Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite

Biesner, Tobias; Roh, Seulki; Pustogow, Andrej; Zheng, Hong; Mitchell, J. F.; Dressel, Martin

doi:10.1103/physrevb.105.l060410

Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite

Journal Article · Fri Feb 25 00:00:00 EST 2022 · Physical Review. B

DOI:https://doi.org/10.1103/physrevb.105.l060410· OSTI ID:1868999

^[1]; ^[1]; ^[2]; Zheng, Hong ^[3]; ^[3]; Dressel, Martin ^[1]

Univ. Stuttgart (Germany)
TU Wien, Vienna (Austria)
Argonne National Lab. (ANL), Argonne, IL (United States)

Time-domain magneto-THz spectroscopy is utilized to study the frustrated magnet averievite Cu_5–xZn_xV₂O₁₀(CsCl). Pronounced THz resonances are observed in unsubstituted samples (x = 0) when cooling below the onset of short-range magnetic correlations. The influence of external magnetic effects confirms the magnetic origin of these resonances. Increasing Zn substitution suppresses the resonances, as frustration effects dominate, reflecting the nonmagnetic phases for x > 0.25 compounds. The temperature evolution of the THz spectra is complemented with electron spin resonance spectroscopy. This comparison allows a direct probe of the different contributions from magnetic order, frustration, and structural properties in the phase diagram of averievite. Furthermore, our results illustrate the effect of magnetic interactions in THz spectra of frustrated magnets.

View Accepted Manuscript (DOE)

Research Organization:: Argonne National Laboratory (ANL), Argonne, IL (United States)

Sponsoring Organization:: Deutsche Forschungsgemeinschaft (DFG); USDOE Office of Science (SC), Basic Energy Sciences (BES). Materials Sciences & Engineering Division

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1868999

Journal Information:: Physical Review. B, Journal Name: Physical Review. B Journal Issue: 6 Vol. 105; ISSN 2469-9950

Publisher:: American Physical Society (APS)Copyright Statement

Country of Publication:: United States

Language:: English

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Magnetic terahertz resonances above the Néel temperature in the frustrated kagome antiferromagnet averievite

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