World beyond the nearest neighbors

Egami, Takeshi; Ryu, Chae Woo

doi:10.1088/1361-648x/acbe24

World beyond the nearest neighbors

Journal Article · Thu Mar 02 23:00:00 EST 2023 · Journal of Physics. Condensed Matter

DOI:https://doi.org/10.1088/1361-648x/acbe24· OSTI ID:1960698

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Univ. of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States). Materials Science & Technology Division
Univ. of Tennessee, Knoxville, TN (United States); Hongik University, Seoul (Korea, Republic of)

The structure beyond the nearest neighbor atoms in liquid and glass is characterized by the medium-range order (MRO). In the conventional approach, the MRO is considered to result directly from the short-range order (SRO) in the nearest neighbors. To this bottom–up approach starting with the SRO, we propose to add a top–down approach in which global collective forces drive liquid to form density waves. The two approaches are in conflict with each other, and the compromise produces the structure with the MRO. The driving force to produce density waves provides the stability and stiffness to the MRO, and controls various mechanical properties. This dual framework provides a novel perspective for description of the structure and dynamics of liquid and glass.

View Accepted Manuscript (DOE)

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1960698

Journal Information:: Journal of Physics. Condensed Matter, Journal Name: Journal of Physics. Condensed Matter Journal Issue: 17 Vol. 35; ISSN 0953-8984

Publisher:: IOP PublishingCopyright Statement

Country of Publication:: United States

Language:: English

References (40)

