The effect of helium on cavity swelling in dual-ion irradiated Fe and Fe-10Cr ferritic alloys

Lin, Yan-Ru; Bhattacharya, Arunodaya; Zinkle, Steven J.

doi:10.1016/j.jnucmat.2022.153907

Title: The effect of helium on cavity swelling in dual-ion irradiated Fe and Fe-10Cr ferritic alloys

Journal Article · Fri Jul 08 00:00:00 EDT 2022 · Journal of Nuclear Materials

DOI:https://doi.org/10.1016/j.jnucmat.2022.153907· OSTI ID:1876306

^[1];

^[2]; Zinkle, Steven J. ^[1]

University of Tennessee, Knoxville, TN (United States); Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)

We report Ferritic-martensitic (FM) steels for in-vessel components in proposed fusion reactors are expected to suffer from high levels of displacement damage and helium (He) generation by neutron transmutation. However, a thorough understanding of the He synergistic effects on the cavity swelling in FM steels is still not well established. To gain fundamental insights into the He effect on cavity swelling, high purity Fe and Fe-10 wt.% Cr ferritic model alloys were irradiated with 8 MeV Ni ions and co-implanted He ions at 400 to 550 °C up to 30 displacements per atom (dpa) with He implantation rates of 0.1, 10 and 50 appm He/dpa. The current study focuses on the 50 appm He/dpa, 500 °C behavior vs. 0.1 and 10 appm He/dpa. Irradiation-induced defects, including cavities, dislocation loops, and dislocation networks were characterized using transmission electron microscopy (TEM). In the grain interior, a bimodal cavity size distribution was observed in the 10 and 50 appm He/dpa samples, but not for 0.1 appm He/dpa. Cavity swelling was maximized at intermediate He implantation rates of ~10 appm He/dpa for both ion-irradiated Fe and Fe-10Cr alloys. The cavity swelling behavior as a function of He implantation rate appears to be controlled by the He/dpa-dependent variation of cavity sink strengths. Treating small bubbles as biased sinks for interstitial absorption can significantly increase the ratio of biased to unbiased sink strengths (Q) and results in maximized cavity swelling for a Q ratio close to one.

View Accepted Manuscript (DOE)

Cite

Export

Save

Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Fusion Energy Sciences (FES); Euratom Research and Training Program; State of Tennessee; Tennessee Higher Education Commission (THEC)

Grant/Contract Number:: AC05-00OR22725; SC0006661; 633053

OSTI ID:: 1876306

Journal Information:: Journal of Nuclear Materials, Vol. 569, Issue n/a; ISSN 0022-3115

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

References (55)

