Spin-orbit–coupled exciton-polariton condensates in lead halide perovskites

Spencer, Michael S.; Fu, Yongping; Schlaus, Andrew P.; Hwang, Doyk; Dai, Yanan; Smith, Matthew D.; Gamelin, Daniel R.; Zhu, X. -Y.

doi:10.1126/sciadv.abj7667

Spin-orbit–coupled exciton-polariton condensates in lead halide perovskites

Journal Article · Wed Dec 01 00:00:00 EST 2021 · Science Advances

DOI:https://doi.org/10.1126/sciadv.abj7667· OSTI ID:1904328

^[1]; ^[2]; Schlaus, Andrew P. ^[2]; ^[2]; ^[2]; ^[3]; ^[3]; ^[2]

Columbia Univ., New York, NY (United States); OSTI
Columbia Univ., New York, NY (United States)
Univ. of Washington, Seattle, WA (United States)

Spin-orbit coupling (SOC) is responsible for a range of spintronic and topological processes in condensed matter. Here, we show photonic analogs of SOCs in exciton-polaritons and their condensates in microcavities composed of birefringent lead halide perovskite single crystals. The presence of crystalline anisotropy coupled with splitting in the optical cavity of the transverse electric and transverse magnetic modes gives rise to a non-Abelian gauge field, which can be described by the Rashba-Dresselhaus Hamiltonian near the degenerate points of the two polarization modes. With increasing density, the exciton-polaritons with pseudospin textures undergo phase transitions to competing condensates with orthogonal polarizations. Unlike their pure photonic counterparts, these exciton-polaritons and condensates inherit nonlinearity from their excitonic components and may serve as quantum simulators of many-body SOC processes.

View Accepted Manuscript (DOE)

Research Organization:: Columbia Univ., New York, NY (United States)

Sponsoring Organization:: USDOE Office of Science (SC)

Grant/Contract Number:: SC0019443

OSTI ID:: 1904328

Journal Information:: Science Advances, Journal Name: Science Advances Journal Issue: 49 Vol. 7; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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