Understanding the Single Atom Doping Effects in Oxygen Reduction with Atomically Precise Metal Nanoclusters

Li, Site; Nagarajan, Anantha Venkataraman; Zhao, Shuo; Mpourmpakis, Giannis; Jin, Rongchao

doi:10.1021/acs.jpcc.1c08356

Understanding the Single Atom Doping Effects in Oxygen Reduction with Atomically Precise Metal Nanoclusters

Journal Article · Mon Nov 08 00:00:00 EST 2021 · Journal of Physical Chemistry. C

DOI:https://doi.org/10.1021/acs.jpcc.1c08356· OSTI ID:1859207

Li, Site ^[1]; Nagarajan, Anantha Venkataraman ^[2]; Zhao, Shuo ^[1]; ^[2]; ^[1]

Department of Chemistry, Carnegie Mellon University, Pittsburgh, Pennsylvania 15213, United States
Department of Chemical Engineering, University of Pittsburgh, Pittsburgh, Pennsylvania 15261, United States

Not Available

View Journal Article

Sponsoring Organization:: USDOE

Grant/Contract Number:: FE0026825

OSTI ID:: 1859207

Alternate ID(s):: OSTI ID: 1978016

Journal Information:: Journal of Physical Chemistry. C, Journal Name: Journal of Physical Chemistry. C Journal Issue: 45 Vol. 125; ISSN 1932-7447

Publisher:: American Chemical SocietyCopyright Statement

Country of Publication:: United States

Language:: English

References (36)