Materials challenges in nuclear energy Zinkle, S. J.; Was, G. S. Acta Materialia, Vol. 61, Issue 3 https://doi.org/10.1016/j.actamat.2012.11.004	journal	February 2013
On the origin of primary ½ a0 <111> and a0 <100> loops in irradiated Fe(Cr) alloys Schäublin, R.; Décamps, B.; Prokhodtseva, A. Acta Materialia, Vol. 133 https://doi.org/10.1016/j.actamat.2017.02.041	journal	July 2017
Fissile core and Tritium-Breeding Blanket: structural materials and their requirements Boutard, Jean-Louis; Alamo, Ana; Lindau, Rainer Comptes Rendus Physique, Vol. 9, Issue 3-4 https://doi.org/10.1016/j.crhy.2007.11.004	journal	April 2008
Atomic Configuration of Point Defect Clusters in Ion-Irradiated Silicon Carbide Lin, Y. R.; Chen, L. G.; Hsieh, C. Y. Scientific Reports, Vol. 7, Issue 1 https://doi.org/10.1038/s41598-017-15037-w	journal	November 2017
The influence of helium on cavity evolution in ion-irradiated T91 Monterrosa, Anthony M.; Jiao, Zhijie; Was, Gary S. Journal of Nuclear Materials, Vol. 509 https://doi.org/10.1016/j.jnucmat.2018.06.033	journal	October 2018
Effects of carbonitrides and carbides on microstructure and properties of castable nanostructured alloys Tan, L.; Graening, T.; Hu, X. Journal of Nuclear Materials, Vol. 540 https://doi.org/10.1016/j.jnucmat.2020.152376	journal	November 2020
Temperature-dependent cavity swelling in dual-ion irradiated Fe and Fe-Cr ferritic alloys Lin, Yan-Ru; Bhattacharya, Arunodaya; Chen, Da Acta Materialia, Vol. 207 https://doi.org/10.1016/j.actamat.2021.116660	journal	April 2021
Critical radius for bias-driven swelling — a further analysis and its application to bimodal cavity size distributions Hishinuma, A.; Mansur, L. K. Journal of Nuclear Materials, Vol. 118, Issue 1 https://doi.org/10.1016/0022-3115(83)90184-8	journal	August 1983
Experimental effects of helium on cavity formation during irradiation—a review Farrell, K. Radiation Effects, Vol. 53, Issue 3-4 https://doi.org/10.1080/00337578008207114	journal	January 1980
Helium and point defect accumulation: (i) microstructure and mechanical behaviour Schäublin, Robin; Henry, Jean; Dai, Yong Comptes Rendus Physique, Vol. 9, Issue 3-4 https://doi.org/10.1016/j.crhy.2008.01.003	journal	April 2008
Mechanisms of helium interaction with radiation effects in metals and alloys: A review Mansur, L. K.; Coghlan, W. A. Journal of Nuclear Materials, Vol. 119, Issue 1 https://doi.org/10.1016/0022-3115(83)90047-8	journal	November 1983
An integrated model for materials in a fusion power plant: transmutation, gas production, and helium embrittlement under neutron irradiation Gilbert, M. R.; Dudarev, S. L.; Zheng, S. Nuclear Fusion, Vol. 52, Issue 8 https://doi.org/10.1088/0029-5515/52/8/083019	journal	August 2012
Embrittlement of reduced-activation ferritic/martensitic steels irradiated in HFIR at 300°C and 400°C Klueh, R. L.; Sokolov, M. A.; Shiba, K. Journal of Nuclear Materials, Vol. 283-287 https://doi.org/10.1016/S0022-3115(00)00086-6	journal	December 2000
Helium causing disappearance of a/2<111> dislocation loops in binary Fe-Cr ferritic alloys Bhattacharya, Arunodaya; Henry, Jean; Décamps, Brigitte Journal of Nuclear Materials, Vol. 556 https://doi.org/10.1016/j.jnucmat.2021.153213	journal	December 2021
Microstructural evolution in dual-ion irradiated 316ss under various helium injection schedules Kohyama, Akira; Ayrault, Guy; Igata, Naohiro Journal of Nuclear Materials, Vol. 122, Issue 1-3 https://doi.org/10.1016/0022-3115(84)90600-7	journal	May 1984
Unified theoretical analysis of experimental swelling data for irradiated austenitic and ferritic/martensitic alloys Lee, E. H.; Mansur, L. K. Metallurgical Transactions A, Vol. 21, Issue 4 https://doi.org/10.1007/BF02656524	journal	April 1990
Simulation irradiation studies on iron Kuramoto, Eiichi; Yoshida, Naoaki; Tsukuda, Noboru Journal of Nuclear Materials, Vol. 104 https://doi.org/10.1016/0022-3115(82)90746-2	journal	January 1981
Development of next generation tempered and ODS reduced activation ferritic/martensitic steels for fusion energy applications Zinkle, S. J.; Boutard, J. L.; Hoelzer, D. T. Nuclear Fusion, Vol. 57, Issue 9 https://doi.org/10.1088/1741-4326/57/9/092005	journal	June 2017
Neutronics aspects of the FESS-FNSF Davis, A.; Harb, M.; El-Guebaly, L. Fusion Engineering and Design, Vol. 135 https://doi.org/10.1016/j.fusengdes.2017.06.008	journal	October 2018
Void Swelling in Metals and Alloys Under Irradiation: An Assessment of the Theory Mansur, L. K. Nuclear Technology, Vol. 40, Issue 1 https://doi.org/10.13182/NT78-2	journal	August 1978
Formulation of voids and bubbles as biased sinks to crystalline point defects Luo, Jing; Xin, Yong; Sun, Zhipeng Scripta Materialia, Vol. 197 https://doi.org/10.1016/j.scriptamat.2021.113806	journal	May 2021
He and Cr effects on radiation damage formation in ion-irradiated pure iron and Fe–5.40wt.% Cr: A transmission electron microscopy study Brimbal, Daniel; Meslin, Estelle; Henry, Jean Acta Materialia, Vol. 61, Issue 13 https://doi.org/10.1016/j.actamat.2013.04.070	journal	August 2013
Dislocation loops in ultra-high purity Fe(Cr) alloys after 7.2 MeV proton irradiation Chen, J.; Duval, F.; Jung, P. Journal of Nuclear Materials, Vol. 503 https://doi.org/10.1016/j.jnucmat.2018.02.042	journal	May 2018
The effect of radiation upon diffusion in metals Sizmann, Rudolf Journal of Nuclear Materials, Vol. 69-70 https://doi.org/10.1016/0022-3115(78)90256-8	journal	February 1978
Analytical solutions for helium bubble and critical radius parameters using a hard sphere equation of state Stoller, R. E.; Odette, G. R. Journal of Nuclear Materials, Vol. 131, Issue 2-3 https://doi.org/10.1016/0022-3115(85)90450-7	journal	April 1985
Understanding bubble and void nucleation in dual ion irradiated T91 steel using single parameter experiments Taller, Stephen; Was, Gary S. Acta Materialia, Vol. 198 https://doi.org/10.1016/j.actamat.2020.07.060	journal	October 2020
On the status and prospects for nanostructured ferritic alloys for nuclear fission and fusion application with emphasis on the underlying science Odette, G. Robert Scripta Materialia, Vol. 143 https://doi.org/10.1016/j.scriptamat.2017.06.021	journal	January 2018
The Role of Co-injected Helium on Swelling and Cavity Evolution at High Damage Levels in Ferritic-Martensitic Steels Woodley, D.; Taller, S.; Jiao, Z. Journal of Nuclear Materials, Vol. 550 https://doi.org/10.1016/j.jnucmat.2021.152912	journal	July 2021
