:00:00 EDT 2023 · Acta Materialia

DOI:https://doi.org/10.1016/j.actamat.2023.119234· OSTI ID:2007055

^[1]; ; Lam, Sebastian; Sleugh, Andrew; ; ; ; Hosemann, Peter;

SLAC National Accelerator Laborator

Mechanistic understanding of hydrogen embrittlement is critical to the transport and storage of hydrogen as a sustainable fuel. Experimental observation of dynamic fracture processes in hydrogen environments has been challenging. Here, in-situ transmission X-ray microscopy is used to image polycrystalline iron foils that are concurrently strained and electrochemically charged with hydrogen. Using this technique, voids and microcracks down to ∼30 nm in size are identified at or near the crack tip and tracked as strain is increased. We observe both hydrogen-induced transgranular failure and hydrogen-induced intergranular failure with distinct fracture processes. We find that transgranular fracture occurs through the formation of sharp branched structures at the main crack tip that are reminiscent of slip band formation. This is followed by void growth and coalescence, and interaction with secondary cracks that lead to propagation of the main crack. Intergranular fracture is found to occur through void coalescence along grain boundaries, along with significant secondary cracking near the crack tip. The crack growth rate is greater for void-mediated intergranular failure than for slip-mediated transgranular failure. Additionally, the removal of hydrogen results in recovered ductility for a crack initially propagated under hydrogen charging.

View Accepted Manuscript (DOE)

Research Organization:: SLAC National Accelerator Laboratory (SLAC), Menlo Park, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Scientific User Facilities (SUF)

Grant/Contract Number:: AC02-76SF00515

OSTI ID:: 2007055

Alternate ID(s):: OSTI ID: 2204951

Journal Information:: Acta Materialia, Journal Name: Acta Materialia Vol. 259; ISSN 1359-6454

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

References (69)