Molecular and solid-state tests of density functional approximations: LSD, GGAs, and meta-GGAs Kurth, Stefan; Perdew, John P.; Blaha, Peter International Journal of Quantum Chemistry, Vol. 75, Issue 4-5 https://doi.org/10.1002/(SICI)1097-461X(1999)75:4/5<889::AID-QUA54>3.0.CO;2-8	journal	January 1999
Oxygen Reduction Reaction on Pt and Pt Bimetallic Surfaces: A Selective Review Marković, N. M.; Schmidt, T. J.; Stamenković, V. Fuel Cells, Vol. 1, Issue 2 https://doi.org/10.1002/1615-6854(200107)1:2<105::AID-FUCE105>3.0.CO;2-9	journal	July 2001
Pt‐Based Nanocrystal for Electrocatalytic Oxygen Reduction Zhao, Zipeng; Chen, Changli; Liu, Zeyan Advanced Materials, Vol. 31, Issue 31 https://doi.org/10.1002/adma.201808115	journal	December 2018
Heteroatom Effects on the Optical and Electrochemical Properties of Ag ₂₅ (SR) ₁₈ and Its Dopants Kang, Xi; Chen, Shuang; Jin, Shan ChemElectroChem, Vol. 3, Issue 8 https://doi.org/10.1002/celc.201600038	journal	March 2016
Elucidating the stability of ligand-protected Au nanoclusters under electrochemical reduction of CO2 Nagarajan, Anantha Venkataraman; Juarez-Mosqueda, Rosalba; Cowan, Michael J. SN Applied Sciences, Vol. 2, Issue 4 https://doi.org/10.1007/s42452-020-2488-7	journal	March 2020
A review of Fe–N/C and Co–N/C catalysts for the oxygen reduction reaction Bezerra, Cicero W.B.; Zhang, Lei; Lee, Kunchan Electrochimica Acta, Vol. 53, Issue 15, p. 4937-4951 https://doi.org/10.1016/j.electacta.2008.02.012	journal	June 2008
Enhanced oxygen reduction activity of PtCu nanoparticles by morphology tuning and transition-metal doping Wu, Dengfeng; Yang, Yang; Dai, Changqing International Journal of Hydrogen Energy, Vol. 45, Issue 7 https://doi.org/10.1016/j.ijhydene.2019.12.003	journal	February 2020
Molecular metal nanoclusters for ORR, HER and OER: Achievements, opportunities and challenges Qin, Dong-Dong; Tang, Yun; Ma, Guanyu International Journal of Hydrogen Energy, Vol. 46, Issue 51 https://doi.org/10.1016/j.ijhydene.2021.05.096	journal	July 2021
Electrochemistry of Atomically Precise Metal Nanoclusters Kwak, Kyuju; Lee, Dongil Accounts of Chemical Research, Vol. 52, Issue 1 https://doi.org/10.1021/acs.accounts.8b00379	journal	November 2018
Toward Active-Site Tailoring in Heterogeneous Catalysis by Atomically Precise Metal Nanoclusters with Crystallographic Structures Jin, Rongchao; Li, Gao; Sharma, Sachil Chemical Reviews https://doi.org/10.1021/acs.chemrev.0c00495	journal	September 2020
Atomically Precise Colloidal Metal Nanoclusters and Nanoparticles: Fundamentals and Opportunities Jin, Rongchao; Zeng, Chenjie; Zhou, Meng Chemical Reviews, Vol. 116, Issue 18 https://doi.org/10.1021/acs.chemrev.5b00703	journal	September 2016
Atomically Precise Noble Metal Nanoclusters as Efficient Catalysts: A Bridge between Structure and Properties Du, Yuanxin; Sheng, Hongting; Astruc, Didier Chemical Reviews, Vol. 120, Issue 2 https://doi.org/10.1021/acs.chemrev.8b00726	journal	March 2019
Rh-Doped Pt–Ni Octahedral Nanoparticles: Understanding the Correlation between Elemental Distribution, Oxygen Reduction Reaction, and Shape Stability Beermann, Vera; Gocyla, Martin; Willinger, Elena Nano Letters, Vol. 16, Issue 3 https://doi.org/10.1021/acs.nanolett.5b04636	journal	February 2016
Ga–Doped Pt–Ni Octahedral Nanoparticles as a Highly Active and Durable Electrocatalyst for Oxygen Reduction Reaction Lim, JeongHoon; Shin, Hyeyoung; Kim, MinJoong Nano Letters, Vol. 18, Issue 4 https://doi.org/10.1021/acs.nanolett.8b00028	journal	March 2018
Porous Carbon-Supported Gold Nanoparticles for Oxygen Reduction Reaction: Effects of Nanoparticle Size Wang, Likai; Tang, Zhenghua; Yan, Wei ACS Applied Materials & Interfaces, Vol. 8, Issue 32 https://doi.org/10.1021/acsami.6b02223	journal	August 2016
Monopalladium Substitution in Gold Nanoclusters Enhances CO ₂ Electroreduction Activity and Selectivity Li, Site; Alfonso, Dominic; Nagarajan, Anantha Venkataraman ACS Catalysis, Vol. 10, Issue 20 https://doi.org/10.1021/acscatal.0c02266	journal	September 2020
Oxygen Electrocatalysis by [Au ₂₅ (SR) ₁₈ ]: Charge, Doping, and Ligand Removal Effect Sun, Fang; Deng, Chaofang; Tian, Shufang ACS Catalysis, Vol. 11, Issue 13 https://doi.org/10.1021/acscatal.1c01030	journal	June 2021
Influence of Atomic-Level Morphology on Catalysis: The Case of Sphere and Rod-Like Gold Nanoclusters for CO ₂ Electroreduction Zhao, Shuo; Austin, Natalie; Li, Mo ACS Catalysis, Vol. 8, Issue 6 https://doi.org/10.1021/acscatal.8b00365	journal	April 2018
Factors Governing Oxygen Reduction in Solid Oxide Fuel Cell Cathodes ^† Adler, Stuart B. Chemical Reviews, Vol. 104, Issue 10 https://doi.org/10.1021/cr020724o	journal	October 2004
