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Comparing Parallel Plastic‐to‐X Pathways and Their Role in a Circular Economy for PET Bottles

Journal Article · · Advanced Sustainable Systems
Abstract

The United States generates the most plastic waste of any country and is a top contributor to global plastic pollution. Multiple end‐of‐life strategies must be implemented to minimize environmental impacts and retain valuable plastic material, but it is challenging to compare options that generate products with different lifetimes and utilities. Herein, they present a material flow model equipped with consequential life cycle assessment, cost analysis, and a plastic circularity indicator that considers product quality and lifetime. The model is used to estimate the greenhouse gas (GHG) emissions, circularity, and cost of polyethylene terephthalate (PET) bottle mechanical downcycling to lower‐quality resin, closed‐loop glycolysis to food‐grade PET, upcycling to glass fiber‐reinforced plastic, and conversion to non‐plastic products (electricity, oil) on a United States economy‐wide basis for the year 2020. A brute force algorithm suggests that a combination of 68% glycolysis, 11% mechanical recycling, 6% upcycling, 9% landfilling, and 5% incineration can minimize the cost and GHG emissions and maximize the circularity of the current PET economy. However, uncertainty around transportation distances, materials recovery facility efficiencies, and recycling yields can result in different “optimal” pathway mixes. This flexible framework enables informed decision‐making to move toward a cost‐ and environment‐conscious circular economy for plastic.

Research Organization:
National Renewable Energy Laboratory (NREL), Golden, CO (United States)
Sponsoring Organization:
USDOE; USDOE Office of Energy Efficiency and Renewable Energy (EERE), Energy Efficiency Office. Industrial Efficiency & Decarbonization Office (IEDO)
Grant/Contract Number:
AC36-08GO28308
OSTI ID:
1985190
Alternate ID(s):
OSTI ID: 1992026
OSTI ID: 1995331
Report Number(s):
NREL/JA--6A20-85165; 2300068
Journal Information:
Advanced Sustainable Systems, Journal Name: Advanced Sustainable Systems Journal Issue: 9 Vol. 8; ISSN 2366-7486
Publisher:
Wiley Blackwell (John Wiley & Sons)Copyright Statement
Country of Publication:
Germany
Language:
English

References (29)

Beyond Mechanical Recycling: Giving New Life to Plastic Waste journal June 2020
Mechanical Recycling of Packaging Plastics: A Review journal September 2020
TRACI 2.0: the tool for the reduction and assessment of chemical and other environmental impacts 2.0 journal January 2011
Think before you throw! An analysis of behavioral interventions targeting PET bottle recycling in the United States journal June 2023
Application of life cycle assessment (LCA) for municipal solid waste management: a case study of Sakarya journal May 2015
Life cycle assessment of end-of-life treatments for plastic film waste journal November 2018
Towards a circular economy for PET bottle resin using a system dynamics inspired material flow model journal January 2023
Combining Reclaimed PET with Bio-based Monomers Enables Plastics Upcycling journal April 2019
Manufacturing energy and greenhouse gas emissions associated with plastics consumption journal January 2021
Systems Analysis for PET and Olefin Polymers in a Circular Economy journal January 2019
Towards a circular economy for plastic packaging wastes – the environmental potential of chemical recycling journal November 2020
Assessing scaling effects of circular economy strategies: A case study on plastic bottle closed-loop recycling in the USA PET market journal November 2020
Environmental and economic implications of U.S. postconsumer plastic waste management journal April 2021
Quantification and evaluation of plastic waste in the United States journal August 2022
Plastic recycling in a circular economy; determining environmental performance through an LCA matrix model approach journal February 2021
Dynamic Material Flow Analysis of PET, PE, and PP Flows in Europe: Evaluation of the Potential for Circular Economy journal November 2020
Systems Analysis Approach to Polyethylene Terephthalate and Olefin Plastics Supply Chains in the Circular Economy: A Review of Data Sets and Models journal May 2021
Consequential Life Cycle Assessment and Optimization of High-Density Polyethylene Plastic Waste Chemical Recycling journal August 2021
Material Flow Analysis and Life Cycle Assessment of Polyethylene Terephthalate and Polyolefin Plastics Supply Chains in the United States journal September 2022
Circular Economy Sustainability Analysis Framework for Plastics: Application for Poly(ethylene Terephthalate) (PET) journal January 2023
Technical, Economic, and Environmental Comparison of Closed-Loop Recycling Technologies for Common Plastics journal January 2023
System Analyses of High-Value Chemicals and Fuels from a Waste High-Density Polyethylene Refinery. Part 1: Conceptual Design and Techno-Economic Assessment journal November 2019
Plastic waste as a fuel - CO2-neutral or not? journal January 2009
Agent-embedded system dynamics (aeSD) modeling approach for analyzing worker policies: a research case on construction worker absenteeism journal May 2021
Production, use, and fate of all plastics ever made journal July 2017
Achieving net-zero greenhouse gas emission plastics by a circular carbon economy journal October 2021
Polymeric Cracking of Waste Polyethylene Terephthalate to Chemicals and Energy journal July 2011
Do We Need a New Sustainability Assessment Method for the Circular Economy? A Critical Literature Review journal January 2021
Catalytic Fast Pyrolysis of Poly (Ethylene Terephthalate) (PET) with Zeolite and Nickel Chloride journal March 2020