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Title: Balancing Functionality and Printability: High-Loading Polymer Resins for Direct Ink Writing

Journal Article · · Polymers

Although direct ink writing (DIW) allows the rapid fabrication of unique 3D printed objects, the resins—or “inks”—available for this technique are in short supply and often offer little functionality, leading to the development of new, custom inks. However, when creating new inks, the ability of the ink to lead to a successful print, or the “printability,” must be considered. Thus, this work examined the effect of filler composition/concentration, printing parameters, and lattice structure on the printability of new polysiloxane inks incorporating high concentrations (50–70 wt%) of metallic and ceramic fillers as well as emulsions. Results suggest that strut diameter and spacing ratio have the most influence on the printability of DIW materials and that the printability of silica- and metal-filled inks is more predictable than ceramic-filled inks. Additionally, higher filler loadings and SC geometries led to stiffer printed parts than lower loadings and FCT geometries, and metal-filled inks were more thermally stable than ceramic-filled inks. The findings in this work provide important insights into the tradeoffs associated with the development of unique and/or multifunctional DIW inks, printability, and the final material’s performance.

Research Organization:
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC52-06NA25396; 89233218CNA000001
OSTI ID:
1896516
Alternate ID(s):
OSTI ID: 1900488
Report Number(s):
LA-UR-22-30284; POLYCK; PII: polym14214661
Journal Information:
Polymers, Journal Name: Polymers Vol. 14 Journal Issue: 21; ISSN 2073-4360
Publisher:
MDPI AGCopyright Statement
Country of Publication:
Switzerland
Language:
English

References (20)

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