Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements

Maclean, Adrian M.; Li, Ying; Crescenzo, Giuseppe V.; Smith, Natalie R.; Karydis, Vlassis A.; Tsimpidi, Alexandra P.; Butenhoff, Christopher L.; Faiola, Celia L.; Lelieveld, Jos; Nizkorodov, Sergey A.; Shiraiwa, Manabu; Bertram, Allan K.

doi:10.1021/acsearthspacechem.1c00296

Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements

Journal Article · 30 November 2021 · ACS Earth and Space Chemistry

DOI:https://doi.org/10.1021/acsearthspacechem.1c00296· OSTI ID:1978329

^[1]; Li, Ying ^[2]; ^[1]; Smith, Natalie R. ^[2]; Karydis, Vlassis A. ^[3]; Tsimpidi, Alexandra P. ^[4]; Butenhoff, Christopher L. ^[5]; ^[6]; ^[7]; ^[2]; ^[2]; ^[1]

Department of Chemistry, University of British Columbia, Vancouver, British Columbia V6T 1Z1, Canada
Department of Chemistry, University of California Irvine, Irvine, California 92697, United States
Institute of Energy & Climate Research, IEK-8: Troposphere, Forschungszentrum Jülich GmbH, 52428 Jülich, Germany
Institute of Energy & Climate Research, IEK-8: Troposphere, Forschungszentrum Jülich GmbH, 52428 Jülich, Germany; Institute for Environmental Research & Sustainable Development, National Observatory of Athens, 15236 Palea Penteli, Greece
Dept. of Physics, Portland State University, Portland, Oregon 97201, United States
Department of Chemistry, University of California Irvine, Irvine, California 92697, United States; Department of Ecology and Evolutionary Biology, University of California Irvine, Irvine, California 92697, United States
Atmospheric Chemistry Department, Max Planck Institute for Chemistry, 55128 Mainz, Germany; Climate and Atmosphere Research Center, The Cyprus Institute, 1645 Nicosia, Cyprus

Not provided.

Research Organization:: Univ. of California, Irvine, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

DOE Contract Number:: SC0018349; SC0022139

OSTI ID:: 1978329

Journal Information:: ACS Earth and Space Chemistry, Vol. 5, Issue 12; ISSN 2472-3452

Publisher:: American Chemical Society (ACS)

Country of Publication:: United States

Language:: English

References (113)

