Temporal and spatial trends in total PCB and PCB congeners in biota in a river-reservoir system
Conference
·
OSTI ID:197543
- Academy of Natural Sciences of Philadelphia, PA (United States). Environmental Research Division
Since 1984, biennial studies of PCBs have been conducted in fishes, crayfish and insects in the Housatonic River, CT., and additional data are available from earlier studies. PCB data quantitated from presumptive Aroclor concentrations overestimated total PCB concentrations ([TPCB]) by about 13%, although the estimates by the 2 methods were very highly correlated. Ages of all fish specimens were determined. Spatial and temporal trends in [TPCB] were analyzed using ANCOVA to adjust for relationships between [TPCB] and age, lipid content, location and sex. Adjusted [TPCB] consistently decreased in the downstream direction. [TPCB] decreased within the years after cessation of direct inputs (around 1978). However, in the 1984--1992 period [TPCB] trends were weak and variable. Concentrations in 1994 were lower than previous years (statistical comparisons showing 1994 to be the lowest year or among a group of years with the lowest concentrations). Between year differences were probably related to temperature, storm flows and other factors affecting availability and accumulation. These variations were greater in riverine sites than in reservoirs. In brown trout, [TPCB] increased rapidly within 1--2 months after stocking. Over longer periods, [TPCB] were more closely related to seasonal cycles in lipid content rather than to time in river. Increases in [TPCB] with age were most evident for long-lived species in reservoirs. Several congeners which are abundant in Aroclors 1254 and 1260 predominated the samples. However, spatial and temporal differences in accumulation of different congeners were evident. Spatial differences in the concentration of some marker congeners reflected enrichment of these congeners from original Aroclor 1254 and 1260 sources, as well as supplemental inputs of Aroclor 1242.
- OSTI ID:
- 197543
- Report Number(s):
- CONF-9511137--; ISBN 1-880611-03-1
- Country of Publication:
- United States
- Language:
- English
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