Role of chemical disorder on radiation-induced defect production and damage evolution in NiFeCoCr

Zhou, Yufan; Velişa, Gihan; San, Saro; Crespillo, Miguel L.; Fan, Zhe; Bei, Hongbin; Weber, William J.; Xiu, Pengyuan; Wang, Lumin; Tuomisto, Filip; Ching, Wai-Yim; Zhang, Yanwen

doi:10.1016/j.jnucmat.2022.153689

Title: Role of chemical disorder on radiation-induced defect production and damage evolution in NiFeCoCr

Journal Article · Fri Jul 01 00:00:00 EDT 2022 · Journal of Nuclear Materials

DOI:https://doi.org/10.1016/j.jnucmat.2022.153689· OSTI ID:1875335

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Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Horia Hulubei National Institute for Physics and Nuclear Engineering, Magurele (Romania)
Univ. of Missouri, Kansas City, MO (United States)
Univ. of Tennessee, Knoxville, TN (United States)
Zhejiang Univ., Hangzhou (China)
Univ. of Michigan, Ann Arbor, MI (United States)
Univ. of Helsinki (Finland). Helsinki Institute of Physics and Department of Physics
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)

Understanding chemical disorder in many concentrated solid solution alloys (CSAs) at the levels of electrons and atoms has attracted increasing attention as a path forward to reveal and identify underlying mechanisms for extraordinary mechanical properties and improved radiation tolerance. Single-phase NiFeCoCr CSA is a common base for many high-entropy alloys (HEAs) that have shown improved mechanical strength and radiation tolerance. In this study, defect production and damage evolution in NiFeCoCr under ion irradiation at room temperature to dose over 20 dpa are determined using ion channeling technique along both <100> and <110> directions utilizing multiple probing beam energies. The results obtained from the multi-axial and multi-energy channeling analysis are compared with those previously obtained for Ni crystals irradiated under similar conditions. The influence of chemical complexity on defect production and clustering at early-stage under room temperature irradiation up to dose of 1 dpa is discussed based on positron annihilation spectroscopy results. Defect structure evaluation in Ni and NiFeCoCr is also discussed based on transmission electron microscopy results over a prolonged irradiation at both room and elevated temperatures. Compared with chemically complex NiFeCoCr, larger dislocation loops thus less lattice strain are expected to form in pure Ni. Moreover, the role of chemical disorder in this CSA is also investigated based on ab initio calculations using large supercells. Finally, to understand the impact of chemical complexity effect on defect structure evolution, this integrated research effort attempts to link the relatively large charge redistribution due to difference in valence electron counts resulting from alloying different 3d transition metal elements, moderate lattice distortion arising from similar adaptable atomic size, and notable suppressed or delayed damage evolution in NiFeCoCr.

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Research Organization:: Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC05-00OR22725

OSTI ID:: 1875335

Alternate ID(s):: OSTI ID: 1862712

Journal Information:: Journal of Nuclear Materials, Vol. 565, Issue N/A; ISSN 0022-3115

Publisher:: ElsevierCopyright Statement

Country of Publication:: United States

Language:: English

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