Secondary organic aerosol formation in cloud droplets and aqueous particles (aqSOA): a review of laboratory, field and model studies Ervens, B.; Turpin, B. J.; Weber, R. J. Atmospheric Chemistry and Physics, Vol. 11, Issue 21 https://doi.org/10.5194/acp-11-11069-2011	journal	January 2011
The formation, properties and impact of secondary organic aerosol: current and emerging issues Hallquist, M.; Wenger, J. C.; Baltensperger, U. Atmospheric Chemistry and Physics, Vol. 9, Issue 14 https://doi.org/10.5194/acp-9-5155-2009	journal	January 2009
Aerosol Health Effects from Molecular to Global Scales Shiraiwa, Manabu; Ueda, Kayo; Pozzer, Andrea Environmental Science & Technology, Vol. 51, Issue 23 https://doi.org/10.1021/acs.est.7b04417	journal	November 2017
Health Effects of Fine Particulate Air Pollution: Lines that Connect Pope, C. Arden; Dockery, Douglas W. Journal of the Air & Waste Management Association, Vol. 56, Issue 6 https://doi.org/10.1080/10473289.2006.10464485	journal	June 2006
The contribution of outdoor air pollution sources to premature mortality on a global scale Lelieveld, J.; Evans, J. S.; Fnais, M. Nature, Vol. 525, Issue 7569 https://doi.org/10.1038/nature15371	journal	September 2015
Clean air in the Anthropocene Lelieveld, Jos Faraday Discussions, Vol. 200 https://doi.org/10.1039/c7fd90032e	journal	January 2017
Glass transition and phase state of organic compounds: dependency on molecular properties and implications for secondary organic aerosols in the atmosphere Koop, Thomas; Bookhold, Johannes; Shiraiwa, Manabu Physical Chemistry Chemical Physics, Vol. 13, Issue 43 https://doi.org/10.1039/c1cp22617g	journal	January 2011
Heterogeneous ice nucleation of viscous secondary organic aerosol produced from ozonolysis of α -pinene Ignatius, Karoliina; Kristensen, Thomas B.; Järvinen, Emma Atmospheric Chemistry and Physics, Vol. 16, Issue 10 https://doi.org/10.5194/acp-16-6495-2016	journal	January 2016
Heterogeneous nucleation of ice particles on glassy aerosols under cirrus conditions Murray, Benjamin J.; Wilson, Theodore W.; Dobbie, Steven Nature Geoscience, Vol. 3, Issue 4 https://doi.org/10.1038/ngeo817	journal	March 2010
Ice cloud processing of ultra-viscous/glassy aerosol particles leads to enhanced ice nucleation ability Wagner, R.; Möhler, O.; Saathoff, H. Atmospheric Chemistry and Physics, Vol. 12, Issue 18 https://doi.org/10.5194/acp-12-8589-2012	journal	January 2012
The Role of Organic Aerosol in Atmospheric Ice Nucleation: A Review Knopf, Daniel A.; Alpert, Peter A.; Wang, Bingbing ACS Earth and Space Chemistry, Vol. 2, Issue 3 https://doi.org/10.1021/acsearthspacechem.7b00120	journal	January 2018
A biogenic secondary organic aerosol source of cirrus ice nucleating particles Wolf, Martin J.; Zhang, Yue; Zawadowicz, Maria A. Nature Communications, Vol. 11, Issue 1 https://doi.org/10.1038/s41467-020-18424-6	journal	October 2020
Competition between water uptake and ice nucleation by glassy organic aerosol particles Berkemeier, T.; Shiraiwa, M.; Pöschl, U. Atmospheric Chemistry and Physics, Vol. 14, Issue 22 https://doi.org/10.5194/acp-14-12513-2014	journal	January 2014
Modeling kinetic partitioning of secondary organic aerosol and size distribution dynamics: representing effects of volatility, phase state, and particle-phase reaction Zaveri, R. A.; Easter, R. C.; Shilling, J. E. Atmospheric Chemistry and Physics, Vol. 14, Issue 10 https://doi.org/10.5194/acp-14-5153-2014	journal	January 2014
Growth Kinetics and Size Distribution Dynamics of Viscous Secondary Organic Aerosol Zaveri, Rahul A.; Shilling, John E.; Zelenyuk, Alla Environmental Science & Technology, Vol. 52, Issue 3 https://doi.org/10.1021/acs.est.7b04623	journal	January 2018
Size distribution dynamics reveal particle-phase chemistry in organic aerosol formation Shiraiwa, M.; Yee, L. D.; Schilling, K. A. Proceedings of the National Academy of Sciences, Vol. 110, Issue 29 https://doi.org/10.1073/pnas.1307501110	journal	July 2013
Modeling the effect of non-ideality, dynamic mass transfer and viscosity on SOA formation in a 3-D air quality model Kim, Youngseob; Sartelet, Karine; Couvidat, Florian Atmospheric Chemistry and Physics, Vol. 19, Issue 2 https://doi.org/10.5194/acp-19-1241-2019	journal	January 2019
