Topology induced crossover between Langevin, subdiffusion, and Brownian diffusion regimes in supercooled water

Zhu, Kaicheng; Naserifar, Saber; Goddard, William A.; Su, Haibin

doi:10.1039/D2CP04645H

Title: Topology induced crossover between Langevin, subdiffusion, and Brownian diffusion regimes in supercooled water

Journal Article · Wed Apr 12 00:00:00 EDT 2023 · Physical Chemistry Chemical Physics. PCCP

DOI:https://doi.org/10.1039/D2CP04645H· OSTI ID:1967509

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Department of Chemistry, The Hong Kong University of Science and Technology, Kowloon, Hong Kong
Materials and Process Simulation Center, California Institute of Technology, Pasadena, California, USA, 91125

Translational diffusion couples with dynamic reorganization of hydrogen-bond networks in supercooled water. The topological transformation explains the fragile-to-strong transition at around 230 K.

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Sponsoring Organization:: USDOE

OSTI ID:: 1967509

Journal Information:: Physical Chemistry Chemical Physics. PCCP, Journal Name: Physical Chemistry Chemical Physics. PCCP Vol. 25 Journal Issue: 15; ISSN 1463-9076

Publisher:: Royal Society of Chemistry (RSC)Copyright Statement

Country of Publication:: United Kingdom

Language:: English

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