On the fracture morphology of metallic glasses Spaepen, Frans Acta Metallurgica, Vol. 23, Issue 5 https://doi.org/10.1016/0001-6160(75)90102-9	journal	May 1975
Plastic deformation in metallic glasses Argon, A. S. Acta Metallurgica, Vol. 27, Issue 1 https://doi.org/10.1016/0001-6160(79)90055-5	journal	January 1979
An atomistic study of deformation of amorphous metals Srolovitz, D.; Vitek, V.; Egami, T. Acta Metallurgica, Vol. 31, Issue 2 https://doi.org/10.1016/0001-6160(83)90110-4	journal	February 1983
Structure of Metallic Alloy Glasses Cargill III, G. S. Solid State Physics https://doi.org/10.1016/S0081-1947(08)60337-9	book	January 1975
Universal nature of the saddle states of structural excitations in metallic glasses Ding, J.; Li, L.; Wang, N. Materials Today Physics, Vol. 17 https://doi.org/10.1016/j.mtphys.2021.100359	journal	March 2021
Above Saddle-Point Regions of Order in a Sea of Chaos in the Vibrational Dynamics of KCN Párraga, H.; Arranz, F. J.; Benito, R. M. The Journal of Physical Chemistry A, Vol. 122, Issue 13 https://doi.org/10.1021/acs.jpca.8b00113	journal	March 2018
A Geometrical Approach to the Structure Of Liquids Bernal, J. D. Nature, Vol. 183, Issue 4655 https://doi.org/10.1038/183141a0	journal	January 1959
Supercooled liquids and the glass transition Debenedetti, Pablo G.; Stillinger, Frank H. Nature, Vol. 410, Issue 6825 https://doi.org/10.1038/35065704	journal	March 2001
Atomic packing and short-to-medium-range order in metallic glasses Sheng, H. W.; Luo, W. K.; Alamgir, F. M. Nature, Vol. 439, Issue 7075 https://doi.org/10.1038/nature04421	journal	January 2006
Universal structural parameter to quantitatively predict metallic glass properties Ding, Jun; Cheng, Yong-Qiang; Sheng, Howard Nature Communications, Vol. 7, Issue 1 https://doi.org/10.1038/ncomms13733	journal	December 2016
Energy landscape-driven non-equilibrium evolution of inherent structure in disordered material Fan, Yue; Iwashita, Takuya; Egami, Takeshi Nature Communications, Vol. 8, Issue 1 https://doi.org/10.1038/ncomms15417	journal	May 2017
A structural model for metallic glasses Miracle, Daniel B. Nature Materials, Vol. 3, Issue 10 https://doi.org/10.1038/nmat1219	journal	September 2004
Thermodynamic signature of growing amorphous order in glass-forming liquids Biroli, G.; Bouchaud, J. -P.; Cavagna, A. Nature Physics, Vol. 4, Issue 10 https://doi.org/10.1038/nphys1050	journal	August 2008
Non-monotonic temperature evolution of dynamic correlations in glass-forming liquids Kob, Walter; Roldán-Vargas, Sándalo; Berthier, Ludovic Nature Physics, Vol. 8, Issue 2 https://doi.org/10.1038/nphys2133	journal	October 2011
Unveiling the predictive power of static structure in glassy systems Bapst, V.; Keck, T.; Grabska-Barwińska, A. Nature Physics, Vol. 16, Issue 4 https://doi.org/10.1038/s41567-020-0842-8	journal	April 2020
Curie-Weiss behavior of liquid structure and ideal glass state Ryu, C. W.; Dmowski, W.; Kelton, K. F. Scientific Reports, Vol. 9, Issue 1 https://doi.org/10.1038/s41598-019-54758-y	journal	December 2019
Role of Repulsive Forces in Determining the Equilibrium Structure of Simple Liquids Weeks, John D.; Chandler, David; Andersen, Hans C. The Journal of Chemical Physics, Vol. 54, Issue 12 https://doi.org/10.1063/1.1674820	journal	June 1971
Saddle-point solutions and grazing bifurcations in an impacting system Mason, Joanna F.; Piiroinen, Petri T. Chaos: An Interdisciplinary Journal of Nonlinear Science, Vol. 22, Issue 1 https://doi.org/10.1063/1.3673786	journal	March 2012
Structural defects in amorphous solids Statistical analysis of a computer model Srolovitz, D.; Maeda, K.; Vitek, V. Philosophical Magazine A, Vol. 44, Issue 4 https://doi.org/10.1080/01418618108239553	journal	October 1981
Order, frustration, and defects in liquids and glasses Nelson, David R. Physical Review B, Vol. 28, Issue 10 https://doi.org/10.1103/PhysRevB.28.5515	journal	November 1983
Order in metallic glasses and icosahedral crystals Sachdev, Subir; Nelson, David R. Physical Review B, Vol. 32, Issue 7 https://doi.org/10.1103/PhysRevB.32.4592	journal	October 1985
Glass transition in metallic glasses: A microscopic model of topological fluctuations in the bonding network Egami, T.; Poon, S. J.; Zhang, Z. Physical Review B, Vol. 76, Issue 2 https://doi.org/10.1103/PhysRevB.76.024203	journal	July 2007
Ideality of liquid structure: A case study for metallic alloy liquids Ryu, Chae Woo; Dmowski, Wojciech; Egami, Takeshi Physical Review E, Vol. 101, Issue 3 https://doi.org/10.1103/PhysRevE.101.030601	journal	March 2020
Origin of liquid fragility Ryu, Chae Woo; Egami, Takeshi Physical Review E, Vol. 102, Issue 4 https://doi.org/10.1103/PhysRevE.102.042615	journal	October 2020
Medium-range atomic correlation in simple liquids. I. Distinction from short-range order Ryu, Chae Woo; Egami, Takeshi Physical Review E, Vol. 104, Issue 6 https://doi.org/10.1103/PhysRevE.104.064109	journal	December 2021
Medium-range atomic correlation in simple liquids. II. Theory of temperature dependence Egami, Takeshi; Ryu, Chae Woo Physical Review E, Vol. 104, Issue 6 https://doi.org/10.1103/PhysRevE.104.064110	journal	December 2021
Dynamics of viscoplastic deformation in amorphous solids Falk, M. L.; Langer, J. S. Physical Review E, Vol. 57, Issue 6 https://doi.org/10.1103/PhysRevE.57.7192	journal	June 1998
Static point-to-set correlations in glass-forming liquids Berthier, Ludovic; Kob, Walter Physical Review E, Vol. 85, Issue 1 https://doi.org/10.1103/PhysRevE.85.011102	journal	January 2012
Crossovers in the dynamics of supercooled liquids probed by an amorphous wall Hocky, Glen M.; Berthier, Ludovic; Kob, Walter Physical Review E, Vol. 89, Issue 5 https://doi.org/10.1103/PhysRevE.89.052311	journal	May 2014
Elastic Heterogeneity in Metallic Glasses Dmowski, W.; Iwashita, T.; Chuang, C. -P. Physical Review Letters, Vol. 105, Issue 20 https://doi.org/10.1103/PhysRevLett.105.205502	journal	November 2010
Probing a Liquid to Glass Transition in Equilibrium Kob, Walter; Berthier, Ludovic Physical Review Letters, Vol. 110, Issue 24 https://doi.org/10.1103/PhysRevLett.110.245702	journal	June 2013
Identifying Structural Flow Defects in Disordered Solids Using Machine-Learning Methods Cubuk, E. D.; Schoenholz, S. S.; Rieser, J. M. Physical Review Letters, Vol. 114, Issue 10 https://doi.org/10.1103/PhysRevLett.114.108001	journal	March 2015
Atomic Dynamics in Simple Liquid: de Gennes Narrowing Revisited Wu, Bin; Iwashita, Takuya; Egami, Takeshi Physical Review Letters, Vol. 120, Issue 13 https://doi.org/10.1103/PhysRevLett.120.135502	journal	March 2018
Nonaffine Strains Control Ductility of Metallic Glasses Wang, Hui; Dmowski, Wojciech; Tong, Yang Physical Review Letters, Vol. 128, Issue 15 https://doi.org/10.1103/PhysRevLett.128.155501	journal	April 2022
Should All Crystals Be bcc? Landau Theory of Solidification and Crystal Nucleation Alexander, S.; McTague, J. Physical Review Letters, Vol. 41, Issue 10 https://doi.org/10.1103/PhysRevLett.41.702	journal	September 1978
Direct Experimental Evidence of a Growing Length Scale Accompanying the Glass Transition Berthier, L. Science, Vol. 310, Issue 5755 https://doi.org/10.1126/science.1120714	journal	December 2005
Formation of Glasses from Liquids and Biopolymers Angell, C. A. Science, Vol. 267, Issue 5206 https://doi.org/10.1126/science.267.5206.1924	journal	March 1995
Why Is the Range of Timescale So Wide in Glass-Forming Liquid? Egami, Takeshi; Ryu, Chae Woo Frontiers in Chemistry, Vol. 8 https://doi.org/10.3389/fchem.2020.579169	journal	September 2020
Structural Principles in Liquids and Glasses: Bottom-Up or Top-Down Egami, Takeshi; Ryu, Chae Woo Frontiers in Materials, Vol. 9 https://doi.org/10.3389/fmats.2022.874191	journal	June 2022
Local Density Correlations in Liquids Egami, Takeshi Frontiers in Physics, Vol. 8 https://doi.org/10.3389/fphy.2020.00050	journal	February 2020

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