Challenges and opportunities for adsorption-based CO2 capture from natural gas combined cycle emissions

Siegelman, Rebecca L.; Milner, Phillip J.; Kim, Eugene J.; Weston, Simon C.; Long, Jeffrey R.

doi:10.1039/c9ee00505f

Title: Challenges and opportunities for adsorption-based CO₂ capture from natural gas combined cycle emissions

Journal Article · Wed May 08 00:00:00 EDT 2019 · Energy & Environmental Science

DOI:https://doi.org/10.1039/c9ee00505f· OSTI ID:1975809

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^[2]; Kim, Eugene J. ^[3];

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University of California, Berkeley, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
University of California, Berkeley, CA (United States); Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States); Cornell University, Ithaca, NY (United States)
University of California, Berkeley, CA (United States)
ExxonMobil Research and Engineering Company, Annandale, NJ (United States)

In recent years, the power sector has shown a growing reliance on natural gas, a cleaner-burning fuel than coal that emits approximately half as much CO₂ per kW h of energy produced. This rapid growth in the consumption of natural gas has led to increased CO₂ emissions from gas-fired power plants. To limit the contribution of fossil fuel combustion to atmospheric CO₂ levels, carbon capture and sequestration has been proposed as a potential emission mitigation strategy. However, despite extensive exploration of solid adsorbents for CO₂ capture, few studies have examined the performance of adsorbents in post-combustion capture processes specific to natural gas flue emissions. In this perspective, we emphasize the importance of considering gas-fired power plants alongside coal-fired plants in future analyses of carbon capture materials. We address specific challenges and opportunities related to adsorptive carbon capture from the emissions of gas-fired plants and discuss several promising candidate materials. Lastly, we suggest experiments to determine the viability of new CO₂ capture materials for this separation. This broadening in the scope of current carbon capture research is urgently needed to accelerate the deployment of transformational carbon capture technologies.

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Research Organization:: Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Chemical Sciences, Geosciences & Biosciences Division (CSGB)

Grant/Contract Number:: AC02-05CH11231

OSTI ID:: 1975809

Journal Information:: Energy & Environmental Science, Vol. 12, Issue 7; ISSN 1754-5692

Publisher:: Royal Society of ChemistryCopyright Statement

Country of Publication:: United States

Language:: English

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