Factors controlling the evaporation of secondary organic aerosol from α‐pinene ozonolysis Yli‐Juuti, Taina; Pajunoja, Aki; Tikkanen, Olli‐Pekka Geophysical Research Letters, Vol. 44, Issue 5 https://doi.org/10.1002/2016GL072364	journal	March 2017
Effect of the Aerosol-Phase State on Secondary Organic Aerosol Formation from the Reactive Uptake of Isoprene-Derived Epoxydiols (IEPOX) Zhang, Yue; Chen, Yuzhi; Lambe, Andrew T. Environmental Science & Technology Letters, Vol. 5, Issue 3 https://doi.org/10.1021/acs.estlett.8b00044	journal	February 2018
The influence of physical state on shikimic acid ozonolysis: a case for in situ microspectroscopy Steimer, S. S.; Lampimäki, M.; Coz, E. Atmospheric Chemistry and Physics, Vol. 14, Issue 19 https://doi.org/10.5194/acp-14-10761-2014	journal	January 2014
Highly Viscous States Affect the Browning of Atmospheric Organic Particulate Matter Liu, Pengfei; Li, Yong Jie; Wang, Yan ACS Central Science, Vol. 4, Issue 2 https://doi.org/10.1021/acscentsci.7b00452	journal	January 2018
Influence of relative humidity on the heterogeneous oxidation of secondary organic aerosol Li, Ziyue; Smith, Katherine A.; Cappa, Christopher D. Atmospheric Chemistry and Physics, Vol. 18, Issue 19 https://doi.org/10.5194/acp-18-14585-2018	journal	January 2018
Gas uptake and chemical aging of semisolid organic aerosol particles Shiraiwa, M.; Ammann, M.; Koop, T. Proceedings of the National Academy of Sciences, Vol. 108, Issue 27 https://doi.org/10.1073/pnas.1103045108	journal	June 2011
Chemical Reactivity and Liquid/Nonliquid States of Secondary Organic Material Li, Yong Jie; Liu, Pengfei; Gong, Zhaoheng Environmental Science & Technology, Vol. 49, Issue 22 https://doi.org/10.1021/acs.est.5b03392	journal	October 2015
Heterogeneous oxidation of amorphous organic aerosol surrogates by O₃, NO₃, and OH at typical tropospheric temperatures Li, Jienan; Forrester, Seanna M.; Knopf, Daniel A. Atmospheric Chemistry and Physics, Vol. 20, Issue 10 https://doi.org/10.5194/acp-20-6055-2020	journal	January 2020
Interfacial Dimerization by Organic Radical Reactions during Heterogeneous Oxidative Aging of Oxygenated Organic Aerosols Zhao, Zixu; Tolentino, Ricardo; Lee, Jennifer The Journal of Physical Chemistry A, Vol. 123, Issue 50 https://doi.org/10.1021/acs.jpca.9b10779	journal	November 2019
Experimental determination of chemical diffusion within secondary organic aerosol particles Abramson, Evan; Imre, Dan; Beránek, Josef Physical Chemistry Chemical Physics, Vol. 15, Issue 8 https://doi.org/10.1039/c2cp44013j	journal	January 2013
Effect of varying experimental conditions on the viscosity of α -pinene derived secondary organic material Grayson, James W.; Zhang, Yue; Mutzel, Anke Atmospheric Chemistry and Physics, Vol. 16, Issue 10 https://doi.org/10.5194/acp-16-6027-2016	journal	January 2016
Diffusion of Organic Molecules as a Function of Temperature in a Sucrose Matrix (a Proxy for Secondary Organic Aerosol) Kiland, Kristian J.; Maclean, Adrian M.; Kamal, Saeid The Journal of Physical Chemistry Letters, Vol. 10, Issue 19 https://doi.org/10.1021/acs.jpclett.9b02182	journal	September 2019
Unified Description of Diffusion Coefficients from Small to Large Molecules in Organic–Water Mixtures Evoy, Erin; Kamal, Saeid; Patey, Grenfell N. The Journal of Physical Chemistry A, Vol. 124, Issue 11 https://doi.org/10.1021/acs.jpca.9b11271	journal	February 2020
Predictions of diffusion rates of large organic molecules in secondary organic aerosols using the Stokes–Einstein and fractional Stokes–Einstein relations Evoy, Erin; Maclean, Adrian M.; Rovelli, Grazia Atmospheric Chemistry and Physics, Vol. 19, Issue 15 https://doi.org/10.5194/acp-19-10073-2019	journal	January 2019
Diffusivity measurements of volatile organics in levitated viscous aerosol particles Bastelberger, Sandra; Krieger, Ulrich K.; Luo, Beiping Atmospheric Chemistry and Physics, Vol. 17, Issue 13 https://doi.org/10.5194/acp-17-8453-2017	journal	January 2017
The viscosity of atmospherically relevant organic particles Reid, Jonathan P.; Bertram, Allan K.; Topping, David O. Nature Communications, Vol. 9, Issue 1 https://doi.org/10.1038/s41467-018-03027-z	journal	March 2018
