Enhanced crevice corrosion of stainless steel 316 by degradation of Cr-containing hollandite crevice former

Guo, Xiaolei; Lei, Penghui; Mohanty, Chandi; Yao, Tiankai; Lian, Jie; Frankel, Gerald S.

doi:10.1016/j.corsci.2022.110462

Enhanced crevice corrosion of stainless steel 316 by degradation of Cr-containing hollandite crevice former

Journal Article · Sat Jun 25 00:00:00 EDT 2022 · Corrosion Science

DOI:https://doi.org/10.1016/j.corsci.2022.110462· OSTI ID:1881004

Guo, Xiaolei ^[1]; Lei, Penghui ^[2]; Mohanty, Chandi ^[3]; Yao, Tiankai ^[2]; Lian, Jie ^[2]; Frankel, Gerald S. ^[3]

The Ohio State Univ., Columbus, OH (United States); The Ohio State University
Rensselaer Polytechnic Inst., Troy, NY (United States)
The Ohio State Univ., Columbus, OH (United States)

This study explores the corrosion interactions between stainless steel 316 (SS316), a candidate nuclear waste canister material, and Cr-containing hollandite (Ba_1.15Cr_2.3Ti_5.7O₁₆), a model ceramic nuclear waste form. The two materials were corroded in close proximity in 0.6 M NaCl solution at 90 °C for 28 days. Severe crevice corrosion was observed on the stainless steel surface after the corrosion experiment, which is likely associated with the rapid accumulation of Cr³⁺ cations originating from both SS316 and the Cr-containing hollandite. Furthermore, the enhanced corrosion of SS316 by the corrosion products of hollandite is quantitatively explained using a classical crevice corrosion model.

View Accepted Manuscript (DOE)

Research Organization:: The Ohio State Univ., Columbus, OH (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: SC0016584

OSTI ID:: 1881004

Alternate ID(s):: OSTI ID: 1875747

Journal Information:: Corrosion Science, Journal Name: Corrosion Science Vol. 205; ISSN 0010-938X

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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36 MATERIALS SCIENCE
Corrosion interaction
Crevice corrosion
High level waste
Hollandite
Nuclear waste form
Stainless steel

Enhanced crevice corrosion of stainless steel 316 by degradation of Cr-containing hollandite crevice former

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