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The influence of hydrostatic pressure and annealing conditions on the magnetostructural transitions in MnCoGe

Journal Article · · Journal of Applied Physics
DOI:https://doi.org/10.1063/5.0053671· OSTI ID:1868094
 [1];  [2];  [3];  [4];  [2];  [5];  [5];  [5];  [2]
  1. Louisiana State Univ., Baton Rouge, LA (United States); Louisiana State University
  2. Louisiana State Univ., Baton Rouge, LA (United States)
  3. National Synchrotron Radiation Research Center, Hsinchu (Taiwan)
  4. Ming Chi University of Technology, New Taipei City (Taiwan)
  5. Southern Illinois Univ., Carbondale, IL (United States)

In this work, the phase transitions of stoichiometric MnCoGe alloys were studied by systematically varying the annealing conditions and applying hydrostatic pressure. First-order martensitic structural transitions from the Ni2In-type hexagonal austenite phase to the TiNiSi-type orthorhombic martensite phase spanned a wide temperature window (>200 K) as a result of quenching the samples at temperatures ranging from the solid phase at 700 °C to the liquid phase at 1150 °C. Despite the large variation in their structural transition temperatures, the changes in cell parameters across the structural transitions and the Curie–Weiss temperatures of the martensite/austenite phase were relatively small. For the sample quenched from 800 °C, coupled magnetostructural transitions were observed, and the largest maximum magnetic entropy change was found to be -ΔSmax = 33:6 J/kg K for a 7-T field change. The coupled magnetostructural transitions and the corresponding magnetic entropy enhancements were found to also be achievable by applying hydrostatic pressures. Meanwhile, as the quenching temperatures or hydrostatic pressures increased, the first-order martensitic structural transition shifted toward lower temperature until it was ultimately absent, in which case only the crystal structure and magnetic transition of the Ni2In-type hexagonal austenite phase were present.

Research Organization:
Louisiana State Univ., Baton Rouge, LA (United States); Southern Illinois Univ., Carbondale, IL (United States)
Sponsoring Organization:
USDOE Office of Science (SC), Basic Energy Sciences (BES); National Science Foundation (NSF); Ministry of Science and Technology of Taiwan (MOST)
Grant/Contract Number:
SC0010521; FG02-06ER46291; SC0010521
OSTI ID:
1868094
Alternate ID(s):
OSTI ID: 1872460
OSTI ID: 1786836
Journal Information:
Journal of Applied Physics, Journal Name: Journal of Applied Physics Journal Issue: 21 Vol. 129; ISSN 0021-8979
Publisher:
American Institute of Physics (AIP)Copyright Statement
Country of Publication:
United States
Language:
English

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