A predictive group-contribution model for the viscosity of aqueous organic aerosol Gervasi, Natalie R.; Topping, David O.; Zuend, Andreas Atmospheric Chemistry and Physics, Vol. 20, Issue 5 https://doi.org/10.5194/acp-20-2987-2020	journal	January 2020
Lability of secondary organic particulate matter Liu, Pengfei; Li, Yong Jie; Wang, Yan Proceedings of the National Academy of Sciences, Vol. 113, Issue 45 https://doi.org/10.1073/pnas.1603138113	journal	October 2016
Viscosity of -pinene secondary organic material and implications for particle growth and reactivity Renbaum-Wolff, L.; Grayson, J. W.; Bateman, A. P. Proceedings of the National Academy of Sciences, Vol. 110, Issue 20 https://doi.org/10.1073/pnas.1219548110	journal	April 2013
Ultra-slow water diffusion in aqueous sucrose glasses Zobrist, Bernhard; Soonsin, Vacharaporn; Luo, Bei P. Physical Chemistry Chemical Physics, Vol. 13, Issue 8 https://doi.org/10.1039/c0cp01273d	journal	January 2011
The Cooling Rate- and Volatility-Dependent Glass-Forming Properties of Organic Aerosols Measured by Broadband Dielectric Spectroscopy Zhang, Yue; Nichman, Leonid; Spencer, Peyton Environmental Science & Technology, Vol. 53, Issue 21 https://doi.org/10.1021/acs.est.9b03317	journal	September 2019
Timescales of secondary organic aerosols to reach equilibrium at various temperatures and relative humidities Li, Ying; Shiraiwa, Manabu Atmospheric Chemistry and Physics, Vol. 19, Issue 9 https://doi.org/10.5194/acp-19-5959-2019	journal	January 2019
Relative humidity-dependent viscosity of secondary organic material from toluene photo-oxidation and possible implications for organic particulate matter over megacities Song, Mijung; Liu, Pengfei F.; Hanna, Sarah J. Atmospheric Chemistry and Physics, Vol. 16, Issue 14 https://doi.org/10.5194/acp-16-8817-2016	journal	January 2016
An amorphous solid state of biogenic secondary organic aerosol particles Virtanen, Annele; Joutsensaari, Jorma; Koop, Thomas Nature, Vol. 467, Issue 7317 https://doi.org/10.1038/nature09455	journal	October 2010
Mixing times of organic molecules within secondary organic aerosol particles: a global planetary boundary layer perspective Maclean, Adrian M.; Butenhoff, Christopher L.; Grayson, James W. Atmospheric Chemistry and Physics, Vol. 17, Issue 21 https://doi.org/10.5194/acp-17-13037-2017	journal	January 2017
Global distribution of particle phase state in atmospheric secondary organic aerosols Shiraiwa, Manabu; Li, Ying; Tsimpidi, Alexandra P. Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms15002	journal	April 2017
Predicting secondary organic aerosol phase state and viscosity and its effect on multiphase chemistry in a regional-scale air quality model Schmedding, Ryan; Rasool, Quazi Z.; Zhang, Yue Atmospheric Chemistry and Physics, Vol. 20, Issue 13 https://doi.org/10.5194/acp-20-8201-2020	journal	January 2020
Diurnal and Seasonal Variations in the Phase State of Secondary Organic Aerosol Material over the Contiguous US Simulated in CMAQ Li, Ying; Carlton, Annmarie G.; Shiraiwa, Manabu ACS Earth and Space Chemistry, Vol. 5, Issue 8 https://doi.org/10.1021/acsearthspacechem.1c00094	journal	July 2021
Organic condensation: a vital link connecting aerosol formation to cloud condensation nuclei (CCN) concentrations Riipinen, I.; Pierce, J. R.; Yli-Juuti, T. Atmospheric Chemistry and Physics, Vol. 11, Issue 8 https://doi.org/10.5194/acp-11-3865-2011	journal	January 2011
Rainforest Aerosols as Biogenic Nuclei of Clouds and Precipitation in the Amazon Poschl, U.; Martin, S. T.; Sinha, B. Science, Vol. 329, Issue 5998 https://doi.org/10.1126/science.1191056	journal	September 2010
An overview of the Amazonian Aerosol Characterization Experiment 2008 (AMAZE-08) Martin, S. T.; Andreae, M. O.; Althausen, D. Atmospheric Chemistry and Physics, Vol. 10, Issue 23 https://doi.org/10.5194/acp-10-11415-2010	journal	January 2010
MWH's Water Treatment: Principles and Design Crittenden, John C.; Trussell, R. Rhodes; Hand, David W. https://doi.org/10.1002/9781118131473	book	March 2012
Secondary Organic Aerosol Formation from Healthy and Aphid-Stressed Scots Pine Emissions Faiola, Celia L.; Pullinen, Iida; Buchholz, Angela ACS Earth and Space Chemistry, Vol. 3, Issue 9 https://doi.org/10.1021/acsearthspacechem.9b00118	journal	August 2019