Modeling of hydrogen-assisted ductile crack propagation in metals and alloys Ahn, D. C.; Sofronis, P.; Dodds, R. International Journal of Fracture, Vol. 145, Issue 2 https://doi.org/10.1007/s10704-007-9112-3	journal	September 2007
In Situ Experiments with X ray Tomography: an Attractive Tool for Experimental Mechanics Buffiere, J. -Y.; Maire, E.; Adrien, J. Experimental Mechanics, Vol. 50, Issue 3 https://doi.org/10.1007/s11340-010-9333-7	journal	January 2010
Role of Crystallographic Texture in Hydrogen-Induced Cracking of Low Carbon Steels for Sour Service Piping Venegas, V.; Caleyo, F.; Hallen, J. M. Metallurgical and Materials Transactions A, Vol. 38, Issue 5 https://doi.org/10.1007/s11661-007-9130-9	journal	April 2007
Hydrogen Embrittlement Understood Robertson, Ian M.; Sofronis, P.; Nagao, A. Metallurgical and Materials Transactions A, Vol. 46, Issue 6 https://doi.org/10.1007/s11661-015-2836-1	journal	March 2015
The role of dislocations in the growth of nanosized voids in ductile failure of metals Meyers, Marc A.; Traiviratana, Sirirat; Lubarda, V. A. JOM, Vol. 61, Issue 2 https://doi.org/10.1007/s11837-009-0025-7	journal	February 2009
Equilibrium aspects of hydrogen-induced cracking of steels Oriani, R. A.; Josephic, P. H. Acta Metallurgica, Vol. 22, Issue 9 https://doi.org/10.1016/0001-6160(74)90061-3	journal	September 1974
Hydrogen embrittlement of α titanium: In situ tem studies Shih, D. S.; Robertson, I. M.; Birnbaum, H. K. Acta Metallurgica, Vol. 36, Issue 1 https://doi.org/10.1016/0001-6160(88)90032-6	journal	January 1988
Crack extension by alternating shear Pelloux, R. M. N. Engineering Fracture Mechanics, Vol. 1, Issue 4 https://doi.org/10.1016/0013-7944(70)90008-1	journal	April 1970
An analysis of ductile rupture in notched bars Needleman, A.; Tvergaard, V. Journal of the Mechanics and Physics of Solids, Vol. 32, Issue 6 https://doi.org/10.1016/0022-5096(84)90031-0	journal	January 1984
Embrittlement of interfaces by solute segregation Rice, James R.; Wang, Jian-Sheng Materials Science and Engineering: A, Vol. 107 https://doi.org/10.1016/0921-5093(89)90372-9	journal	January 1989
Hydrogen-enhanced localized plasticity—a mechanism for hydrogen-related fracture Birnbaum, H. K.; Sofronis, P. Materials Science and Engineering: A, Vol. 176, Issue 1-2 https://doi.org/10.1016/0921-5093(94)90975-X	journal	March 1994
Ductile fracture by vacancy condensation in f.c.c. single crystals Cuitiño, A. M.; Ortiz, M. Acta Materialia, Vol. 44, Issue 2 https://doi.org/10.1016/1359-6454(95)00220-0	journal	February 1996
Texture, formability, lamellar tearing and HIC susceptibility of ferritic and low-carbon HSLA steels Verdeja, J. I.; Asensio, J.; Pero-Sanz, J. A. Materials Characterization, Vol. 50, Issue 1 https://doi.org/10.1016/S1044-5803(03)00106-2	journal	January 2003
Void growth by dislocation emission Lubarda, V. A.; Schneider, M. S.; Kalantar, D. H. Acta Materialia, Vol. 52, Issue 6 https://doi.org/10.1016/j.actamat.2003.11.022	journal	April 2004
Grain-boundary engineering markedly reduces susceptibility to intergranular hydrogen embrittlement in metallic materials Bechtle, S.; Kumar, M.; Somerday, B. P. Acta Materialia, Vol. 57, Issue 14 https://doi.org/10.1016/j.actamat.2009.05.012	journal	August 2009
Recent developments in the study of hydrogen embrittlement: Hydrogen effect on dislocation nucleation Barnoush, Afrooz; Vehoff, Horst Acta Materialia, Vol. 58, Issue 16 https://doi.org/10.1016/j.actamat.2010.05.057	journal	September 2010
On the formation and nature of quasi-cleavage fracture surfaces in hydrogen embrittled steels Martin, May L.; Fenske, Jamey A.; Liu, Grace S. Acta Materialia, Vol. 59, Issue 4 https://doi.org/10.1016/j.actamat.2010.11.024	journal	February 2011
Hydrogen embrittlement of ferritic steels: Observations on deformation microstructure, nanoscale dimples and failure by nanovoiding Neeraj, T.; Srinivasan, R.; Li, Ju Acta Materialia, Vol. 60, Issue 13-14 https://doi.org/10.1016/j.actamat.2012.06.014	journal	August 2012
