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Optimally tuned starting point for single-shot GW calculations of solids

Journal Article · · Physical Review Materials
 [1];  [1];  [2];  [1];  [3];  [3];  [3];  [4]
  1. Univ. of California, Berkeley, CA (United States)
  2. Univ. of Oxford (United Kingdom). Clarendon Lab.
  3. Weizmann Institute of Science, Rehovot (Israel)
  4. Univ. of California, Berkeley, CA (United States); Lawrence Berkeley National Lab. (LBNL), Berkeley, CA (United States)
The dependence of ab initio many-body perturbation theory within the $$\textit{GW}$$ approximation on the eigensystem used in calculating quasiparticle corrections limits this method's predictive power. Here, we investigate the accuracy of the recently developed Wannier-localized optimally tuned screened range-separated hybrid (WOT-SRSH) functional as a generalized Kohn-Sham starting point for single-shot $$\textit{GW}$$ ($$G_0W_0$$) calculations for a range of semiconductors and insulators. Comparison to calculations based on well-established functionals, namely, PBE, PBE0, and HSE, as well as to self-consistent GW schemes and to experiment, shows that band gaps computed via $$G_0W_0$$@WOT-SRSH have a level of precision and accuracy that is comparable to that of more advanced methods such as quasiparticle self-consistent $$\textit{GW}$$ and eigenvalue self-consistent $$\textit{GW}$$. In this work, we also find that $$G_0W_0$$@WOT-SRSH improves the description of states deeper in the valence band manifold. Finally, we show that $$G_0W_0$$@WOT-SRSH significantly reduces the sensitivity of computed band gaps to ambiguities in the underlying WOT-SRSH tuning procedure.
Research Organization:
Lawrence Berkeley National Laboratory (LBNL), Berkeley, CA (United States). National Energy Research Scientific Computing Center (NERSC)
Sponsoring Organization:
Engineering and Physical Sciences Research Council (EPSRC); Extreme Science and Engineering Discovery Environment; USDOE Office of Science (SC), Basic Energy Sciences (BES) (SC-22); United States-Israel Binational Science Foundation (BSF)
Grant/Contract Number:
AC02-05CH11231
OSTI ID:
1878321
Journal Information:
Physical Review Materials, Journal Name: Physical Review Materials Journal Issue: 5 Vol. 6; ISSN 2475-9953
Publisher:
American Physical Society (APS)Copyright Statement
Country of Publication:
United States
Language:
English

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