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Particle–hole asymmetric superconducting coherence peaks in overdoped cuprates

Journal Article · · Nature Physics
 [1];  [1];  [2];  [1];  [2];  [1];  [1];  [3];  [4];  [2];  [5];  [6]
  1. Tsinghua Univ., Beijing (China)
  2. Chinese Academy of Sciences (CAS), Beijing (China)
  3. Renmin Univ. of China, Beijing (China)
  4. Max Planck Institute of Solid State Research, Stuttgart (Germany)
  5. Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
  6. Tsinghua Univ., Beijing (China); Frontier Science Center for Quantum Information, Beijing (China)
As doping increases in cuprate superconductors, the superconducting transition temperature increases to a maximum at the so-called optimal doping, and then decreases in the overdoped regime. In the past few decades, research has primarily focused on the underdoped and optimally doped regions of the phase diagram. Here, phenomena such as the pseudogap and strange metal non-superconducting states make it difficult to determine the superconducting pairing mechanism. More recently, experiments have shown unconventional behaviour in strongly overdoped cuprates, in both the normal and superconducting states. However, a real-space investigation of the unconventional superconductivity in the absence of the pseudogap is lacking, and the superconductor-to-metal phase transition in the overdoped regime remains controversial. Here we use scanning tunnelling microscopy to investigate the atomic-scale electronic structure of overdoped Bi2Sr2Can–1CunO2n + 4 + δ cuprates. We show that, at low energies, the spectroscopic maps are well described by dispersive d-wave quasiparticle interference patterns. However, as the bias increases to the superconducting coherence peak energy, a periodic and non-dispersive pattern emerges. The position of the coherence peaks exhibits particle–hole asymmetry that modulates with the same period. Finally, we propose that this behaviour is due to quasiparticle interference caused by pair-breaking scattering between flat antinodal Bogoliubov bands.
Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States)
Sponsoring Organization:
Beijing Advanced Innovation Center for Future Chip (ICFC); Chinese Academy of Sciences (CAS); Gordon and Betty Moore Foundation; Ministry of Science and Technology, China (MOST); National Natural Science Foundation of China (NSFC); Tencent Foundation; USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division; USDOE Office of Science (SC), High Energy Physics (HEP)
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1906829
Journal Information:
Nature Physics, Journal Name: Nature Physics Journal Issue: 5 Vol. 18; ISSN 1745-2473
Publisher:
Nature Publishing Group (NPG)Copyright Statement
Country of Publication:
United States
Language:
English

References (47)

