Photoluminescence of Cr3+ in β-Ga2O3 and (Al0.1Ga0.9)2O3 under pressure

Barmore, Lauren M.; Jesenovec, Jani; McCloy, John S.; McCluskey, Matthew D.

doi:10.1063/5.0149900

Title: Photoluminescence of Cr³⁺ in β-Ga₂O₃ and (Al_0.1Ga_0.9)₂O₃ under pressure

Journal Article · Wed May 03 00:00:00 EDT 2023 · Journal of Applied Physics

DOI:https://doi.org/10.1063/5.0149900· OSTI ID:1986488

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Washington State University, Pullman, WA (United States)

The effects of pressure on single crystals of Cr-doped gallium oxide (β-Ga₂O₃:Cr³⁺) and aluminum gallium oxide [(Al_0.1Ga_0.9)₂O₃] were examined by measuring the wavelength shift in the spectral R lines. Photoluminescence (PL) spectra of these materials were collected from samples in diamond anvil cells at pressures up to 9 GPa. The β-Ga₂O₃:Cr³⁺ R lines were found to shift linearly under hydrostatic pressure. The (Al_0.1Ga_0.9)₂O₃ R lines also show a linear shift but the R₁ line shifted less than for β-Ga₂O₃:Cr³⁺. The ratio of R₂ to R₁ peak areas vs pressure is dominated by nonradiative recombination. X-ray diffraction measurements of (Al_0.1Ga_0.9)₂O₃ indicate that its equation of state is similar to that of β-Ga₂O₃. β-Ga₂O₃:Cr³⁺ was examined under non-hydrostatic conditions by using mineral oil as a pressure transmitting medium. Similar to the case in ruby, the R₁ line is much more sensitive to non-hydrostatic stress than R₂. Spatially resolved PL of a sample at 8 GPa in mineral oil showed significant variations in the R₁ emission wavelength. Furthermore, these results suggest that the R₁ line can serve as a sensitive probe of alloy composition and non-hydrostatic stress, while the R₂ line is insensitive to these perturbations.

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Research Organization:: Washington State Univ., Pullman, WA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA), Office of Defense Programs (DP); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division (MSE)

Grant/Contract Number:: NA0003957; FG02-07ER46386; AC02-05CH11231

OSTI ID:: 1986488

Alternate ID(s):: OSTI ID: 2315020

Journal Information:: Journal of Applied Physics, Vol. 133, Issue 17; ISSN 0021-8979

Publisher:: American Institute of Physics (AIP)Copyright Statement

Country of Publication:: United States

Language:: English

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Title: Photoluminescence of Cr3+ in β-Ga2O3 and (Al0.1Ga0.9)2O3 under pressure

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Title: Photoluminescence of Cr³⁺ in β-Ga₂O₃ and (Al_0.1Ga_0.9)₂O₃ under pressure