Influence of chemical disorder on energy dissipation and defect evolution in advanced alloys

Zhang, Yanwen; Jin, Ke; Xue, Haizhou; Lu, Chenyang; Olsen, Raina J.; Beland, Laurent K.; Ullah, Mohammad W.; Zhao, Shijun; Bei, Hongbin; Aidhy, Dilpuneet S.; Samolyuk, German D.; Wang, Lumin; Caro, Magdalena; Caro, Alfredo; Stocks, G. Malcolm; Larson, Ben C.; Robertson, Ian M.; Correa, Alfredo A.; Weber, William J.

doi:10.1557/jmr.2016.269

Title: Influence of chemical disorder on energy dissipation and defect evolution in advanced alloys

Journal Article · Fri Aug 26 00:00:00 EDT 2016 · Journal of Materials Research

DOI:https://doi.org/10.1557/jmr.2016.269· OSTI ID:1866534

Zhang, Yanwen ^[1]; Jin, Ke ^[1]; Xue, Haizhou ^[2]; Lu, Chenyang ^[3]; Olsen, Raina J. ^[1]; Beland, Laurent K. ^[1]; Ullah, Mohammad W. ^[1]; Zhao, Shijun ^[1]; Bei, Hongbin ^[1]; Aidhy, Dilpuneet S. ^[4]; Samolyuk, German D. ^[1]; Wang, Lumin ^[3]; Caro, Magdalena ^[5]; Caro, Alfredo ^[5]; Stocks, G. Malcolm ^[1]; Larson, Ben C. ^[1]; Robertson, Ian M. ^[6]; Correa, Alfredo A. ^[7]; Weber, William J. ^[8]

Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States)
Univ. of Tennessee, Knoxville, TN (United States)
Univ. of Michigan, Ann Arbor, MI (United States)
Univ. of Wyoming, Laramie, WY (United States)
Los Alamos National Lab. (LANL), Los Alamos, NM (United States)
Univ. of Wisconsin, Madison, WI (United States)
Lawrence Livermore National Lab. (LLNL), Livermore, CA (United States)
Oak Ridge National Lab. (ORNL), Oak Ridge, TN (United States); Univ. of Tennessee, Knoxville, TN (United States)

We report that historically, alloy development with better radiation performance has been focused on traditional alloys with one or two principal element(s) and minor alloying elements, where enhanced radiation resistance depends on microstructural or nanoscale features to mitigate displacement damage. In sharp contrast to traditional alloys, recent advances of single-phase concentrated solid solution alloys (SP-CSAs) have opened up new frontiers in materials research. In these alloys, a random arrangement of multiple elemental species on a crystalline lattice results in disordered local chemical environments and unique site-to-site lattice distortions. Based on closely integrated computational and experimental studies using a novel set of SP-CSAs in a face-centered cubic structure, we have explicitly demonstrated that increasing chemical disorder can lead to a substantial reduction in electron mean free paths, as well as electrical and thermal conductivity, which results in slower heat dissipation in SP-CSAs. The chemical disorder also has a significant impact on defect evolution under ion irradiation. Considerable improvement in radiation resistance is observed with increasing chemical disorder at electronic and atomic levels. Finally, the insights into defect dynamics may provide a basis for understanding elemental effects on evolution of radiation damage in irradiated materials and may inspire new design principles of radiation-tolerant structural alloys for advanced energy systems.

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Research Organization:: Lawrence Livermore National Laboratory (LLNL), Livermore, CA (United States); Oak Ridge National Laboratory (ORNL), Oak Ridge, TN (United States)

Sponsoring Organization:: USDOE National Nuclear Security Administration (NNSA); USDOE Office of Science (SC), Basic Energy Sciences (BES)

Grant/Contract Number:: AC52-07NA27344; AC05-00OR22725; AC02-05CH11231

OSTI ID:: 1866534

Alternate ID(s):: OSTI ID: 1319193

Report Number(s):: LLNL-JRNL-834139; 1031874; TRN: US2306056

Journal Information:: Journal of Materials Research, Vol. 31, Issue 16; ISSN 0884-2914

Publisher:: Materials Research SocietyCopyright Statement

Country of Publication:: United States

Language:: English

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Cited by: 87 works

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