Effects of processing temperature on the corrosion and tribocorrosion resistance of perhydropolysilazane-derived coatings on AISI 304 steel

Wang, Wenbo; Tamakloe, Senam; Deng, Zhifei; Li, Ling; Cai, Wenjun; Lu, Kathy

doi:10.1016/j.surfcoat.2022.128463

Effects of processing temperature on the corrosion and tribocorrosion resistance of perhydropolysilazane-derived coatings on AISI 304 steel

Journal Article · Thu Apr 21 00:00:00 EDT 2022 · Surface and Coatings Technology

DOI:https://doi.org/10.1016/j.surfcoat.2022.128463· OSTI ID:1977677

Wang, Wenbo ^[1]; Tamakloe, Senam ^[2]; Deng, Zhifei ^[2]; Li, Ling ^[2]; Cai, Wenjun ^[2]; Lu, Kathy ^[2]

Virginia Polytechnic Inst. and State Univ. (Virginia Tech), Blacksburg, VA (United States); OSTI
Virginia Polytechnic Inst. and State Univ. (Virginia Tech), Blacksburg, VA (United States)

Ensuring a highly corrosion and erosion resistant surface is critical to the reliability and structural integrity of steel canisters for long-term nuclear waste storage in corrosive environments. In this work, perhydropolysilazane (PHPS)-derived coating has been successfully applied to enhance the pitting and tribocorrosion resistance of 304 stainless steels in 0.6 M NaCl solution. Two types of coatings were synthesized on the stainless steel substrate by crosslinking PHPS at room temperature or 600 °C, resulting in different mechanical and corrosion performance. Further, Raman spectra revealed that Si-O bonds were generated in the coating crosslinked at room temperature after corrosion, while absent in that pyrolyzed at 600 °C. In tribocorrosion tests, both coatings were protective to the steel substrate, with the protective effect being more pronounced in the 600 °C pyrolyzed coating. Overall, the PHPS-derived coating synthesized at 600 °C exhibited better protection for steel in wear and corrosion coexisting environments than those synthesized at room temperature.

View Accepted Manuscript (DOE)

Research Organization:: Virginia Polytechnic Inst. and State Univ. (Virginia Tech), Blacksburg, VA (United States)

Sponsoring Organization:: National Science Foundation (NSF); USDOE; USDOE Office of Nuclear Energy (NE)

Grant/Contract Number:: NE0008963

OSTI ID:: 1977677

Alternate ID(s):: OSTI ID: 1867525

Journal Information:: Surface and Coatings Technology, Journal Name: Surface and Coatings Technology Journal Issue: C Vol. 439; ISSN 0257-8972

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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36 MATERIALS SCIENCE
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corrosion
nuclear waste canisters
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tribocorrosion

Effects of processing temperature on the corrosion and tribocorrosion resistance of perhydropolysilazane-derived coatings on AISI 304 steel

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