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Relaxation dynamics in excited helium nanodroplets probed with high resolution, time-resolved photoelectron spectroscopy

Journal Article · · Physical Chemistry Chemical Physics. PCCP
DOI:https://doi.org/10.1039/D2CP03335F· OSTI ID:1899749
 [1];  [2];  [2];  [3];  [4];  [5];  [4];  [1];  [6];  [5];  [7];  [1];  [8];  [6];  [4];  [4];  [4];  [9];  [1];  [6] more »;  [1];  [10] « less
  1. Department of Physics, University of Connecticut, Storrs, Connecticut, 06269, USA
  2. Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark
  3. Istituto di Fotonica e Nanotecnologie, Consiglio Nazionale delle Ricerche, 20133 Milano, Italy, Dipartimento di Fisica Politecnico, 20133 Milano, Italy
  4. Elettra-Sincrotrone Trieste S.C.p.A., 34149 Basovizza Trieste, Italy
  5. Department of Physics, Indian Institute of Technology-Madras, Chennai 600036, India
  6. Institute of Physics, University of Freiburg, 79104 Freiburg im Breisgau, Germany
  7. Department of Physics, Ludwig-Maximilians-Universität Munich, 85748 Garching, Germany, Max Planck Institute of Quantum Optics, 85748 Garching, Germany, SLAC National Accelerator Laboratory, Menlo Park 94025, CA, USA, Department of Applied Physics, Stanford University, Stanford 94305, CA, USA
  8. Indian Institute of Science Education and Research, Pune 411008, India
  9. Department of Physics, Ludwig-Maximilians-Universität Munich, 85748 Garching, Germany, Max Planck Institute of Quantum Optics, 85748 Garching, Germany
  10. Department of Physics and Astronomy, Aarhus University, 8000 Aarhus C, Denmark, Department of Physics, Indian Institute of Technology-Madras, Chennai 600036, India

The ultrafast relaxation dynamics of excited helium nanodroplets were studied using time-resolved photoelectron spectroscopy. We observed an efficient population of triplet atomic states as well as the formation of the first excimer state of He 2 *.

Sponsoring Organization:
USDOE
Grant/Contract Number:
SC0012376
OSTI ID:
1899749
Journal Information:
Physical Chemistry Chemical Physics. PCCP, Journal Name: Physical Chemistry Chemical Physics. PCCP Journal Issue: 47 Vol. 24; ISSN 1463-9076; ISSN PPCPFQ
Publisher:
Royal Society of Chemistry (RSC)Copyright Statement
Country of Publication:
United Kingdom
Language:
English

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