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The new Device for Indirect Capture Experiments on Radionuclides at LANSCE: Efforts on measuring the resonance(s) responsible for the extremely large 88Zr (n,γ) cross section

Journal Article · · EPJ Web of Conferences (Online)
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  1. Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

The thermal neutron capture cross section of 88Zr was recently reported to be the second largest in nature with the largest resonance integral measured. Presumably, these very large values are caused by a resonance or resonances very near thermal energy. Determining their energies and widths, and hence the shape of the cross section away from thermal energies,is useful for applications. The short half-life (83.4 days) and associated large background, renders direct measurements of the neutron capture cross section impossible using current techniques. However, it is possible to measure the total neutron cross section, and hence the resonance properties, using the newly commissioned Device for Indirect Capture Experiments on Radionuclides (DICER) at the Los Alamos Neutron Science Center (LANSCE). Transmission measurements are utilized as a surrogate method to perform capture measurements. The 88Zr needed for a DICER measurement was produced at the Isotope Production Facility (IPF) and cleanly separated from the production target material. A description of the new instrument, efforts and preliminary results on 88Zr will be presented.

Research Organization:
Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA); USDOE Laboratory Directed Research and Development (LDRD) Program
Grant/Contract Number:
89233218CNA000001
OSTI ID:
1990120
Report Number(s):
LA-UR-22-29884
Journal Information:
EPJ Web of Conferences (Online), Journal Name: EPJ Web of Conferences (Online) Vol. 284; ISSN 2100-014X
Publisher:
EDP SciencesCopyright Statement
Country of Publication:
United States
Language:
English

References (13)

The first generation of γ-rays from hot nuclei
  • Guttormsen, M.; Ramsøy, T.; Rekstad, J.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 255, Issue 3 https://doi.org/10.1016/0168-9002(87)91221-6
journal April 1987
Direct measurements of neutron capture on radioactive isotopes journal September 2007
The Los Alamos Neutron Science Center
  • Lisowski, Paul W.; Schoenberg, Kurt F.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 562, Issue 2 https://doi.org/10.1016/j.nima.2006.02.178
journal June 2006
Physics design of the next-generation spallation neutron target-moderator-reflector-shield assembly at LANSCE
  • Zavorka, Lukas; Mocko, Michael J.; Koehler, Paul E.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 901 https://doi.org/10.1016/j.nima.2018.06.018
journal September 2018
New capability for neutron transmission measurements at LANSCE: The DICER instrument
  • Stamatopoulos, A.; Koehler, P.; Couture, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 1025 https://doi.org/10.1016/j.nima.2021.166166
journal February 2022
The surprisingly large neutron capture cross-section of 88Zr journal January 2019
Aqueous harvesting of Zr 88 at a radioactive-ion-beam facility for cross-section measurements journal February 2021
γ -ray strength function method and its application to Pd 107 journal December 2010
Photoneutron cross sections for Mo isotopes: A step toward a unified understanding of ( γ , n ) and ( n , γ ) reactions journal July 2013
Improved 192 , 194 , 195 , 196 Pt( n , γ ) and 192 Ir( n , γ ) astrophysical reaction rates journal September 2013
Novel technique for Constraining r -Process ( n , γ ) Reaction Rates journal December 2014
Constraining Neutron Capture Cross Sections for Unstable Nuclei with Surrogate Reaction Data and Theory journal July 2018
Updated User's Guide for Sammy: Multilevel R-Matrix Fits to Neutron Data Using Bayes' Equations report October 2008

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