Efficient light-emitting diodes based on oriented perovskite nanoplatelets

Cui, Jieyuan; Liu, Yang; Deng, Yunzhou; Lin, Chen; Fang, Zhishan; Xiang, Chensheng; Bai, Peng; Du, Kai; Zuo, Xiaobing; Wen, Kaichuan; Gong, Shaolong; He, Haiping; Ye, Zhizhen; Gao, Yunan; Tian, He; Zhao, Baodan; Wang, Jianpu; Jin, Yizheng

doi:10.1126/sciadv.abg8458

Title: Efficient light-emitting diodes based on oriented perovskite nanoplatelets

Journal Article · Fri Oct 08 00:00:00 EDT 2021 · Science Advances

DOI:https://doi.org/10.1126/sciadv.abg8458· OSTI ID:1854138

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Zhejiang Univ., Hangzhou (China)
Peking Univ., Beijing (China)
Argonne National Lab. (ANL), Argonne, IL (United States)
Nanjing Tech Univ. (China)
Wuhan Univ. (China)
Zhejiang Univ., Hangzhou (China); Zhejiang Univ., Wenzhou (China)

Solution-processed planar perovskite light-emitting diodes (LEDs) promise high-performance and cost-effective electroluminescent devices ideal for large-area display and lighting applications. Exploiting emission layers with high ratios of horizontal transition dipole moments (TDMs) is expected to boost the photon outcoupling of planar LEDs. However, LEDs based on anisotropic perovskite nanoemitters remain to be inefficient (external quantum efficiency, EQE <5%) due to the difficulties of simultaneously controlling the orientations of TDMs, achieving high photoluminescence quantum yields (PLQYs) and realizing charge balance in the films of assembled nanostructures. Here, we demonstrate efficient electroluminescence from an in situ grown perovskite film composed of a monolayer of face-on oriented nanoplatelets. The ratio of horizontal TDMs of the perovskite nanoplatelet film is ~84%, which leads to a light-outcoupling efficiency of ~31%, substantially higher than that of isotropic emitters (~23%). In consequence, LEDs with a peak EQE of 23.6% are achieved, representing highly efficient planar perovskite LEDs.

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Research Organization:: Argonne National Lab. (ANL), Argonne, IL (United States)

Sponsoring Organization:: USDOE Office of Science (SC); National Key Research and Development Program of China; National Natural Science Foundation of China (NSFC); Fundamental Research Funds for the Central Universities; Natural Science Foundation of Zhejiang Province

Grant/Contract Number:: AC02-06CH11357

OSTI ID:: 1854138

Journal Information:: Science Advances, Vol. 7, Issue 41; ISSN 2375-2548

Publisher:: AAASCopyright Statement

Country of Publication:: United States

Language:: English

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