Elucidating the variables affecting accelerated fatigue crack growth of steels in hydrogen gas with low oxygen concentrations Somerday, B. P.; Sofronis, P.; Nibur, K. A. Acta Materialia, Vol. 61, Issue 16 https://doi.org/10.1016/j.actamat.2013.07.001	journal	September 2013
Hydrogen-assisted decohesion and localized plasticity in dual-phase steel Koyama, Motomichi; Tasan, Cemal Cem; Akiyama, Eiji Acta Materialia, Vol. 70 https://doi.org/10.1016/j.actamat.2014.01.048	journal	May 2014
Hydrogen-induced intergranular failure of iron Wang, Shuai; Martin, May L.; Sofronis, Petros Acta Materialia, Vol. 69 https://doi.org/10.1016/j.actamat.2014.01.060	journal	May 2014
Crack and blister initiation and growth in purified iron due to hydrogen loading Tiegel, Marie C.; Martin, May L.; Lehmberg, Annegret K. Acta Materialia, Vol. 115 https://doi.org/10.1016/j.actamat.2016.05.034	journal	August 2016
Hydrogen embrittlement revealed via novel in situ fracture experiments using notched micro-cantilever specimens Deng, Yun; Barnoush, Afrooz Acta Materialia, Vol. 142 https://doi.org/10.1016/j.actamat.2017.09.057	journal	January 2018
The predominant role of strain-induced vacancies in hydrogen embrittlement of steels: Overview Nagumo, Michihiko; Takai, Kenichi Acta Materialia, Vol. 165 https://doi.org/10.1016/j.actamat.2018.12.013	journal	February 2019
Enumeration of the hydrogen-enhanced localized plasticity mechanism for hydrogen embrittlement in structural materials Martin, May L.; Dadfarnia, Mohsen; Nagao, Akihide Acta Materialia, Vol. 165 https://doi.org/10.1016/j.actamat.2018.12.014	journal	February 2019
Assessment of hydrogen embrittlement via image-based techniques in Al–Zn–Mg–Cu aluminum alloys Su, Hang; Toda, Hiroyuki; Shimizu, Kazuyuki Acta Materialia, Vol. 176 https://doi.org/10.1016/j.actamat.2019.06.056	journal	September 2019
Quantities and distribution of strain-induced vacancies and dislocations enhanced by hydrogen in iron Sugiyama, Yuri; Takai, Kenichi Acta Materialia, Vol. 208 https://doi.org/10.1016/j.actamat.2021.116663	journal	April 2021
Suppressed hydrogen embrittlement of high-strength Al alloys by Mn-rich intermetallic compound particles Xu, Yuantao; Toda, Hiroyuki; Shimizu, Kazuyuki Acta Materialia, Vol. 236 https://doi.org/10.1016/j.actamat.2022.118110	journal	September 2022
Hydrogen-enhanced grain boundary vacancy stockpiling causes transgranular to intergranular fracture transition Ding, Yu; Yu, Haiyang; Lin, Meichao Acta Materialia, Vol. 239 https://doi.org/10.1016/j.actamat.2022.118279	journal	October 2022
In situ characterisation of the strain fields of intragranular slip bands in ferrite by high-resolution electron backscatter diffraction Koko, Abdalrhaman; Elmukashfi, Elsiddig; Becker, Thorsten H. Acta Materialia, Vol. 239 https://doi.org/10.1016/j.actamat.2022.118284	journal	October 2022
Effect of alloying elements on hydrogen enhanced decohesion in bcc iron Kholtobina, Anastasiia S.; Ecker, Werner; Pippan, Reinhard Computational Materials Science, Vol. 188 https://doi.org/10.1016/j.commatsci.2020.110215	journal	February 2021
Pronounced transition of crack initiation and propagation modes in the hydrogen-related failure of a Ni-based superalloy 718 under internal and external hydrogen conditions Ogawa, Yuhei; Takakuwa, Osamu; Okazaki, Saburo Corrosion Science, Vol. 161 https://doi.org/10.1016/j.corsci.2019.108186	journal	December 2019
Effect of hydrogen charging time on hydrogen blister and hydrogen-induced cracking of pure iron Li, Xinfeng; Huang, Weihong; Wu, Xubin Corrosion Science, Vol. 181 https://doi.org/10.1016/j.corsci.2020.109200	journal	April 2021
Hydrogen damage of steels: A case study and hydrogen embrittlement model Djukic, M. B.; Sijacki Zeravcic, V.; Bakic, G. M. Engineering Failure Analysis, Vol. 58 https://doi.org/10.1016/j.engfailanal.2015.05.017	journal	December 2015
The synergistic action and interplay of hydrogen embrittlement mechanisms in steels and iron: Localized plasticity and decohesion Djukic, Milos B.; Bakic, Gordana M.; Sijacki Zeravcic, Vera Engineering Fracture Mechanics, Vol. 216 https://doi.org/10.1016/j.engfracmech.2019.106528	journal	July 2019