Multi-layered Scots pine forests in boreal Sweden result from mass regeneration and size stratification Lundqvist, Lars; Ahlström, Martin A.; Petter Axelsson, E. Forest Ecology and Management, Vol. 441 https://doi.org/10.1016/j.foreco.2019.03.044	journal	June 2019
Composition and volatility of secondary organic aerosol (SOA) formed from oxidation of real tree emissions compared to simplified volatile organic compound (VOC) systems Ylisirniö, Arttu; Buchholz, Angela; Mohr, Claudia Atmospheric Chemistry and Physics, Vol. 20, Issue 9 https://doi.org/10.5194/acp-20-5629-2020	journal	January 2020
Secondary organic aerosol from VOC mixtures in an oxidation flow reactor Ahlberg, Erik; Falk, John; Eriksson, Axel Atmospheric Environment, Vol. 161 https://doi.org/10.1016/j.atmosenv.2017.05.005	journal	July 2017
Secondary organic aerosol reduced by mixture of atmospheric vapours McFiggans, Gordon; Mentel, Thomas F.; Wildt, Jürgen Nature, Vol. 565, Issue 7741 https://doi.org/10.1038/s41586-018-0871-y	journal	January 2019
Terpene Composition Complexity Controls Secondary Organic Aerosol Yields from Scots Pine Volatile Emissions Faiola, C. L.; Buchholz, A.; Kari, E. Scientific Reports, Vol. 8, Issue 1 https://doi.org/10.1038/s41598-018-21045-1	journal	February 2018
Relaxation in liquids, polymers and plastic crystals — strong/fragile patterns and problems Angell, C. A. Journal of Non-Crystalline Solids, Vol. 131-133 https://doi.org/10.1016/0022-3093(91)90266-9	journal	June 1991
Liquid Fragility and the Glass Transition in Water and Aqueous Solutions Angell, C. A. Chemical Reviews, Vol. 102, Issue 8 https://doi.org/10.1021/cr000689q	journal	August 2002
Entropy and fragility in supercooling liquids Angell, C. A. Journal of Research of the National Institute of Standards and Technology, Vol. 102, Issue 2 https://doi.org/10.6028/jres.102.013	journal	March 1997
Predicting the glass transition temperature and viscosity of secondary organic material using molecular composition DeRieux, Wing-Sy Wong; Li, Ying; Lin, Peng Atmospheric Chemistry and Physics, Vol. 18, Issue 9 https://doi.org/10.5194/acp-18-6331-2018	journal	January 2018
Viscosity of concentrated sucrose and trehalose aqueous solutions including the supercooled regime Longinotti, M. Paula; Corti, Horacio R. Journal of Physical and Chemical Reference Data, Vol. 37, Issue 3 https://doi.org/10.1063/1.2932114	journal	September 2008
Toward closure between predicted and observed particle viscosity over a wide range of temperatures and relative humidity Kasparoglu, Sabin; Li, Ying; Shiraiwa, Manabu Atmospheric Chemistry and Physics, Vol. 21, Issue 2 https://doi.org/10.5194/acp-21-1127-2021	journal	January 2021
Estimating Secondary Organic Aerosol Production from Toluene Photochemistry in a Megacity of China Gao, Yaqin; Wang, Hongli; Zhang, Xuan Environmental Science & Technology, Vol. 53, Issue 15 https://doi.org/10.1021/acs.est.9b00651	journal	July 2019
Organic Aerosol Mixing Observed by Single-Particle Mass Spectrometry Robinson, Ellis Shipley; Saleh, Rawad; Donahue, Neil M. The Journal of Physical Chemistry A, Vol. 117, Issue 51 https://doi.org/10.1021/jp405789t	journal	November 2013
Liquid–liquid phase separation and viscosity within secondary organic aerosol generated from diesel fuel vapors Song, Mijung; Maclean, Adrian M.; Huang, Yuanzhou Atmospheric Chemistry and Physics, Vol. 19, Issue 19 https://doi.org/10.5194/acp-19-12515-2019	journal	January 2019
Elucidating secondary organic aerosol from diesel and gasoline vehicles through detailed characterization of organic carbon emissions Gentner, D. R.; Isaacman, G.; Worton, D. R. Proceedings of the National Academy of Sciences, Vol. 109, Issue 45 https://doi.org/10.1073/pnas.1212272109	journal	October 2012
The Atmospheric Aerosol-Forming Potential of Whole Gasoline Vapor Odum, J. R. Science, Vol. 276, Issue 5309 https://doi.org/10.1126/science.276.5309.96	journal	April 1997
Distribution, magnitudes, reactivities, ratios and diurnal patterns of volatile organic compounds in the Valley of Mexico during the MCMA 2002 & 2003 field campaigns Velasco, E.; Lamb, B.; Westberg, H. Atmospheric Chemistry and Physics, Vol. 7, Issue 2 https://doi.org/10.5194/acp-7-329-2007	journal	January 2007