Thiolate Ligands as a Double-Edged Sword for CO Oxidation on CeO ₂ Supported Au ₂₅ (SCH ₂ CH ₂ Ph) ₁₈ Nanoclusters Wu, Zili; Jiang, De-en; Mann, Amanda K. P. Journal of the American Chemical Society, Vol. 136, Issue 16 https://doi.org/10.1021/ja5018706	journal	April 2014
[Ag ₂₅ (SR) ₁₈ ] ⁻ : The “Golden” Silver Nanoparticle Joshi, Chakra P.; Bootharaju, Megalamane S.; Alhilaly, Mohammad J. Journal of the American Chemical Society, Vol. 137, Issue 36 https://doi.org/10.1021/jacs.5b07088	journal	September 2015
Total Structure and Electronic Structure Analysis of Doped Thiolated Silver [MAg ₂₄ (SR) ₁₈ ] ^2– (M = Pd, Pt) Clusters Yan, Juanzhu; Su, Haifeng; Yang, Huayan Journal of the American Chemical Society, Vol. 137, Issue 37 https://doi.org/10.1021/jacs.5b07186	journal	September 2015
Sharp Transition from Nonmetallic Au ₂₄₆ to Metallic Au ₂₇₉ with Nascent Surface Plasmon Resonance Higaki, Tatsuya; Zhou, Meng; Lambright, Kelly J. Journal of the American Chemical Society, Vol. 140, Issue 17 https://doi.org/10.1021/jacs.8b02487	journal	April 2018
Origin of the Overpotential for Oxygen Reduction at a Fuel-Cell Cathode Nørskov, J. K.; Rossmeisl, J.; Logadottir, A. The Journal of Physical Chemistry B, Vol. 108, Issue 46 https://doi.org/10.1021/jp047349j	journal	November 2004
Multiscale Modeling Reveals Poisoning Mechanisms of MgO-Supported Au Clusters in CO Oxidation Stamatakis, Michail; Christiansen, Matthew A.; Vlachos, Dionisios G. Nano Letters, Vol. 12, Issue 7 https://doi.org/10.1021/nl301318b	journal	June 2012
Quantum sized, thiolate-protected gold nanoclusters Jin, Rongchao Nanoscale, Vol. 2, Issue 3 https://doi.org/10.1039/B9NR00160C	journal	January 2010
Charge state-dependent catalytic activity of [Au ₂₅ (SC ₁₂ H ₂₅ ) ₁₈ ] nanoclusters for the two-electron reduction of dioxygen to hydrogen peroxide Lu, Yizhong; Jiang, Yuanyuan; Gao, Xiaohui Chem. Commun., Vol. 50, Issue 62 https://doi.org/10.1039/C4CC01841A	journal	January 2014
Oxygen reduction catalyzed by gold nanoclusters supported on carbon nanosheets Wang, Qiannan; Wang, Likai; Tang, Zhenghua Nanoscale, Vol. 8, Issue 12 https://doi.org/10.1039/C6NR00400H	journal	January 2016
Elucidating the active sites for CO ₂ electroreduction on ligand-protected Au ₂₅ nanoclusters Austin, Natalie; Zhao, Shuo; McKone, James R. Catalysis Science & Technology, Vol. 8, Issue 15 https://doi.org/10.1039/C8CY01099D	journal	January 2018
Monodisperse nanoparticles for catalysis and nanomedicine Muzzio, Michelle; Li, Junrui; Yin, Zhouyang Nanoscale, Vol. 11, Issue 41 https://doi.org/10.1039/C9NR06080D	journal	January 2019
Sub-nanometre sized metal clusters: from synthetic challenges to the unique property discoveries Lu, Yizhong; Chen, Wei Chemical Society Reviews, Vol. 41, Issue 9 https://doi.org/10.1039/c2cs15325d	journal	January 2012
Active sites of ligand-protected Au ₂₅ nanoparticle catalysts for CO ₂ electroreduction to CO Alfonso, Dominic R.; Kauffman, Douglas; Matranga, Christopher The Journal of Chemical Physics, Vol. 144, Issue 18 https://doi.org/10.1063/1.4948792	journal	May 2016
A full understanding of oxygen reduction reaction mechanism on Au(1 1 1) surface Yang, Yang; Dai, Changqing; Fisher, Adrian Journal of Physics: Condensed Matter, Vol. 29, Issue 36 https://doi.org/10.1088/1361-648X/aa7db6	journal	August 2017
The density functional formalism, its applications and prospects Jones, R. O.; Gunnarsson, O. Reviews of Modern Physics, Vol. 61, Issue 3 https://doi.org/10.1103/RevModPhys.61.689	journal	July 1989
High-performance transition metal-doped Pt3Ni octahedra for oxygen reduction reaction Huang, X.; Zhao, Z.; Cao, L. Science, Vol. 348, Issue 6240 https://doi.org/10.1126/science.aaa8765	journal	June 2015
Three-orders-of-magnitude variation of carrier lifetimes with crystal phase of gold nanoclusters Zhou, Meng; Higaki, Tatsuya; Hu, Guoxiang Science, Vol. 364, Issue 6437 https://doi.org/10.1126/science.aaw8007	journal	April 2019

Similar Records

Understanding the Single Atom Doping Effects in Oxygen Reduction with Atomically Precise Metal Nanoclusters

Journal Article · Sun Nov 07 23:00:00 EST 2021 · Journal of Physical Chemistry. C · OSTI ID:1978016

Metallic Hydrogen in Atomically Precise Gold Nanoclusters

Journal Article · Wed May 17 00:00:00 EDT 2017 · Chemistry of Materials · OSTI ID:1479679

Single-Atomic Ruthenium Catalytic Sites on Nitrogen-Doped Graphene for Oxygen Reduction Reaction in Acidic Medium

Journal Article · Tue Jun 27 20:00:00 EDT 2017 · ACS Nano · OSTI ID:1414051

Understanding the Single Atom Doping Effects in Oxygen Reduction with Atomically Precise Metal Nanoclusters

Citation Formats

References (36)

Similar Records

Related Subjects