World beyond the nearest neighbors

Egami, Takeshi; Ryu, Chae Woo

doi:10.1088/1361-648x/acbe24

World beyond the nearest neighbors

Journal Article · Fri Mar 03 00:00:00 EST 2023 · Journal of Physics. Condensed Matter

DOI:https://doi.org/10.1088/1361-648x/acbe24· OSTI ID:1960698

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Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division
Univ. of Tennessee, Knoxville, TN (United States); Hongik University, Seoul (Korea, Republic of)

The structure beyond the nearest neighbor atoms in liquid and glass is characterized by the medium-range order (MRO). In the conventional approach, the MRO is considered to result directly from the short-range order (SRO) in the nearest neighbors. To this bottom–up approach starting with the SRO, we propose to add a top–down approach in which global collective forces drive liquid to form density waves. The two approaches are in conflict with each other, and the compromise produces the structure with the MRO. The driving force to produce density waves provides the stability and stiffness to the MRO, and controls various mechanical properties. This dual framework provides a novel perspective for description of the structure and dynamics of liquid and glass.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1960698

Journal Information:: Journal of Physics. Condensed Matter, Journal Name: Journal of Physics. Condensed Matter Journal Issue: 17 Vol. 35; ISSN 0953-8984

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United States

Language:: English

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