14 MeV nickel-ion irradiated HT-9 ferritic steel with and without helium pre-implantation Kai, J. J.; Kulcinski, G. L. Journal of Nuclear Materials, Vol. 175, Issue 3 https://doi.org/10.1016/0022-3115(90)90211-5	journal	December 1990
55Fe effect on enhancing ferritic steel He/dpa ratio in fission reactor irradiations to simulate fusion conditions Liu, Haibo; Abdou, Mohamed A.; Greenwood, Larry R. Fusion Engineering and Design, Vol. 88, Issue 11 https://doi.org/10.1016/j.fusengdes.2013.05.067	journal	November 2013
Molecular statics calculations of the biases and point defect capture volumes of small cavities Kohnert, Aaron A.; Cusentino, Mary Alice; Wirth, Brian D. Journal of Nuclear Materials, Vol. 499 https://doi.org/10.1016/j.jnucmat.2017.12.005	journal	February 2018
Atomic configuration of irradiation-induced planar defects in 3C-SiC Lin, Y. R.; Ho, C. Y.; Hsieh, C. Y. Applied Physics Letters, Vol. 104, Issue 12 https://doi.org/10.1063/1.4869829	journal	March 2014
Impact of He and Cr on defect accumulation in ion-irradiated ultrahigh-purity Fe(Cr) alloys Prokhodtseva, A.; Décamps, B.; Ramar, A. Acta Materialia, Vol. 61, Issue 18 https://doi.org/10.1016/j.actamat.2013.08.007	journal	October 2013
Recent Progress in Developing and Qualifying Nanostructured Ferritic Alloys for Advanced Fission and Fusion Applications Odette, G. R. JOM, Vol. 66, Issue 12 https://doi.org/10.1007/s11837-014-1207-5	journal	November 2014
A dual ion irradiation study of helium–dpa interactions on cavity evolution in tempered martensitic steels and nanostructured ferritic alloys Yamamoto, Takuya; Wu, Yuan; Robert Odette, G. Journal of Nuclear Materials, Vol. 449, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2014.01.040	journal	June 2014
Radiation and helium effects on microstructures, nano-indentation properties and deformation behavior in ferrous alloys Katoh, Y.; Ando, M.; Kohyama, A. Journal of Nuclear Materials, Vol. 323, Issue 2-3 https://doi.org/10.1016/j.jnucmat.2003.08.007	journal	December 2003
Dramatic reduction of void swelling by helium in ion-irradiated high purity α -iron Bhattacharya, Arunodaya; Meslin, Estelle; Henry, Jean Materials Research Letters, Vol. 6, Issue 7 https://doi.org/10.1080/21663831.2018.1462266	journal	April 2018
Helium accumulation in metals during irradiation – where do we stand? Trinkaus, H.; Singh, B. N. Journal of Nuclear Materials, Vol. 323, Issue 2-3 https://doi.org/10.1016/j.jnucmat.2003.09.001	journal	December 2003
On the potentiality of using ferritic/martensitic steels as structural materials for fusion reactors Baluc, N.; Schäublin, R.; Spätig, P. Nuclear Fusion, Vol. 44, Issue 1 https://doi.org/10.1088/0029-5515/44/1/006	journal	December 2003
Single- and dual-beam in situ irradiations of high-purity iron in a transmission electron microscope: Effects of heavy ion irradiation and helium injection Brimbal, Daniel; Décamps, Brigitte; Henry, Jean Acta Materialia, Vol. 64 https://doi.org/10.1016/j.actamat.2013.10.052	journal	February 2014
Simulation of first wall damage: Effects of the method of gas implantation Packan, N. H.; Farrell, K. Journal of Nuclear Materials, Vol. 85-86 https://doi.org/10.1016/0022-3115(79)90338-6	journal	December 1979
Multiscale modelling of defect kinetics in irradiated iron Fu, Chu-Chun; Torre, Jacques Dalla; Willaime, François Nature Materials, Vol. 4, Issue 1 https://doi.org/10.1038/nmat1286	journal	December 2004
Cavity growth mechanism maps Goodhew, P. J. Scripta Metallurgica, Vol. 18, Issue 10 https://doi.org/10.1016/0036-9748(84)90180-7	journal	October 1984
Predicting structural material degradation in advanced nuclear reactors with ion irradiation Taller, Stephen; VanCoevering, Gerrit; Wirth, Brian D. Scientific Reports, Vol. 11, Issue 1 https://doi.org/10.1038/s41598-021-82512-w	journal	February 2021
Effect of pre-implanted helium on void swelling evolution in self-ion irradiated HT9 Getto, E.; Jiao, Z.; Monterrosa, A. M. Journal of Nuclear Materials, Vol. 462 https://doi.org/10.1016/j.jnucmat.2015.01.045	journal	July 2015
II. Effect of oxygen and helium on void formation in metals Zinkle, S. J.; Wolfer, W. G.; Kulcinski, G. L. Philosophical Magazine A, Vol. 55, Issue 1 https://doi.org/10.1080/01418618708209804	journal	January 1987
Dynamic observation of dual-beam irradiated Fe and Fe-10Cr alloys at 435 °C Lin, Yan-Ru; Chen, Wei-Ying; Li, Meimei Acta Materialia, Vol. 209 https://doi.org/10.1016/j.actamat.2021.116793	journal	May 2021
The effect of stress on the microstructure of neutron irradiated cold worked type 316 stainless steel Brager, H. R.; Gilbert, E. R.; Straalsund, J. L. Radiation Effects, Vol. 21, Issue 1 https://doi.org/10.1080/10420157408230810	journal	January 1974
Bubble formation in helium-implanted nanostructured ferritic alloys at elevated temperatures Lin, Yan-Ru; Chen, Wei-Ying; Tan, Lizhen Acta Materialia, Vol. 217 https://doi.org/10.1016/j.actamat.2021.117165	journal	September 2021
Comparison between bulk and thin foil ion irradiation of ultra high purity Fe Prokhodtseva, A.; Décamps, B.; Schäublin, R. Journal of Nuclear Materials, Vol. 442, Issue 1-3 https://doi.org/10.1016/j.jnucmat.2013.04.032	journal	November 2013
Materials for future nuclear energy systems Was, G. S.; Petti, D.; Ukai, S. Journal of Nuclear Materials, Vol. 527 https://doi.org/10.1016/j.jnucmat.2019.151837	journal	December 2019
Designing Radiation Resistance in Materials for Fusion Energy Zinkle, S. J.; Snead, L. L. Annual Review of Materials Research, Vol. 44, Issue 1 https://doi.org/10.1146/annurev-matsci-070813-113627	journal	July 2014
Radiation tolerance of neutron-irradiated model Fe–Cr–Al alloys Field, Kevin G.; Hu, Xunxiang; Littrell, Kenneth C. Journal of Nuclear Materials, Vol. 465 https://doi.org/10.1016/j.jnucmat.2015.06.023	journal	October 2015
Effect of saddle point anisotropy of point defects on their absorption by dislocations and cavities Carpentier, D.; Jourdan, T.; Le Bouar, Y. Acta Materialia, Vol. 136 https://doi.org/10.1016/j.actamat.2017.07.013	journal	September 2017
On the use of SRIM for calculating vacancy production: Quick calculation and full-cascade options Agarwal, S.; Lin, Y.; Li, C. Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms, Vol. 503 https://doi.org/10.1016/j.nimb.2021.06.018	journal	September 2021