Eddy covariance flux measurements of pollutant gases in urban Mexico City Velasco, E.; Pressley, S.; Grivicke, R. Atmospheric Chemistry and Physics, Vol. 9, Issue 19 https://doi.org/10.5194/acp-9-7325-2009	journal	January 2009
Temperature dependence of yields of secondary organic aerosols from the ozonolysis of α -pinene and limonene Saathoff, H.; Naumann, K. -H.; Möhler, O. Atmospheric Chemistry and Physics, Vol. 9, Issue 5 https://doi.org/10.5194/acp-9-1551-2009	journal	January 2009
Second-generation products contribute substantially to the particle-phase organic material produced by β-caryophyllene ozonolysis Li, Y. J.; Chen, Q.; Guzman, M. I. Atmospheric Chemistry and Physics, Vol. 11, Issue 1 https://doi.org/10.5194/acp-11-121-2011	journal	January 2011
Effect of relative humidity on the composition of secondary organic aerosol from the oxidation of toluene Hinks, Mallory L.; Montoya-Aguilera, Julia; Ellison, Lucas Atmospheric Chemistry and Physics, Vol. 18, Issue 3 https://doi.org/10.5194/acp-18-1643-2018	journal	January 2018
Real-Time Aerosol Density Determination Utilizing a Modified Scanning Mobility Particle Sizer—Aerosol Particle Mass Analyzer System Malloy, Quentin G. J.; Nakao, Shunsuke; Qi, Li Aerosol Science and Technology, Vol. 43, Issue 7 https://doi.org/10.1080/02786820902832960	journal	June 2009
Formation and chemical aging of secondary organic aerosol during the β-caryophyllene oxidation Tasoglou, A.; Pandis, S. N. Atmospheric Chemistry and Physics, Vol. 15, Issue 11 https://doi.org/10.5194/acp-15-6035-2015	journal	January 2015
Laboratory and Ambient Particle Density Determinations using Light Scattering in Conjunction with Aerosol Mass Spectrometry Cross, Eben S.; Slowik, Jay G.; Davidovits, Paul Aerosol Science and Technology, Vol. 41, Issue 4 https://doi.org/10.1080/02786820701199736	journal	March 2007
Measurements of Secondary Organic Aerosol from Oxidation of Cycloalkenes, Terpenes, and m -Xylene Using an Aerodyne Aerosol Mass Spectrometer Bahreini, R.; Keywood, M. D.; Ng, N. L. Environmental Science & Technology, Vol. 39, Issue 15 https://doi.org/10.1021/es048061a	journal	August 2005
Secondary organic aerosol formation from m-xylene, toluene, and benzene Ng, N. L.; Kroll, J. H.; Chan, A. W. H. Atmospheric Chemistry and Physics, Vol. 7, Issue 14 https://doi.org/10.5194/acp-7-3909-2007	journal	January 2007
The Temperature Dependence of the Viscosity of Supercooled Water Hallett, J. Proceedings of the Physical Society, Vol. 82, Issue 6 https://doi.org/10.1088/0370-1328/82/6/326	journal	December 1963
ORACLE (v1.0): module to simulate the organic aerosol composition and evolution in the atmosphere Tsimpidi, A. P.; Karydis, V. A.; Pozzer, A. Geoscientific Model Development, Vol. 7, Issue 6 https://doi.org/10.5194/gmd-7-3153-2014	journal	January 2014
ORACLE 2-D (v2.0): an efficient module to compute the volatility and oxygen content of organic aerosol with a global chemistry–climate model Tsimpidi, Alexandra P.; Karydis, Vlassis A.; Pozzer, Andrea Geoscientific Model Development, Vol. 11, Issue 8 https://doi.org/10.5194/gmd-11-3369-2018	journal	January 2018
Molecular corridors and kinetic regimes in the multiphase chemical evolution of secondary organic aerosol Shiraiwa, M.; Berkemeier, T.; Schilling-Fahnestock, K. A. Atmospheric Chemistry and Physics, Vol. 14, Issue 16 https://doi.org/10.5194/acp-14-8323-2014	journal	January 2014
Aerosol mass spectrometer constraint on the global secondary organic aerosol budget Spracklen, D. V.; Jimenez, J. L.; Carslaw, K. S. Atmospheric Chemistry and Physics, Vol. 11, Issue 23 https://doi.org/10.5194/acp-11-12109-2011	journal	January 2011
Molecular and physical characteristics of aerosol at a remote free troposphere site: implications for atmospheric aging Schum, Simeon K.; Zhang, Bo; Džepina, Katja Atmospheric Chemistry and Physics, Vol. 18, Issue 19 https://doi.org/10.5194/acp-18-14017-2018	journal	January 2018
Volatility and Viscosity Are Correlated in Terpene Secondary Organic Aerosol Formed in a Flow Reactor Champion, Wyatt M.; Rothfuss, Nicholas E.; Petters, Markus D. Environmental Science & Technology Letters, Vol. 6, Issue 9 https://doi.org/10.1021/acs.estlett.9b00412	journal	August 2019