Hydrogen-assisted, intergranular, fatigue crack-growth in ferritic iron: Influences of hydrogen-gas pressure and temperature variation Ogawa, Yuhei; Umakoshi, Kensuke; Nakamura, Masami International Journal of Fatigue, Vol. 140 https://doi.org/10.1016/j.ijfatigue.2020.105806	journal	November 2020
Hydrogen-microvoid interactions at continuum scale Yu, Haiyang; Olsen, Jim Stian; He, Jianying International Journal of Hydrogen Energy, Vol. 43, Issue 21 https://doi.org/10.1016/j.ijhydene.2018.04.064	journal	May 2018
Strain rate and hydrogen effects on crack growth from a notch in a Fe-high-Mn steel containing 1.1 wt% solute carbon Najam, Hina; Koyama, Motomichi; Bal, Burak International Journal of Hydrogen Energy, Vol. 45, Issue 1 https://doi.org/10.1016/j.ijhydene.2019.10.227	journal	January 2020
The effects of double notches on the mechanical properties of a high-strength pipeline steel under hydrogen atmosphere Zhang, Shuai; An, Teng; Zheng, Shuqi International Journal of Hydrogen Energy, Vol. 45, Issue 43 https://doi.org/10.1016/j.ijhydene.2020.06.058	journal	September 2020
Effect of hydrogen on fracture locus of Fe–16Mn–0.6C–2.15Al TWIP steel Bal, Burak; Çetin, Barış; Bayram, Ferdi Caner International Journal of Hydrogen Energy, Vol. 45, Issue 58 https://doi.org/10.1016/j.ijhydene.2020.09.083	journal	November 2020
Strain rate sensitivity of hydrogen-assisted ε-martensitic transformation and associated hydrogen embrittlement in high-Mn steel Hao, Chunxi; Koyama, Motomichi; Ajito, Saya International Journal of Hydrogen Energy, Vol. 46, Issue 53 https://doi.org/10.1016/j.ijhydene.2021.05.162	journal	August 2021
Hydrogen embrittlement controlled by reaction of dislocation with grain boundary in alpha-iron Wan, Liang; Geng, Wen Tong; Ishii, Akio International Journal of Plasticity, Vol. 112 https://doi.org/10.1016/j.ijplas.2018.08.013	journal	January 2019
A quantum-mechanically informed continuum model of hydrogen embrittlement Serebrinsky, S. Journal of the Mechanics and Physics of Solids, Vol. 52, Issue 10 https://doi.org/10.1016/j.jmps.2004.02.010	journal	October 2004
A fracture criterion for the notch strength of high strength steels in the presence of hydrogen Ayas, C.; Deshpande, V. S.; Fleck, N. A. Journal of the Mechanics and Physics of Solids, Vol. 63 https://doi.org/10.1016/j.jmps.2013.10.002	journal	February 2014
The effect of sample thickness on micro-mesoscale tensile properties of 304SS, HT-9, and CuCrZr Dong, A.; Vo, H.; Olivas, E. Journal of Nuclear Materials, Vol. 575 https://doi.org/10.1016/j.jnucmat.2022.154207	journal	March 2023
Interaction of hydrogen with crack-tip plasticity: effects of constraint on void growth Liang, Y.; Sofronis, P.; Dodds, R. H. Materials Science and Engineering: A, Vol. 366, Issue 2 https://doi.org/10.1016/j.msea.2003.09.052	journal	February 2004
Evaluation of hydrogen induced damage of steels by different test methods Rosenberg, G.; Sinaiova, I. Materials Science and Engineering: A, Vol. 682 https://doi.org/10.1016/j.msea.2016.11.067	journal	January 2017
Influence of nanovoids in the hydrogen embrittlement fracture of Al–Zn–Mg–Cu alloys Shimizu, Kazuyuki; Toda, Hiroyuki; Kadogawa, Chihiro Materialia, Vol. 11 https://doi.org/10.1016/j.mtla.2020.100667	journal	June 2020
EBSD study of hydrogen-induced cracking in API-5L-X46 pipeline steel Venegas, V.; Caleyo, F.; González, J. L. Scripta Materialia, Vol. 52, Issue 2 https://doi.org/10.1016/j.scriptamat.2004.09.015	journal	January 2005
Revisiting hydrogen embrittlement models and hydrogen-induced homogeneous nucleation of dislocations Kirchheim, Reiner Scripta Materialia, Vol. 62, Issue 2 https://doi.org/10.1016/j.scriptamat.2009.09.037	journal	January 2010
In-situ micro-cantilever bending test in environmental scanning electron microscope: Real time observation of hydrogen enhanced cracking Deng, Y.; Hajilou, T.; Wan, D. Scripta Materialia, Vol. 127 https://doi.org/10.1016/j.scriptamat.2016.08.026	journal	January 2017