Similar Records

Temperature-dependent cavity swelling in dual-ion irradiated Fe and Fe-Cr ferritic alloys

Journal Article · Tue Jan 19 00:00:00 EST 2021 · Acta Materialia · OSTI ID:1876306

Lin, Yan-Ru; Bhattacharya, Arunodaya; Chen, Da; +3 more

The role of Cr concentration and temperature on cavity swelling with co-injected helium in dual-ion irradiated Fe and Fe-Cr alloys

Journal Article · Tue Sep 13 00:00:00 EDT 2022 · Materials & Design · OSTI ID:1876306

Lin, Yan-Ru; Bhattacharya, Arunodaya; Chen, Da; +4 more

Dynamic observation of dual-beam irradiated Fe and Fe-10Cr alloys at 435 °C

Journal Article · Sat May 01 00:00:00 EDT 2021 · Acta Materialia · OSTI ID:1876306

Lin, Yan-Ru; Chen, Wei-Ying; Li, Meimei; +2 more

Related Subjects

36 MATERIALS SCIENCE
helium effects
radiation damage
ferritic alloy
cavity swelling
transmission electron microscopy

Title: The effect of helium on cavity swelling in dual-ion irradiated Fe and Fe-10Cr ferritic alloys

Citation Formats

References (55)

Similar Records

Related Subjects