Colloidal Semiconductor Nanocrystal Lasers and Laser Diodes

Ahn, Namyoung; Livache, Clément; Pinchetti, Valerio; Klimov, Victor I.

doi:10.1021/acs.chemrev.2c00865

Colloidal Semiconductor Nanocrystal Lasers and Laser Diodes

Journal Article · Wed Jun 28 00:00:00 EDT 2023 · Chemical Reviews

DOI:https://doi.org/10.1021/acs.chemrev.2c00865· OSTI ID:1987574

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Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Lasers and optical amplifiers based on solution-processable materials have been long-desired devices for their compatibility with virtually any substrate, scalability, and ease of integration with on-chip photonics and electronics. These devices have been pursued across a wide range of materials including polymers, small molecules, perovskites, and chemically prepared colloidal semiconductor nanocrystals, also commonly referred to as colloidal quantum dots. The latter materials are especially attractive for implementing optical-gain media as in addition to being compatible with inexpensive and easily scalable chemical techniques, they offer multiple advantages derived from a zero-dimensional character of their electronic states. These include a size-tunable emission wavelength, low optical gain thresholds, and weak sensitivity of lasing characteristics to variations in temperature. Here we review the status of colloidal nanocrystal lasing devices, most recent advances in this field, outstanding challenges, and the ongoing progress toward technological viable devices including colloidal quantum dot laser diodes.

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Research Organization:: Los Alamos National Laboratory (LANL), Los Alamos, NM (United States)

Sponsoring Organization:: USDOE Laboratory Directed Research and Development (LDRD) Program

Grant/Contract Number:: 89233218CNA000001

OSTI ID:: 1987574

Alternate ID(s):: OSTI ID: 1989167

Report Number(s):: LA-UR-23-23343

Journal Information:: Chemical Reviews, Journal Name: Chemical Reviews Journal Issue: 13 Vol. 123; ISSN 0009-2665

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Journal Article · Sun Feb 14 19:00:00 EST 2021 · Nature Reviews. Materials · OSTI ID:1864315

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