Hydrogen assisted crack initiation in metals under monotonic loading: A new experimental approach Arora, Aman; Kumar, Rakesh; Singh, Harpreet Theoretical and Applied Fracture Mechanics, Vol. 112 https://doi.org/10.1016/j.tafmec.2021.102917	journal	April 2021
Hydrogen-Enhanced Vacancy Diffusion in Metals Du, Jun-Ping; Geng, W. T.; Arakawa, Kazuto The Journal of Physical Chemistry Letters, Vol. 11, Issue 17 https://doi.org/10.1021/acs.jpclett.0c01798	journal	July 2020
In Operando X-ray Diffraction and Transmission X-ray Microscopy of Lithium Sulfur Batteries Nelson, Johanna; Misra, Sumohan; Yang, Yuan Journal of the American Chemical Society, Vol. 134, Issue 14 https://doi.org/10.1021/ja2121926	journal	March 2012
Hydrogenated vacancies lock dislocations in aluminium Xie, Degang; Li, Suzhi; Li, Meng Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms13341	journal	November 2016
The dual role of coherent twin boundaries in hydrogen embrittlement Seita, Matteo; Hanson, John P.; Gradečak, Silvija Nature Communications, Vol. 6, Issue 1 https://doi.org/10.1038/ncomms7164	journal	February 2015
Crystallographic character of grain boundaries resistant to hydrogen-assisted fracture in Ni-base alloy 725 Hanson, John P.; Bagri, Akbar; Lind, Jonathan Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-05549-y	journal	August 2018
The Hydrogen Economy Crabtree, George W.; Dresselhaus, Mildred S.; Buchanan, Michelle V. Physics Today, Vol. 57, Issue 12 https://doi.org/10.1063/1.1878333	journal	December 2004
Effect of amorphization-mediated plasticity on the hydrogen-void interaction in ideal lattices under hydrostatic tension Zhao, Kai; He, Jianying; Ringdalen, Inga Gudem Journal of Applied Physics, Vol. 123, Issue 24 https://doi.org/10.1063/1.5029953	journal	June 2018
TXM-Wizard : a program for advanced data collection and evaluation in full-field transmission X-ray microscopy Liu, Yijin; Meirer, Florian; Williams, Phillip A. Journal of Synchrotron Radiation, Vol. 19, Issue 2 https://doi.org/10.1107/S0909049511049144	journal	January 2012
Crack Interaction, Coalescence and Mixed mode Fracture Mechanics Wang, Y. -Z.; Atkinson, J. D.; Akid, R. Fatigue & Fracture of Engineering Materials and Structures, Vol. 19, Issue 4 https://doi.org/10.1111/j.1460-2695.1996.tb00979.x	journal	April 1996
Continuum Theory of Ductile Rupture by Void Nucleation and Growth: Part I—Yield Criteria and Flow Rules for Porous Ductile Media Gurson, A. L. Journal of Engineering Materials and Technology, Vol. 99, Issue 1 https://doi.org/10.1115/1.3443401	journal	January 1977
Origin of micrometer-scale dislocation motion during hydrogen desorption Koyama, Motomichi; Taheri-Mousavi, Seyedeh Mohadeseh; Yan, Haoxue Science Advances, Vol. 6, Issue 23 https://doi.org/10.1126/sciadv.aaz1187	journal	June 2020
Cementite-particle solution and influence of interstitials on machinability of low-carbon steel Hau-Bracamonte, J. L.; Wise, M. L. H. Metals Technology, Vol. 9, Issue 1 https://doi.org/10.1179/030716982803285666	journal	January 1982
Discussion of some recent literature on hydrogen-embrittlement mechanisms: addressing common misunderstandings Lynch, Stan Corrosion Reviews, Vol. 37, Issue 5 https://doi.org/10.1515/corrrev-2019-0017	journal	June 2019
Hydrogen embrittlement (HE) phenomena and mechanisms Lynch, S. P. Stress Corrosion Cracking, p. 90-130 https://doi.org/10.1533/9780857093769.1.90	book	January 2011
Formation of Manganese Sulfide in Low Carbon Steel Ito, Yoichi; Yonezawa, Noboru; Matsubara, Kaichi Tetsu-to-Hagane, Vol. 68, Issue 10 https://doi.org/10.2355/tetsutohagane1955.68.10_1569	journal	January 1982
Role of Hydrogen-Charging on Nucleation and Growth of Ductile Damage in Austenitic Stainless Steels Maire, Eric; Grabon, Stanislas; Adrien, Jérôme Materials, Vol. 12, Issue 9 https://doi.org/10.3390/ma12091426	journal	May 2019
Ab Initio Study of the Combined Effects of Alloying Elements and H on Grain Boundary Cohesion in Ferritic Steels P. A. Subramanyam, Aparna; Azócar Guzmán, Abril; Vincent, Smobin Metals, Vol. 9, Issue 3 https://doi.org/10.3390/met9030291	journal	March 2019

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