A ‘checkerboard’ electronic crystal state in lightly hole-doped Ca2-xNaxCuO2Cl2 journal August 2004
How Cooper pairs vanish approaching the Mott insulator in Bi2Sr2CaCu2O8+δ journal August 2008
Quantum oscillations in an overdoped high-Tc superconductor journal October 2008
Intra-unit-cell electronic nematicity of the high-Tc copper-oxide pseudogap states journal July 2010
Fluctuating stripes at the onset of the pseudogap in the high-Tc superconductor Bi2Sr2CaCu2O8+x journal December 2010
Dependence of the critical temperature in overdoped copper oxides on superfluid density journal August 2016
Spontaneous breaking of rotational symmetry in copper oxide superconductors journal July 2017
Visualizing the atomic-scale electronic structure of the Ca2CuO2Cl2 Mott insulator journal January 2013
Point nodes persisting far beyond Tc in Bi2212 journal July 2015
Persistence of magnetic excitations in La2−xSrxCuO4 from the undoped insulator to the heavily overdoped non-superconducting metal journal August 2013
A momentum-dependent perspective on quasiparticle interference in Bi2Sr2CaCu2O8+δ journal August 2009
Phase-fluctuating superconductivity in overdoped La2−xSrxCuO4 journal March 2011
Energy gaps in high-transition-temperature cuprate superconductors journal June 2014
Quasiparticle interference and superconducting gap in Ca2−xNaxCuO2Cl2 journal October 2007
Coherent organization of electronic correlations as a mechanism to enhance and stabilize high-T C cuprate superconductivity journal January 2018
Phase diagram of Bi2Sr2CaCu2O8+δ revisited journal December 2018
Directly visualizing the sign change of d-wave superconducting gap in Bi2Sr2CaCu2O8+δ by phase-referenced quasiparticle interference journal April 2019
Disappearance of superconductivity due to vanishing coupling in the overdoped Bi$$_{2}$$2Sr$$_{2}$$2CaCu$$_{2}$$2O$$_{8+\delta }$$8+δ journal January 2020
Charge density waves in cuprate superconductors beyond the critical doping journal March 2021
Superconductor-to-metal transition in overdoped cuprates journal April 2021
Re-entrant charge order in overdoped (Bi,Pb)2.12Sr1.88CuO6+δ outside the pseudogap regime journal June 2018
Phase evolution, structural and superconducting properties of Pb-free Bi2Sr2Ca2Cu3O10+ single crystals journal March 2004
Quasiparticle interference and charge order in a heavily overdoped non-superconducting cuprate journal June 2018
Quasiparticle scattering interference in high-temperature superconductors journal January 2003
Effect of oxygen-doping on Bi 2 Sr 2 Ca 2 Cu 3 O 10 + δ vortex matter: Crossover from electromagnetic to Josephson interlayer coupling journal May 2008
Bogoliubov angle and visualization of particle-hole mixture in superconductors journal August 2008
Continuous doping of a cuprate surface: Insights from in situ angle-resolved photoemission journal October 2018
Double pair breaking peak in Raman scattering spectra of the triple-layer cuprate Bi2Sr2Ca2Cu3O10+z journal October 2018
Imaging the Essential Role of Spin Fluctuations in High- T c Superconductivity journal November 2009
Development of Ferromagnetic Fluctuations in Heavily Overdoped ( Bi , Pb ) 2 Sr 2 CuO 6 + δ Copper Oxides journal August 2018
Locating the Missing Superconducting Electrons in the Overdoped Cuprates La 2 − x Sr x CuO 4 journal January 2019
Effect of Structural Supermodulation on Superconductivity in Trilayer Cuprate Bi 2 Sr 2 Ca 2 Cu 3 O 10 + δ journal January 2020
Anomalous Doping Evolution of Superconductivity and Quasiparticle Interference in Bi2Sr2Ca2Cu3O10+δ Trilayer Cuprates journal December 2020
BCS-Like Bogoliubov Quasiparticles in High- T c Superconductors Observed by Angle-Resolved Photoemission Spectroscopy journal May 2003
Fermi Surface and Quasiparticle Excitations of Overdoped Tl 2 Ba 2 CuO 6 + δ journal August 2005
Scanning tunneling spectroscopy of high-temperature superconductors journal March 2007
A Four Unit Cell Periodic Pattern of Quasi-Particle States Surrounding Vortex Cores in Bi2Sr2CaCu2O8+delta journal January 2002
Imaging Quasiparticle Interference in Bi2Sr2CaCu2O8+δ journal July 2002
Atomic-Scale Sources and Mechanism of Nanoscale Electronic Disorder in Bi2Sr2CaCu2O8+  journal August 2005
An Intrinsic Bond-Centered Electronic Glass with Unidirectional Domains in Underdoped Cuprates journal March 2007
Anomalous Criticality in the Electrical Resistivity of La2-xSrxCuO4 journal January 2009
Coherence Factors in a High-Tc Cuprate Probed by Quasi-Particle Scattering Off Vortices journal February 2009
From a Single-Band Metal to a High-Temperature Superconductor via Two Thermal Phase Transitions journal March 2011
Imaging the Impact of Single Oxygen Atoms on Superconducting Bi2+ySr2-yCaCu2O8+x journal July 2012
Fermi Surface and Pseudogap Evolution in a Cuprate Superconductor journal May 2014
Simultaneous Transitions in Cuprate Momentum-Space Topology and Electronic Symmetry Breaking journal May 2014
Discovery of orbital-selective Cooper pairing in FeSe journal July 2017