Humidity-dependent phase state of SOA particles from biogenic and anthropogenic precursors Saukko, E.; Lambe, A. T.; Massoli, P. Atmospheric Chemistry and Physics, Vol. 12, Issue 16 https://doi.org/10.5194/acp-12-7517-2012	journal	January 2012
Predictions of the glass transition temperature and viscosity of organic aerosols from volatility distributions Li, Ying; Day, Douglas A.; Stark, Harald Atmospheric Chemistry and Physics, Vol. 20, Issue 13 https://doi.org/10.5194/acp-20-8103-2020	journal	January 2020
The Influence of Absolute Mass Loading of Secondary Organic Aerosols on Their Phase State Jain, Shashank; Fischer, Kevin; Petrucci, Giuseppe Atmosphere, Vol. 9, Issue 4, p. 131 https://doi.org/10.3390/atmos9040131	journal	March 2018
Global combustion sources of organic aerosols: model comparison with 84 AMS factor-analysis data sets Tsimpidi, Alexandra P.; Karydis, Vlassis A.; Pandis, Spyros N. Atmospheric Chemistry and Physics, Vol. 16, Issue 14 https://doi.org/10.5194/acp-16-8939-2016	journal	January 2016
Model of Emissions of Gases and Aerosol from Nature Version 3 (MEGAN3) for Estimating Biogenic Emissions Guenther, Alex; Jiang, Xiaoyan; Shah, Tejas Air Pollution Modeling and its Application XXVI https://doi.org/10.1007/978-3-030-22055-6_29	book	November 2019
Relative humidity-dependent viscosities of isoprene-derived secondary organic material and atmospheric implications for isoprene-dominant forests Song, M.; Liu, P. F.; Hanna, S. J. Atmospheric Chemistry and Physics, Vol. 15, Issue 9 https://doi.org/10.5194/acp-15-5145-2015	journal	January 2015
Effects of Molecular-Level Compositional Variability in Organic Aerosol on Phase State and Thermodynamic Mixing Behavior Ditto, Jenna C.; Joo, Taekyu; Khare, Peeyush Environmental Science & Technology, Vol. 53, Issue 22 https://doi.org/10.1021/acs.est.9b02664	journal	September 2019
Sub-micrometre particulate matter is primarily in liquid form over Amazon rainforest Bateman, Adam P.; Gong, Zhaoheng; Liu, Pengfei Nature Geoscience, Vol. 9, Issue 1 https://doi.org/10.1038/ngeo2599	journal	December 2015
Mixing of secondary organic aerosols versus relative humidity Ye, Qing; Robinson, Ellis Shipley; Ding, Xiang Proceedings of the National Academy of Sciences, Vol. 113, Issue 45 https://doi.org/10.1073/pnas.1604536113	journal	October 2016
Phase state of ambient aerosol linked with water uptake and chemical aging in the southeastern US Pajunoja, Aki; Hu, Weiwei; Leong, Yu J. Atmospheric Chemistry and Physics, Vol. 16, Issue 17 https://doi.org/10.5194/acp-16-11163-2016	journal	January 2016
Anthropogenic influences on the physical state of submicron particulate matter over a tropical forest Bateman, Adam P.; Gong, Zhaoheng; Harder, Tristan H. Atmospheric Chemistry and Physics, Vol. 17, Issue 3 https://doi.org/10.5194/acp-17-1759-2017	journal	January 2017
Speculations on the movement of polluted air to the Arctic Carlson, Toby N. Atmospheric Environment (1967), Vol. 15, Issue 8 https://doi.org/10.1016/0004-6981(81)90354-1	journal	January 1981
The Saharan Aerosol Long-Range Transport and Aerosol–Cloud-Interaction Experiment: Overview and Selected Highlights Weinzierl, Bernadett; Ansmann, A.; Prospero, J. M. Bulletin of the American Meteorological Society, Vol. 98, Issue 7 https://doi.org/10.1175/bams-d-15-00142.1	journal	July 2017
Aerosol particles at a high-altitude site on the Southeast Tibetan Plateau, China: Implications for pollution transport from South Asia: AEROSOL PARTICLES IN SOUTHEAST TP Zhao, Zhuzi; Cao, Junji; Shen, Zhenxing Journal of Geophysical Research: Atmospheres, Vol. 118, Issue 19 https://doi.org/10.1002/jgrd.50599	journal	October 2013
Synergy between Secondary Organic Aerosols and Long-Range Transport of Polycyclic Aromatic Hydrocarbons Zelenyuk, Alla; Imre, Dan; Beránek, Josef Environmental Science & Technology, Vol. 46, Issue 22 https://doi.org/10.1021/es302743z	journal	November 2012
Temperature effect on phase state and reactivity controls atmospheric multiphase chemistry and transport of PAHs Mu, Qing; Shiraiwa, Manabu; Octaviani, Mega Science Advances, Vol. 4, Issue 3 https://doi.org/10.1126/sciadv.aap7314	journal	March 2018
Global long-range transport and lung cancer risk from polycyclic aromatic hydrocarbons shielded by coatings of organic aerosol Shrivastava, Manish; Lou, Silja; Zelenyuk, Alla Proceedings of the National Academy of Sciences, Vol. 114, Issue 6 https://doi.org/10.1073/pnas.1618475114	journal	January 2017
