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Title: Scalability of Gadolinium-Doped-Water Cherenkov Detectors for Nuclear Nonproliferation

Journal Article · · Physical Review Applied

Antineutrinos are an inextricable element of the fission process. The kiloton-scale KamLAND experiment has demonstrated a capability to detect reactor antineutrinos at a range of a few hundred kilometers. But to detect or rule out the existence of a single small reactor over many kilometers requires a large detector, so large in fact that the optical opacity of the detection medium itself becomes an important factor. If the detector is so large that photons cannot traverse the detector medium to an optical detector, then it becomes impractical. For this reason, gadolinium-doped-water Cherenkov detectors have been proposed for large volumes, due to their appealing light-attenuation properties. Even though Cherenkov emission does not produce many photons and the energy resolution is poor, there may be a place for Gd-doped-water detectors in far-field nuclear-reactor monitoring. Here in this paper, we focus on the reactor-discovery potential of large-volume Gd-doped-water Cherenkov detectors for nuclear-nonproliferation applications. Realistic background models for the worldwide reactor flux, geoneutrinos, cosmogenic fast neutrons, and detector-associated backgrounds are included. We calculate the detector run time required to detect a small 50-MWt reactor at a variety of stand-off distances as a function of detector size. We highlight that, at present, the photomultiplier-tube dark rate and event reconstruction algorithms are the limiting factors to extending such detectors beyond a fiducial mass of approximately 50 kt.

Research Organization:
Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States)
Sponsoring Organization:
USDOE National Nuclear Security Administration (NNSA)
Grant/Contract Number:
AC52-07NA27344; LLNL-JRNL-823255
OSTI ID:
1888848
Alternate ID(s):
OSTI ID: 2223031
Report Number(s):
LLNL-JRNL-823255; PRAHB2; 034059
Journal Information:
Physical Review Applied, Journal Name: Physical Review Applied Vol. 18 Journal Issue: 3; ISSN 2331-7019
Publisher:
American Physical SocietyCopyright Statement
Country of Publication:
United States
Language:
English

References (39)

SciPy 1.0: fundamental algorithms for scientific computing in Python journal February 2020
Precise quasielastic neutrino/nucleon cross-section journal July 2003
Determination of antineutrino spectra from nuclear reactors journal August 2011
Versuch einer Theorie der ?-Strahlen. I journal March 1934
Colloquium : Neutrino detectors as tools for nuclear security journal March 2020
Possibilities of the practical use of neutrinos journal June 1978
Indication of Reactor ν ¯ e Disappearance in the Double Chooz Experiment journal March 2012
A water-based neutron detector as a well multiplicity counter
  • Dazeley, S.; Asghari, A.; Bernstein, A.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 771 https://doi.org/10.1016/j.nima.2014.10.028
journal January 2015
Observation of Electron-Antineutrino Disappearance at Daya Bay journal April 2012
Measurement of Neutrino Oscillation with KamLAND: Evidence of Spectral Distortion journal March 2005
Muon-induced background study for underground laboratories journal March 2006
Antineutrino Spectroscopy with Large Water Čerenkov Detectors journal October 2004
Development of New Data Acquisition System at Super-Kamiokande for Nearby Supernova Bursts journal October 2013
Gamma-ray spectrum from thermal neutron capture on gadolinium-157 journal February 2019
First gadolinium loading to Super-Kamiokande
  • Abe, K.; Bronner, C.; Hayato, Y.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 1027 https://doi.org/10.1016/j.nima.2021.166248
journal March 2022
Limits for qualitative detection and quantitative determination. Application to radiochemistry journal March 1968
Neutrino physics with JUNO journal February 2016
ROOT — An object oriented data analysis framework journal April 1997
Neutrinos Angra experiment: commissioning and first operational measurements journal June 2019
Absorption spectrum (380–700 nm) of pure water II Integrating cavity measurements journal January 1997
An assessment of antineutrino detection as a tool for monitoring nuclear explosions journal January 2001
Array programming with NumPy journal September 2020
Observation of Reactor Electron Antineutrinos Disappearance in the RENO Experiment journal May 2012
Detection of the Free Neutrino: a Confirmation journal July 1956
Gamma-ray spectra from thermal neutron capture on gadolinium-155 and natural gadolinium journal April 2020
Search for Neutrino Oscillations at the Palo Verde Nuclear Reactors journal April 2000
Geoneutrinos and reactor antineutrinos at SNO+ journal May 2016
Когерентное излучение быстрого электрона в среде journal January 1967
Solar neutrino measurements in Super-Kamiokande-IV journal September 2016
Evaluation of gadolinium’s action on water Cherenkov detector systems with EGADS
  • Marti, Ll.; Ikeda, M.; Kato, Y.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 959 https://doi.org/10.1016/j.nima.2020.163549
journal April 2020
Calibration of the Super-Kamiokande detector
  • Abe, K.; Hayato, Y.; Iida, T.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 737 https://doi.org/10.1016/j.nima.2013.11.081
journal February 2014
Matplotlib: A 2D Graphics Environment journal January 2007
Видимое свечение чистых жидкостей под действием γ-радиации journal October 1967
Search for neutrino oscillations on a long base-line at the CHOOZ nuclear power station journal April 2003
First study of neutron tagging with a water Cherenkov detector journal May 2009
A search for cosmogenic production of β-neutron emitting radionuclides in water
  • Dazeley, S.; Askins, M.; Bergevin, M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 821 https://doi.org/10.1016/j.nima.2016.03.014
journal June 2016
Measurement of the neutrino-oxygen neutral-current quasielastic cross section using atmospheric neutrinos at Super-Kamiokande journal February 2019
Measurement of the radon concentration in purified water in the Super-Kamiokande IV detector
  • Nakano, Y.; Hokama, T.; Matsubara, M.
  • Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, Vol. 977 https://doi.org/10.1016/j.nima.2020.164297
journal October 2020
The Sudbury Neutrino Observatory journal November 2009