Lithium and boron isotopic compositions of olivine in chondrules from carbonaceous and ordinary chondrite meteorites: Implications for the origin of solar 11B/10B ratio

Liu, Ming-Chang; Chaussidon, Marc; Matsuda, Nozomi

doi:10.1016/j.gca.2022.12.001

Title: Lithium and boron isotopic compositions of olivine in chondrules from carbonaceous and ordinary chondrite meteorites: Implications for the origin of solar ¹¹B/¹⁰B ratio

Journal Article · Mon Dec 05 00:00:00 EST 2022 · Geochimica et Cosmochimica Acta

DOI:https://doi.org/10.1016/j.gca.2022.12.001· OSTI ID:1903447

Liu, Ming-Chang ^[1]; Chaussidon, Marc ^[2]; Matsuda, Nozomi ^[1]

University of California, Los Angeles, CA (United States)
Université de Paris Cité (France)

We report the origin of solar ¹¹B/¹⁰B ratio ~4 remains an open question. It has been thought that a significant portion of boron in the Solar System was derived from continuous spallation nucleosynthesis during interactions between Galactic Cosmic Rays and C—N—O nuclei in the interstellar medium. However, because GCR-produced boron is characterized by ¹¹B/¹⁰B ~2.5, an endmember with ¹¹B/¹⁰B > 4 is required to account for the solar ¹¹B/¹⁰B ratio. Two leading hypotheses for the sources of ¹¹B-rich components include low energy spallation in the Sun’s parental molecular cloud and the neutrino process during the supernova explosions. In this study, lithium and boron elemental and isotopic compositions of seven porphyritic olivine chondrules and one isolated olivine crystal from four meteorites (Allende, Yamato 81020, Asuka 12236, and QUE 97008) were determined in-situ to help constrain which of the two nucleosynthetic mechanisms has most likely supplied the forming Solar System with extra ¹¹B. Apparent isotopic variations in Li/Si, B/Si, δ⁷Li and δ¹¹B were found in chondrule olivine crystals, but only three chondrules exhibit statistically resolved δ¹¹B heterogeneities. Using these three chondrules as a basis for discussion, we evaluated the processes that could potentially cause elemental and isotopic variations of Li and B. We argue that the data can be best understood in the context of condensation of lithium-boron-rich material onto chondrule precursors in (an) initially heterogeneous gaseous reservoir(s), which could be realized if the Solar System derived ¹¹B-rich components from a supernova or supernovae.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA); National Aeronautics and Space Administration (NASA); French National Research Agency (ANR)

Grant/Contract Number:: AC52-07NA27344; 80NSSC18K0602; 80NSSC20K0759; ANR-15-CE31-0004-1

OSTI ID:: 1903447

Report Number(s):: LLNL-JRNL-840752; 1062445; TRN: US2311337

Journal Information:: Geochimica et Cosmochimica Acta, Vol. 341, Issue N/A; ISSN 0016-7037

Publisher:: Elsevier; The Geochemical Society; The Meteoritical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Journal Article · Sat Dec 01 00:00:00 EST 1990 · Geochimica et Cosmochimica Acta; (USA) · OSTI ID:1903447

Radomsky, P M; Hewins, R H

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58 GEOSCIENCES
79 ASTRONOMY AND ASTROPHYSICS
nucleosynthesis
spallation reactions
chondrules
secondary ion mass spectrometry

Title: Lithium and boron isotopic compositions of olivine in chondrules from carbonaceous and ordinary chondrite meteorites: Implications for the origin of solar 11B/10B ratio

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Title: Lithium and boron isotopic compositions of olivine in chondrules from carbonaceous and ordinary chondrite meteorites: Implications for the origin of solar ¹¹B/¹⁰B ratio