Hybrid magnonics in hybrid perovskite antiferromagnets

Comstock, Andrew H.; Chou, Chung-Tao; Wang, Zhiyu; Wang, Tonghui; Song, Ruyi; Sklenar, Joseph; Amassian, Aram; Zhang, Wei; Lu, Haipeng; Liu, Luqiao; Beard, Matthew C.; Sun, Dali

doi:10.1038/s41467-023-37505-w

Title: Hybrid magnonics in hybrid perovskite antiferromagnets

Journal Article · Sat Apr 01 00:00:00 EDT 2023 · Nature Communications

DOI:https://doi.org/10.1038/s41467-023-37505-w· OSTI ID:1968102

;

; Wang, Zhiyu; Wang, Tonghui;

; Sklenar, Joseph;

; Zhang, Wei;

;

Abstract Hybrid magnonic systems are a newcomer for pursuing coherent information processing owing to their rich quantum engineering functionalities. One prototypical example is hybrid magnonics in antiferromagnets with an easy-plane anisotropy that resembles a quantum-mechanically mixed two-level spin system through the coupling of acoustic and optical magnons. Generally, the coupling between these orthogonal modes is forbidden due to their opposite parity. Here we show that the Dzyaloshinskii–Moriya-Interaction (DMI), a chiral antisymmetric interaction that occurs in magnetic systems with low symmetry, can lift this restriction. We report that layered hybrid perovskite antiferromagnets with an interlayer DMI can lead to a strong intrinsic magnon-magnon coupling strength up to 0.24 GHz, which is four times greater than the dissipation rates of the acoustic/optical modes. Our work shows that the DMI in these hybrid antiferromagnets holds promise for leveraging magnon-magnon coupling by harnessing symmetry breaking in a highly tunable, solution-processable layered magnetic platform.

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Research Organization:: National Renewable Energy Lab. (NREL), Golden, CO (United States); Energy Frontier Research Centers (EFRC) (United States). Center for Hybrid Organic Inorganic Semiconductors for Energy (CHOISE)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); Hong Kong University of Science and Technology; Research Grants Council of Hong Kong; US Air Force Office of Scientific Research (AFOSR)

Grant/Contract Number:: AC36-08GO28308; Center for Hybrid Organic Inorganic Semiconductors for Energy (CHOISE); SC0020992; DMR-2143642; ECS, 26300721; ECCS-1936527; ECCS-1941426; AFOSR-FA2386-21-1-4091; DMR-2104912

OSTI ID:: 1968102

Alternate ID(s):: OSTI ID: 1970461

Report Number(s):: NREL/JA-5900-83150; 1834; PII: 37505

Journal Information:: Nature Communications, Journal Name: Nature Communications Vol. 14 Journal Issue: 1; ISSN 2041-1723

Publisher:: Nature Publishing GroupCopyright Statement

Country of Publication:: United Kingdom

Language:: English

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