Discovery of a Magnetic Dirac System with a Large Intrinsic Nonlinear Hall Effect

Mazzola, Federico; Ghosh, Barun; Fujii, Jun; Acharya, Gokul; Mondal, Debashis; Rossi, Giorgio; Bansil, Arun; Farias, Daniel; Hu, Jin; Agarwal, Amit; Politano, Antonio; Vobornik, Ivana

doi:10.1021/acs.nanolett.2c04194

Title: Discovery of a Magnetic Dirac System with a Large Intrinsic Nonlinear Hall Effect

Journal Article · Mon Jan 23 00:00:00 EST 2023 · Nano Letters

DOI:https://doi.org/10.1021/acs.nanolett.2c04194· OSTI ID:1967523

^[1]; Ghosh, Barun ^[2]; Fujii, Jun ^[3]; Acharya, Gokul ^[4]; Mondal, Debashis ^[3];

^[5]; Bansil, Arun ^[2];

^[6];

^[4]; Agarwal, Amit ^[7];

^[8]; Vobornik, Ivana ^[3]

CNR-IOM TASC Laboratory, Area Science Park, 34149Trieste, Italy, Department of Molecular Sciences and Nanosystems, Ca’ Foscari University of Venice, 30172Venice, Italy
Department of Physics, Northeastern University, Boston, Massachusetts02115, United States
CNR-IOM TASC Laboratory, Area Science Park, 34149Trieste, Italy
Department of Physics, University of Arkansas, Fayetteville, Arkansas72701, United States
University of Milano, 20133Milano, Italy
Departamento de Física de la Materia Condensada, Universidad Autónoma de Madrid, 28049Madrid, Spain, Instituto “Nicolás Cabrera” and Condensed Matter Physics Center (IFIMAC), Universidad Autónoma de Madrid, 28049Madrid, Spain
Department of Physics, Indian Institute of Technology Kanpur, Kanpur208016, India
Department of Physical and Chemical Sciences, University of L’Aquila, Via Vetoio, 67100L’Aquila, Italy

Magnetic materials exhibiting topological Dirac fermions are attracting significant attention for their promising technological potential in spintronics. In these systems, the combined effect of the spin-orbit coupling and magnetic order enables the realization of novel topological phases with exotic transport properties, including the anomalous Hall effect and magneto-chiral phenomena. Furthermore, we report experimental evidence of topological Dirac antiferromagnetism in TaCoTe₂ via angle-resolved photoelectron spectroscopy (ARPES) and first-principles density functional theory (DFT) calculations. In particular, we find the existence of spin-orbit coupling-induced gaps at the Fermi level, consistent with the manifestation of a large intrinsic non-linear Hall conductivity. Remarkably, we find that the latter is extremely sensitive to the orientation of the N´eel vector, suggesting TaCoTe₂ a suitable candidate for the realization of non-volatile spintronic devices with an unprecedented level of intrinsic tunability.

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Research Organization:: Univ. of Arkansas, Fayetteville, AR (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0022006

OSTI ID:: 1967523

Alternate ID(s):: OSTI ID: 1975856

Journal Information:: Nano Letters, Journal Name: Nano Letters Vol. 23 Journal Issue: 3; ISSN 1530-6984

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Title: Discovery of a Magnetic Dirac System with a Large Intrinsic Nonlinear Hall Effect

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