MXene-Based Porous Monoliths

Yang, Yang; Li, Kaijuan; Wang, Yaxin; Wu, Zhanpeng; Russell, Thomas P.; Shi, Shaowei

doi:10.3390/nano12213792

MXene-Based Porous Monoliths

Journal Article · Thu Oct 27 00:00:00 EDT 2022 · Nanomaterials

DOI:https://doi.org/10.3390/nano12213792· OSTI ID:1992321

Yang, Yang ^[1]; Li, Kaijuan ^[1]; Wang, Yaxin ^[1]; Wu, Zhanpeng ^[1]; ^[2]; ^[1]

Beijing University of Chemical Technology (China)
University of Massachusetts, Amherst, MA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

In the past decade, a thriving family of 2D nanomaterials, transition-metal carbides/nitrides (MXenes), have garnered tremendous interest due to its intriguing physical/chemical properties, structural features, and versatile functionality. Integrating these 2D nanosheets into 3D monoliths offers an exciting and powerful platform for translating their fundamental advantages into practical applications. Introducing internal pores, such as isotropic pores and aligned channels, within the monoliths can not only address the restacking of MXenes, but also afford a series of novel and, in some cases, unique structural merits to advance the utility of the MXene-based materials. Here, a brief overview of the development of MXene-based porous monoliths, in terms of the types of microstructures, is provided, focusing on the pore design and how the porous microstructure affects the application performance.

View Accepted Manuscript (DOE)

Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1992321

Journal Information:: Nanomaterials, Journal Name: Nanomaterials Journal Issue: 21 Vol. 12; ISSN 2079-4991

Publisher:: MDPICopyright Statement

Country of Publication:: United States

Language:: English

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Assessment of Occlusal Force and Local Gas Release Using Degradable Bacterial Cellulose/Ti₃C₂T_x MXene Bioaerogel for Oral Healthcare Jin, Xiujuan; Li, Linlin; Zhao, Shufang ACS Nano, Vol. 15, Issue 11 https://doi.org/10.1021/acsnano.1c07891	journal	November 2021
3D Printed Template-Assisted Assembly of Additive-Free Ti₃C₂T_x MXene Microlattices with Customized Structures toward High Areal Capacitance Yang, Chuang; Wu, Xin; Xia, Heyi ACS Nano, Vol. 16, Issue 2 https://doi.org/10.1021/acsnano.1c09622	journal	January 2022
Design of Vertically Aligned Two-Dimensional Heterostructures of Rigid Ti₃C₂T_X MXene and Pliable Vanadium Pentoxide for Efficient Lithium Ion Storage Dai, Henghan; Zhao, Xi; Xu, Hai ACS Nano, Vol. 16, Issue 4 https://doi.org/10.1021/acsnano.1c10212	journal	April 2022
3D-Printed Sodiophilic V₂CT_x/rGO-CNT MXene Microgrid Aerogel for Stable Na Metal Anode with High Areal Capacity Wang, Zixuan; Huang, Zhenxin; Wang, Hui ACS Nano, Vol. 16, Issue 6 https://doi.org/10.1021/acsnano.2c01186	journal	June 2022
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Biomimetic Porous MXene Sediment-Based Hydrogel for High-Performance and Multifunctional Electromagnetic Interference Shielding Yang, Yunfei; Wu, Na; Li, Bin ACS Nano, Vol. 16, Issue 9 https://doi.org/10.1021/acsnano.2c06164	journal	August 2022
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MXene Ti ₃ C ₂ : An Effective 2D Light-to-Heat Conversion Material Li, Renyuan; Zhang, Lianbin; Shi, Le ACS Nano, Vol. 11, Issue 4 https://doi.org/10.1021/acsnano.6b08415	journal	March 2017
3D Synergistical MXene/Reduced Graphene Oxide Aerogel for a Piezoresistive Sensor Ma, Yanan; Yue, Yang; Zhang, Hang ACS Nano, Vol. 12, Issue 4 https://doi.org/10.1021/acsnano.7b06909	journal	March 2018
Graphene-Based Standalone Solar Energy Converter for Water Desalination and Purification Yang, Yang; Zhao, Ruiqi; Zhang, Tengfei ACS Nano, Vol. 12, Issue 1 https://doi.org/10.1021/acsnano.7b08196	journal	January 2018
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Freeze-Casting Produces a Graphene Oxide Aerogel with a Radial and Centrosymmetric Structure Wang, Chunhui; Chen, Xiong; Wang, Bin ACS Nano, Vol. 12, Issue 6 https://doi.org/10.1021/acsnano.8b01747	journal	May 2018
Highly Electrically Conductive Three-Dimensional Ti ₃ C ₂ T _x MXene/Reduced Graphene Oxide Hybrid Aerogels with Excellent Electromagnetic Interference Shielding Performances Zhao, Sai; Zhang, Hao-Bin; Luo, Jia-Qi ACS Nano, Vol. 12, Issue 11 https://doi.org/10.1021/acsnano.8b05739	journal	October 2018
Ti₃C₂T_x-Based Three-Dimensional Hydrogel by a Graphene Oxide-Assisted Self-Convergence Process for Enhanced Photoredox Catalysis Chen, Yan; Xie, Xiuqiang; Xin, Xin ACS Nano, Vol. 13, Issue 1 https://doi.org/10.1021/acsnano.8b06136	journal	December 2018
Sculpting Liquids with Two-Dimensional Materials: The Assembly of Ti ₃ C ₂ T _x MXene Sheets at Liquid–Liquid Interfaces Cain, Jeffrey D.; Azizi, Amin; Maleski, Kathleen ACS Nano, Vol. 13, Issue 11 https://doi.org/10.1021/acsnano.9b05088	journal	October 2019
Vertically Aligned Janus MXene-Based Aerogels for Solar Desalination with High Efficiency and Salt Resistance Zhang, Qi; Yi, Gang; Fu, Ze ACS Nano, Vol. 13, Issue 11 https://doi.org/10.1021/acsnano.9b06180	journal	October 2019
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Highly Stable 3D Ti₃C₂T_x MXene-Based Foam Architectures toward High-Performance Terahertz Radiation Shielding Lin, Zehui; Liu, Ji; Peng, Wei ACS Nano, Vol. 14, Issue 2 https://doi.org/10.1021/acsnano.9b08832	journal	January 2020
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