Bio-inspired strategies for next-generation perovskite solar mobile power sources

Yoon, Jungjin; Hou, Yuchen; Knoepfel, Abbey Marie; Yang, Dong; Ye, Tao; Zheng, Luyao; Yennawar, Neela; Sanghadasa, Mohan; Priya, Shashank; Wang, Kai

doi:10.1039/d0cs01493a

Bio-inspired strategies for next-generation perovskite solar mobile power sources

Journal Article · Fri Oct 08 00:00:00 EDT 2021 · Chemical Society Reviews

DOI:https://doi.org/10.1039/d0cs01493a· OSTI ID:1978747

Yoon, Jungjin ^[1]; ^[2]; ^[2]; Yang, Dong ^[2]; Ye, Tao ^[2]; Zheng, Luyao ^[2]; Yennawar, Neela ^[2]; Sanghadasa, Mohan ^[3]; Priya, Shashank ^[2]; ^[2]

Pennsylvania State University, University Park, PA (United States); OSTI
Pennsylvania State University, University Park, PA (United States)
U.S. Army Combat Capabilities Development Command Aviation & Missile Center, Redstone Arsenal, AL (United States)

Smart electronic devices are becoming ubiquitous due to many appealing attributes including portability, long operational time, rechargeability and compatibility with the user-desired form factor. Integration of mobile power sources (MPS) based on photovoltaic technologies with smart electronics will continue to drive improved sustainability and independence. With high efficiency, low cost, flexibility and lightweight features, halide perovskite photovoltaics have become promising candidates for MPS. Realization of these photovoltaic MPS (PV-MPS) with unconventionally extraordinary attributes requires new ‘out-of-box’ designs. Natural materials have provided promising designing solutions to engineer properties under a broad range of boundary conditions, ranging from molecules, proteins, cells, tissues, apparatus to systems in animals, plants, and humans optimized through billions of years of evolution. Applying bio-inspired strategies in PV-MPS could be biomolecular modification on crystallization at the atomic/meso-scale, bio-structural duplication at the device/system level and bio-mimicking at the functional level to render efficient charge delivery, energy transport/utilization, as well as stronger resistance against environmental stimuli (e.g., self-healing and self-cleaning). In this paper, we discuss the bio-inspired/-mimetic structures, experimental models, and working principles, with the goal of revealing physics and bio-microstructures relevant for PV-MPS. Here the emphasis is on identifying the strategies and material designs towards improvement of the performance of emerging halide perovskite PVs and strategizing their bridge to future MPS.

View Accepted Manuscript (DOE)

Research Organization:: NanoSonic Inc., Pembroke, VA (United States)

Sponsoring Organization:: Air Force Office of Scientific Research; National Science Foundation (NSF); Office of Naval Research; USDOE Office of Science (SC)

Grant/Contract Number:: SC0019844

OSTI ID:: 1978747

Journal Information:: Chemical Society Reviews, Journal Name: Chemical Society Reviews Journal Issue: 23 Vol. 50; ISSN 0306-0012

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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