Assessing the Influence of Secondary Organic versus Primary Carbonaceous Aerosols on Long-Range Atmospheric Polycyclic Aromatic Hydrocarbon Transport Friedman, C. L.; Pierce, J. R.; Selin, N. E. Environmental Science & Technology, Vol. 48, Issue 6 https://doi.org/10.1021/es405219r	journal	March 2014
Climate Change Effects on Secondary Compounds of Forest Trees in the Northern Hemisphere Holopainen, Jarmo K.; Virjamo, Virpi; Ghimire, Rajendra P. Frontiers in Plant Science, Vol. 9 https://doi.org/10.3389/fpls.2018.01445	journal	October 2018
Amplification of plant volatile defence against insect herbivory in a warming Arctic tundra Li, Tao; Holst, Thomas; Michelsen, Anders Nature Plants, Vol. 5, Issue 6 https://doi.org/10.1038/s41477-019-0439-3	journal	June 2019
Heat Waves Change Plant Carbon Allocation Among Primary and Secondary Metabolism Altering CO2 Assimilation, Respiration, and VOC Emissions Werner, Christiane; Fasbender, Lukas; Romek, Katarzyna M. Frontiers in Plant Science, Vol. 11 https://doi.org/10.3389/fpls.2020.01242	journal	August 2020
Testing various mixing rules for calculation of viscosity of petroleum blends Centeno, Guillermo; Sánchez-Reyna, Gabriela; Ancheyta, Jorge Fuel, Vol. 90, Issue 12 https://doi.org/10.1016/j.fuel.2011.02.028	journal	December 2011
Comparison of Approaches for Measuring and Predicting the Viscosity of Ternary Component Aerosol Particles Rovelli, Grazia; Song, Young-Chul; Maclean, Adrian M. Analytical Chemistry, Vol. 91, Issue 8 https://doi.org/10.1021/acs.analchem.8b05353	journal	February 2019
Measurements and Predictions of Binary Component Aerosol Particle Viscosity Song, Young Chul; Haddrell, Allen E.; Bzdek, Bryan R. The Journal of Physical Chemistry A, Vol. 120, Issue 41 https://doi.org/10.1021/acs.jpca.6b07835	journal	October 2016
Joint Impacts of Acidity and Viscosity on the Formation of Secondary Organic Aerosol from Isoprene Epoxydiols (IEPOX) in Phase Separated Particles Zhang, Yue; Chen, Yuzhi; Lei, Ziying ACS Earth and Space Chemistry, Vol. 3, Issue 12 https://doi.org/10.1021/acsearthspacechem.9b00209	journal	October 2019
Increasing Isoprene Epoxydiol-to-Inorganic Sulfate Aerosol Ratio Results in Extensive Conversion of Inorganic Sulfate to Organosulfur Forms: Implications for Aerosol Physicochemical Properties Riva, Matthieu; Chen, Yuzhi; Zhang, Yue Environmental Science & Technology, Vol. 53, Issue 15 https://doi.org/10.1021/acs.est.9b01019	journal	June 2019
Hygroscopic properties of aerosol particles at high relative humidity and their diurnal variations in the North China Plain Liu, P. F.; Zhao, C. S.; Göbel, T. Atmospheric Chemistry and Physics, Vol. 11, Issue 7 https://doi.org/10.5194/acp-11-3479-2011	journal	January 2011
Diurnal variations of cloud and relative humidity profiles across the tropics Chepfer, H.; Brogniez, H.; Noel, V. Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-52437-6	journal	November 2019
Diurnal variation of upper tropospheric humidity and its relations to convective activities over tropical Africa Chung, E. S.; Sohn, B. J.; Schmetz, J. Atmospheric Chemistry and Physics, Vol. 7, Issue 10 https://doi.org/10.5194/acp-7-2489-2007	journal	January 2007
Diurnal Variation in the Troposphere's Energy Balance Foltz, Gary S.; Gray, William M. Journal of the Atmospheric Sciences, Vol. 36, Issue 8 https://doi.org/10.1175/1520-0469(1979)036<1450:dvitte>2.0.co;2	journal	August 1979

Similar Records

Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements

Journal Article · 2021 · ACS Earth and Space Chemistry · OSTI ID:1843603

Maclean, Adrian M.; Li, Ying; Crescenzo, Giuseppe V.; +9 more

Global Simulations of Phase State and Equilibration Time Scales of Secondary Organic Aerosols with GEOS-Chem

Journal Article · 2025 · ACS Earth and Space Chemistry · OSTI ID:2514548

Luu, Regina; Schervish, Meredith; June, Nicole A.; +4 more

Related Subjects

Chemistry
Geochemistry & Geophysics

Global Distribution of the Phase State and Mixing Times within Secondary Organic Aerosol Particles in the Troposphere Based on Room-Temperature Viscosity Measurements

Citation Formats

References (113)

Similar Records

Related Subjects